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The angular dependence (x-ray linear dichroism) of the Cr K pre-edge in MgAl2O4:Cr3+ spinel is measured by means of x-ray absorption near edge structure spectroscopy (XANES) and compared to calculations based on density functional theory…

We solve the nonlinear Maxwell equations in an InP-based dielectric metamaterial, considering both two-photon absorption and photo-induced free-carrier absorption. We obtain the intensity-dependent reflection, absorption, and effective…

Optics · Physics 2018-01-10 Brian Slovick , Lucas Zipp , Srini Krishnamurthy

This paper introduces Spectral Incoherent Diffractive Imaging (SIDI) as a novel method for achieving dark-field imaging of nanostructures with heterogeneous oxidation states. With SIDI, shifts in photoemission profiles can be spatially…

Optics · Physics 2023-12-25 Tamme Wollweber , Kartik Ayyer

Ultrafast degenerate pump-probe experiments performed on a free standing film of double walled carbon nanotubes near the first metallic transition energy of outer tube show ultrafast ($97 fs$) photobleaching followed by a photo-induced…

Other Condensed Matter · Physics 2009-11-13 N. Kamaraju , Sunil Kumar , B. Karthikeyan , Alexander Moravsky , R. O. Loutfy , A. K. Sood

Cesium adsorption structures on Ag(111) were characterized in a low-temperature scanning tunneling microscopy experiment. At low coverages, atomic resolution of individual Cs atoms is occasionally suppressed in regions of an otherwise…

Materials Science · Physics 2009-11-13 M. Ziegler , J. Kroeger , R. Berndt , A. Filinov , M. Bonitz

We establish design principles for light-harvesting antennae whose energy capture scales superlinearly with system size. Controlling the absorber dipole orientations produces sets of `guide-slide' states which promote steady-state…

Quantum Physics · Physics 2019-10-16 William M. Brown , Erik M. Gauger

The integration of two-dimensional (2D) periodic nanopattern defined by nanoimprint lithography and dry etching into aluminum induced crystallization (AIC) based polycrystalline silicon (Poly-Si) thin film solar cells is investigated…

In-depth studies of exoplanetary atmospheres are starting to become reality. In order to unveil their properties in detail, we need spectra with a higher S/N and also more sophisticated analysis methods. With high-resolution spectrographs,…

Earth and Planetary Astrophysics · Physics 2018-10-03 Francesco Borsa , Andrea Zannoni

We have theoretically shown that optical properties of semiconductor nanorods are controlled by 1D excitons. The theory, which takes into account anisotropy of spacial and dielectric confinement, describes size dependence of interband…

Materials Science · Physics 2007-05-23 A. Shabaev , Al. L. Efros

Polarization dependence of the exciton-plasmon-photon conversion in silver nanowire-quantum dots structure was investigated using a scanning confocal microscope system. We found that the fluorescence enhancement of the CdSe nanocrystals was…

We aim to clarify the role that absorption plays in nonlinear optical processes in a variety of metallic nanostructures and show how it relates to emission and conversion efficiency. We define a figure of merit that establishes the…

Applying the novel exact-exchange (EXX) Kohn-Sham method within time-dependent density-functional theory, we obtained the optical absorption spectrum of bulk silicon in good agreement with experiments including excitonic features. Analysis…

Materials Science · Physics 2016-01-01 Yong-Hoon Kim , Andreas Goerling

Higher-order electronic transitions of all inorganic lead halide perovskite quantum dots (QDs) (CsPbX$_3$: X = Cl, Br, I) are hardly detected by traditional spectroscopic techniques due to the condensed electronic level of QDs. This work…

Materials Science · Physics 2023-11-22 Prasenjit Mandal , Ranjani Viswanatha

In semiconductors, exciton or charge carrier diffusivity is typically described as an inherent material property. Here, we show that the transport of excitons (i.e., bound electron-hole pairs) in CsPbBr3 perovskite nanocrystals (NCs)…

Composition-tunable ternary Cd1-xPbxS nanocrystals (NCs) are very important materials for remote sensing and detecting in the infrared (IR) wavelength region. They are, however, almost exclusively prepared by wet chemical routes which leads…

Mesoscale and Nanoscale Physics · Physics 2013-12-16 Guo-Long Tan , Li-Min Liu , Weibing Wu

Enhanced optical absorption of molecules in the vicinity of metallic nanostructures is key to a number of surface-enhanced spectroscopies and of great general interest to the fields of plasmonics and nano-optics. Yet, experimental access to…

We present an experimental study of Z-scan measurements of the nonlinear response of cold Cs atoms in a magneto-optical trap. Numerical simulations of the Z-scan signal accounting for the nonuniform atomic density agree with experimental…

Atomic Physics · Physics 2011-04-21 Yingxue Wang , M. Saffman

The characterization of a third order nonlinear integrated waveguide is reported for the first time by means of a top-hat Dispersive-Scan (D-Scan) technique, a temporal analog of the top-hat Z-Scan. With a single laser beam, and by carrying…

Optics · Physics 2017-10-11 Samuel Serna , Nicolas Dubreuil

Photoabsorption cross sections of small sodium cluster cations (Na$_n^+$, n=3,5,7 and 9) were calculated at various temperatures with the time-dependent local-density-approximation (TDLDA) in conjunction with ab initio molecular dynamics…

Atomic and Molecular Clusters · Physics 2016-09-08 M. Moseler , H. Hakkinen , Uzi Landman

UV-induced photodesorption of ice is a non-thermal evaporation process that can explain the presence of cold molecular gas in a range of interstellar regions. Information on the average UV photodesorption yield of astrophysically important…

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