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Here we have performed detailed first principles calculations for the electronic structure and magnetic properties of Ba$_6$Cr$_2$S$_{10}$ to study the origin of the anti-ferromagnetic exchange interaction between spins on Cr ions for the…

Strongly Correlated Electrons · Physics 2023-08-16 Jianhua Zhu , Jianfeng Zhang , Yilin Zhang , Devashibhai Adroja , Huancheng Yang , Xiancheng Wang , Changqing Jin , Ji Chen , Wei Wu

We report a detailed examination the magnetic structure of anhydrous cupric chloride CuCl2 carried out by powder neutron diffraction, magnetic susceptibility and specific heat measurements on polycrystalline and single crystal samples as…

Strongly Correlated Electrons · Physics 2009-04-21 M. G. Banks , R. K. Kremer , C. Hoch , A. Simon , B. Ouladdiaf , J. -M. Broto , H. Rakoto , C. Lee , M. -H. Whangbo

We report the structural and magnetic properties of a new class of cobaltates with the chemical formula (BaSr)4-xLa2xCo4O15 (x = 0, 0.5 and 1). These compounds crystallize in a hexagonal structure in which cobalt ions are distributed among…

Strongly Correlated Electrons · Physics 2015-06-11 V. O. Garlea , R. Jin , E. Garlea , G. Ehlers , E. Mamontov , D. B. Myers , F. Xie , R. Custelcean

We report density functional studies of the Fe$_{1-x}$Cu$_x$Se alloy done using supercell and coherent potential approximation methods. Magnetic behavior was investigated using the disordered local moment approach. We find that Cu occurs in…

Superconductivity · Physics 2013-08-08 S. Chadov , D. Schärf , G. H. Fecher , C. Felser , L. Zhang , D. J. Singh

Inelastic neutron scattering experiments were performed for the spin-trimer compounds Ca3Cu3-xNix(PO4)4 (x=0,1,2) in order to study the dynamic magnetic properties. The observed excitations can be associated with transitions between the…

Other Condensed Matter · Physics 2009-11-13 A. Podlesnyak , V. Pomjakushin , E. Pomjakushina , K. Conder , A. Furrer

A heterostructure comprised of a 2.7 nm (7 unit-cell) thick layer of the metallic ferromagnet La(2/3)Ca(1/3)MnO(3) and two 50 nm thick layers of the high-temperature superconductor YBa(2)Cu(3)O(7) epitaxially grown on (100) SrTiO3 by…

Strongly Correlated Electrons · Physics 2015-05-14 Z. L. Zhang , U. Kaiser , S. Soltan , H. -U. Habermeier , B. Keimer

Periodic and cluster density-functional theory (DFT) calculations, including DFT+U and hybrid functionals, are applied to study magnetostructural correlations in spin-1/2 frustrated chain compounds CuX2: CuCl2, CuBr2, and a fictitious chain…

Strongly Correlated Electrons · Physics 2013-07-02 S. Lebernegg , M. Schmitt , A. A. Tsirlin , O. Janson , H. Rosner

High-field magnetization of the spin-$1/2$ antiferromagnet $\alpha$-Cu$_2$V$_2$O$_7$ was measured in pulsed magnetic fields of up to 56 T in order to study its magnetic phase diagram. When the field was applied along the easy axis (the…

Strongly Correlated Electrons · Physics 2017-06-21 G. Gitgeatpong , M. Suewattana , Shiwei Zhang , A. Miyake , P. Chanlert , N. Kurita , H. Tanaka , T. J. Sato , Y. Zhao , K. Matan

We have investigated for the first time the magnetic behaviour of an intermetallic compound, Dy4RhAl, crystallizing in Gd4RhIn type cubic structure containing 3 sites for rare-earth (R), by several bulk measurements down to 1.8 K. This work…

Strongly Correlated Electrons · Physics 2023-04-21 K. K. Iyer , S. Matteppanavar , S. Dodamani , K. Maiti , E. V. Sampathkumaran

We theoretically propose a family of $f$-electron based magnets that realizes Kitaev-type bond-dependent anisotropic interactions. Based on {\it ab initio} calculations, we show that $A_2$PrO$_3$ ($A$: alkali metals) crystalize in a…

Strongly Correlated Electrons · Physics 2020-11-03 Seong-Hoon Jang , Ryoya Sano , Yasuyuki Kato , Yukitoshi Motome

Ba$_2$Cu$_3$O$_4$Cl$_2$ has two inter-penetrating square Cu sublattices, one with square root 2 times the in-plane spacing of the other. Isotropic magnetic interactions between the two sublattices are completely frustrated. Quantum…

Strongly Correlated Electrons · Physics 2009-11-11 M. K. Ramazanoglu , P. S. Clegg , S. Wakimoto , R. J. Birgeneau , S. Noro

The Eu-based compound, EuCu2As2, crystallizing in the ThCr2Si2-type tetragonal structure, has been synthesized and its magnetic behavior has been investigated by magnetization (M), heat-capacity (C) and electrical resistivity (rho)…

Strongly Correlated Electrons · Physics 2009-11-11 Kausik Sengupta , P. L. Paulose , E. V. Sampathkumaran , Th. Doert , J. P. F. Jemetio

We determined the crystal structure of Cs$_2$LiRuCl$_6$, which was synthesized first in this work, and investigated its magnetic properties. Cs$_2$LiRuCl$_6$ has a hexagonal structure composed of linear chains of face-sharing RuCl$_6$ and…

We investigate the microscopic model for the frustrated layered antiferromagnets Cs2CuCl4 and Cs2CuBr4 by performing ab initio density functional theory (DFT) calculations and with the help of the tight-binding method. The combination of…

Strongly Correlated Electrons · Physics 2009-11-13 K. Foyevtsova , Y. Zhang , H. O. Jeschke , R. Valenti

We have studied the structural, magnetic properties, and electronic structure of the compound InCuPO5 synthesized by solid state reaction method. The structure of InCuPO5 comprises of S = 1/2 uniform spin chains formed by corner-shared CuO4…

Strongly Correlated Electrons · Physics 2017-05-30 B. Koteswararao , Binoy K. Hazra , Dibyata Rout , P. V. Srinivasarao , S. Srinath , S. K. Panda

The results of first-principles electronic structure calculations for the nitrogen-rich nickel nitrides $ {\rm NiN} $ and $ {\rm Ni_2N} $ are presented. The calculations are based on density functional theory and used the generalized…

Strongly Correlated Electrons · Physics 2018-11-27 Abdesalem Houari , Samir F. Matar , Volker Eyert

Crystal structure, electronic state of Ir$^{4+}$, and magnetic properties of the antifluorite compound K$_2$IrBr$_6$ are studied using high-resolution synchrotron x-ray diffraction, resonant inelastic x-ray scattering (RIXS), thermodynamic…

Strongly Correlated Electrons · Physics 2021-04-02 Nazir Khan , Danil Prishchenko , Mary H. Upton , Vladimir G. Mazurenko , Alexander A. Tsirlin

We report a combined experimental and theoretical study of the spin S=1/2 nanomagnet Cu5(OH)2(NIPA)4*10H2O (Cu5-NIPA). Using thermodynamic, electron spin resonance and 1H nuclear magnetic resonance measurements on one hand, and ab initio…

This study examines the increasing complexity in the magnetic properties of small $n$ = 3, 4, 5, 6 spin-1/2 quantum rings. Using an exact diagonalization of the isotropic Heisenberg Hamiltonian with nearest and next-nearest neighbor…

Materials Science · Physics 2016-09-21 J. T. Haraldsen

The magnetic structure of the antiferromagnetic square cupola compound Ba(TiO)Cu$_4$(PO$_4$)$_4$ with the tetragonal structure is studied with 31P nuclear magnetic resonance techniques. The magnetic hyperfine shift K shows a clear splitting…

Strongly Correlated Electrons · Physics 2020-02-19 Riho Rästa , Ivo Heinmaa , Kenta Kimura , Tsuyoshi Kimura , Raivo Stern