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To translate electrical into optical signals one uses the modulation of either the refractive index or the absorbance of a material by an electric field. Contemporary electroabsorption modulators (EAMs) employ the quantum confined Stark…

This study revisits the electroabsorption (EA) spectrum of polyacetylene, as functions of the electric field strength, isomerization degree, and light polarization states. The EA spectrum of $cis$-$(CH)_x$ reveals an oscillatory feature…

Other Condensed Matter · Physics 2024-05-07 Jaspal Singh Bola , Ryan M. Stolley , Prashanna Poudel , Joel S. Miller , Christoph Boheme , Z. Valy Vardeny

We study the photoabsorption properties of photoactive bulk polymer/ fullerene/nanotube heterojunctions in the near-infrared region. By combining pump-probe spectroscopy and linear response time-dependent density functional theory within…

Single-walled carbon nanotubes are strongly correlated systems with large Coulomb repulsion between two electrons occupying the same $p_z$ orbital. Within a molecular Hamiltonian appropriate for correlated $\pi$-electron systems, we show…

Materials Science · Physics 2009-02-15 Zhendong Wang , Demetra Psiachos , Roberto F. Badilla , Sumit Mazumdar

Cross-polarized absorption peaks of isolated single-walled carbon nanotubes were observed by a polarized photoluminescence excitation (PLE) spectroscopy. Using a simple theory for PL anisotropy, the observed PLE spectra are decomposed into…

Materials Science · Physics 2009-11-11 Yuhei Miyauchi , Mototeru Oba , Shigeo Maruyama

The $k\cdot p$ effective mass approximation (EMA) predicts large, nearly size-independent exciton oscillator strengths in quantum confined semiconductors. Yet, experimental reports have concluded that the total oscillator strength of the…

Mesoscale and Nanoscale Physics · Physics 2017-03-06 Yanhao Tang , Mersedeh Saniepay , Chenjia Mi , Rémi Beaulac , John A. McGuire

Quantum Stark effect in semiconductor nanocrystals is theoretically investigated, using the effective mass formalism within a $4\times 4$ Baldereschi-Lipari Hamiltonian model for the hole states. General expressions are reported for the…

Materials Science · Physics 2009-11-10 Eduardo Ariel Menendez Proupin , Carlos Trallero Giner

Current methods for producing single-walled carbon nanotubes (SWNTs) lead to heterogeneous samples containing mixtures of metallic and semiconducting species with a variety of lengths and defects. Optical detection at the single nanotube…

Electroabsorption (EA) measurements can be used to identify the type of excitons contributing to the absorption spectra of semiconductors which have applications in optoelectronics. However, the inferences from the EA measurement greatly…

Applied Physics · Physics 2020-09-29 Subhamoy Sahoo , Rajdeep Dhar , Sanjoy Jena , Soumya Dutta , Debdutta Ray , Jayeeta Bhattacharyya

Optical properties of single-wall carbon nanotubes (SWCNTs) for light polarized parallel to the nanotube axis have been extensively studied, whereas their response to light polarized perpendicular to the nanotube axis has not been well…

Mesoscale and Nanoscale Physics · Physics 2019-01-23 Fumiya Katsutani , Weilu Gao , Xinwei Li , Yota Ichinose , Yohei Yomogida , Kazuhiro Yanagi , Junichiro Kono

We present a quantitative theory of optical absorption polarized transverse to the tube axes in semiconducting single-walled carbon nanotubes. Transverse optical absorption in semiconducting single-walled carbon nanotubes is to an exciton…

Materials Science · Physics 2009-11-13 Zhendong Wang , Hongbo Zhao , Sumit Mazumdar

We have studied the electronic structure and charge-carrier dynamics of individual single-wall carbon nanotubes (SWNTs) and nanotube ropes using optical and electron-spectroscopic techniques. The electronic structure of semiconducting SWNTs…

Materials Science · Physics 2009-11-10 A. Hagen , G. Moos , V. Talalaev , J. W. Tomm , T. Hertel

We consider the effects of electron-hole interaction, 2D confinement and applied electric field on direct allowed transitions in III-V semiconductors, with InGaAs as a study case. Instead of Coulomb interaction, we use Gaussian potential.…

Computational Physics · Physics 2021-01-18 Yuriy D. Sibirmovsky , Ivan S. Vasil'evskii , Nikolay I. Kargin

Electroabsorption spectroscopy of well-identified index-defined semiconducting carbon nanotubes is reported. The measurement of high definition electroabsorption spectra allows direct indexation with unique nanotube chirality. Results show…

The quasiparticle band structure and optical properties of single-walled zigzag and armchair SiC nanotubes (SiC-NTs) as well as single SiC sheet are investigated by ab initio many-body calculations using the GW and the GW plus…

Mesoscale and Nanoscale Physics · Physics 2011-08-23 H. C. Hsueh , G. Y. Guo , Steven G. Louie

Auger-ionized carriers in a one-dimensional semiconductor are predicted to result in a strong band-gap renormalization. Isolated single-walled carbon nanotubes (SWCNT) under high-intensity laser irradiation exhibit strong nonlinear…

Mesoscale and Nanoscale Physics · Physics 2016-02-26 Mitchell D. Anderson , Meghan N. Beattie , Jack A. Alexander-Webber , Robin J. Nicholas , James M. Fraser

Theory predicts peculiar features for excited-state dynamics in one dimension (1D) that are difficult to be observed experimentally. Single-walled carbon nanotubes (SWNTs) are an excellent approximation to 1D quantum confinement, due to…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Giancarlo Soavi , Francesco Scotognella , Daniele Viola , Timo Hefner , Tobias Hertel , Giulio Cerullo , Guglielmo Lanzani

The Ajiki-Ando (A-A) splitting of single-walled carbon nanotubes(SWNT) originating from the Aharanov-Bohm effect was observed in chiral specific SWNTs by the magneto-absorption measurements conducted at magnetic fields of up to 78 T. The…

Mesoscale and Nanoscale Physics · Physics 2015-05-28 Shojiro Takeyama , Hirofumi Suzuki , Hiroyuki Yokoi , Yoichi Murakami , Shigeo Maruyama

The magnetic field dependence of photoabsorption provides direct insights into the band structure of semiconductors. It is perhaps surprising that there is a large discrepancy between electron, hole, and reduced mass reported in the recent…

Mesoscale and Nanoscale Physics · Physics 2025-01-22 Jack N. Engdahl , Harley D. Scammell , Dmitry K. Efimkin , Oleg P. Sushkov

The recent development of efficient chirality sorting techniques has opened the way to the use of single-walled carbon nanotubes (SWCNTs) in a plethora of nanoelectronic, photovoltaic, and optoelectronic applications. However, to understand…

Mesoscale and Nanoscale Physics · Physics 2019-12-25 María Rosa Preciado-Rivas , Victor Alexander Torres-Sánchez , Duncan J. Mowbray
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