Light-harvesting with guide-slide superabsorbing condensed-matter nanostructures
Abstract
We establish design principles for light-harvesting antennae whose energy capture scales superlinearly with system size. Controlling the absorber dipole orientations produces sets of `guide-slide' states which promote steady-state superabsorbing characteristics in noisy condensed-matter nanostructures. Inspired by natural photosynthetic complexes, we discuss the example of ring-like dipole arrangements and show that, in our setup, vibrational relaxation enhances rather than impedes performance. Remarkably, the superabsorption effect proves robust to O(5%) disorder simultaneously for all relevant system parameters, showing promise for experimental exploration across a broad range of platforms.
Cite
@article{arxiv.1803.08036,
title = {Light-harvesting with guide-slide superabsorbing condensed-matter nanostructures},
author = {William M. Brown and Erik M. Gauger},
journal= {arXiv preprint arXiv:1803.08036},
year = {2019}
}
Comments
Updated to include supporting results in the polaron frame for strong vibrational coupling