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The magnetic structure of the double perovskite compound Sr$_2$CuTeO$_6$ was determined from neutron powder diffraction data. This material is magnetically described as an $S\,{=}\,1/2$ quasi-two-dimensional square-lattice Heisenberg model…

Strongly Correlated Electrons · Physics 2016-03-09 Tomoyuki Koga , Nobuyuki Kurita , Maxim Avdeev , Sergey Danilkin , Taku J. Sato , Hidekazu Tanaka

We present the results of first-principles cluster calculations of the electronic structure of La_2CuO_4. Several clusters containing up to nine copper atoms embedded in a background potential were investigated. Spin-polarized calculations…

Superconductivity · Physics 2015-06-25 P. Husser , H. U. Suter , E. P. Stoll , P. F. Meier

Sr$_2$CuTeO$_6$ presents an opportunity for exploring low-dimensional magnetism on a square lattice of $S=1/2$ Cu$^{2+}$ ions. We employ ab initio multi-reference configuration interaction calculations to unravel the Cu$^{2+}$ electronic…

The hyperfine interactions at the uranium site in the antiferromagnetic USb2 compound were calculated within the density functional theory (DFT) employing augmented plane wave plus local orbital (APW+lo) method. We investigated the…

Strongly Correlated Electrons · Physics 2007-05-23 A. Fathi , S. Jalali Asadabadi , M. G. Rad , H. Amini

Quaternary Heusler alloys Co$_2$Cr$_{1-x}$Fe$_{x}$Al with varying Cr to Fe ratio $x$ were investigated experimentally and theoretically. The electronic structure and spectroscopic properties were calculated using the full relativistic…

Materials based on a crown ether complex together with magnetic ions, especially Cu(II), can be used to synthesize new low dimesional quantum spin systems. We have prepared the new crown ether complex…

We analyze a metal-dielectric structure composed of a silicon nanoparticle coupled to a stack of split-ring resonators, and reveal the possibility of optically-induced antiferromagnetic response of such a hybrid meta-molecule with a…

Inelastic neutron scattering experiments have been carried out on a powder sample of Cu2PO4OH, which consists of diamond-shaped tetramer spin units with S=1/2. We have observed two nearly dispersionless magnetic excitations at E1~12 and…

Materials Science · Physics 2015-12-09 M. Matsuda , S. E. Dissanayake , D. L. Abernathy , K. Totsuka , A. A. Belik

Less common ligand coordination of transition-metal centers is often associated with peculiar valence-shell electron configurations and outstanding physical properties. One example is the Fe$^+$ ion with linear coordination, actively…

Strongly Correlated Electrons · Physics 2020-11-20 R. Murugesan , M. S. Eldeeb , M. Yehia , B. Büchner , V. Kataev , O. Janson , L. Hozoi

We investigate the properties of CuVOF$_4$(H$_2$O)$_6$$\cdot$H$_2$O, in which two different spin species, Cu(II) and V(IV), form antiferromagnetic spin-1/2 dimers with weak interdimer coupling provided via hydrogen bonding. Using…

On the textbook example of an isolated antiferromagnetic Heisenberg dimer, we demonstrate that the magnetic form factor and the magnetic electron density distribution can be extracted from the momentum-dependence of the inelastic neutron…

We have successfully grown sizable single crystals of La_2Cu_{1-z}(Zn,Mg)_zO_4 with up to nearly half of the magnetic Cu sites replaced by non-magnetic Zn and Mg. Neutron scattering, SQUID magnetometry, and complementary quantum Monte Carlo…

Strongly Correlated Electrons · Physics 2009-11-07 O. P. Vajk , M. Greven , P. K. Mang , J. W. Lynn

Three different CrNi2 complexes were synthesized. They differ from each other by the nature of the terminal ligand and of the counter anion : [Cr(CN)4[CN-Ni(tetren)]2]Cl, that crystallizes in two different crystallographic systems and…

Mesoscale and Nanoscale Physics · Physics 2009-09-29 Raluca Tiron , Wolfgang Wernsdorfer , Fabien Tuyeras , Ariane Scuiller , Valerie Marvaud , Michel Verdaguer

Magnetic properties of the antiferromagnet Zn$_{0.15}$Cu$_{1.85}$V$_2$O$_7$ (ZnCVO) have been thoroughly investigated on powder and single-crystal samples. The crystal structure determination using powder x-ray and neutron diffraction…

Strongly Correlated Electrons · Physics 2023-01-02 G. Gitgeatpong , Y. Zhao , J. A. Fernandez-Baca , T. Hong , T. J. Sato , P. Piyawongwatthana , K. Nawa , P. Saeaun , K. Matan

We have employed first principles calculations to study the electronic structure and magnetic properties of the low-dimensional phosphates, Ba2Cu(PO4)2 and Sr2Cu(PO4)2. Using the self-consistent tight-binding lin- earized muffin-tin orbital…

Strongly Correlated Electrons · Physics 2007-09-17 Sarita S. Salunke , M. A. H. Ahsan , R. Nath , A. V. Mahajan , I. Dasgupta

To study the relationship between the properties of low-dimensional spin systems with weakly coupled Cu-triangles and their crystal structure, single crystals of $Cs_3Cu_3Cl_8OH$ (1) and the new $Cs_3Cu_3Cl_{7.6}Br_{0.4}OH$ (2) were grown.…

We investigate the magnetic behavior and critical exponents of quaternary CoFeV$_{0.8}$Mn$_{0.2}$Si Heusler alloy to understand the interactions across the Curie temperature ($T_{\rm C}$). The Rietveld refinement of the x-ray diffraction…

Materials Science · Physics 2023-10-04 Guru Dutt Gupt , P. D. Babu , R. S. Dhaka

The atomic and magnetic structures of (Cu$X$)LaNb$_2$O$_7$ ($X$=Cl and Br) are investigated using the density-functional calculations. Among several dozens of examined structures, an orthorhombic distorted $2\times 2$ structure, in which…

Strongly Correlated Electrons · Physics 2015-05-14 Chung-Yuan Ren , Ching Cheng

We have developed and implemented a self-consistent density functional method using standard norm-conserving pseudopotentials and a flexible, numerical LCAO basis set, which includes multiple-zeta and polarization orbitals. Exchange and…

Heusler alloy Co2FeAl was employed as ferromagnetic layers in Co2FeAl/Ru/Co2FeAl synthetic antiferromagnet structures. The experimental results show that the structure with a Ru thickness of 0.45 nm takes on strongly antiferromagnetic…

Materials Science · Physics 2015-05-13 X. G. Xu , D. L. Zhang , X. Q. Li , J. Bao , Y. Jiang