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The magnetic properties of (Ga,Mn)As thin films depend on both the Mn doping level and the carrier concentration. Using a post growth hydrogenation process we show that it is possible to decrease the hole density from 1.1021 cm-3 to <1017…

The effect of short-time and long-time annealing at 250C on the conductivity, hole density, and Curie temperature of GaMnAs single layers and GaMnAs/InGaMnAs heterostructures is studied by in-situ conductivity measurements as well as Raman…

Condensed Matter · Physics 2009-11-10 W. Limmer , A. Koeder , S. Frank , M. Glunk , W. Schoch , V. Avrutin , K. Zuern , R. Sauer , A. Waag

We have investigated the effects of post growth low temperature annealing on the magnetic, electrical and structural properties of (Ga_0.94,Mn_0.06)(As_0.9,P_0.1) layers grown by molecular beam epitaxy. By controlling the annealing time we…

Ion irradiation of semiconductors is a well understood method to tune the carrier concentration in a controlled manner. We show that the ferromagnetism in GaMnAs films, known to be hole-mediated, can be modified by He ion irradiation. The…

We report the successful passivation of the Mn acceptors in GaMnP upon exposure to a remote dc hydrogen plasma. The as-grown films are non-metallic and ferromagnetic with a Curie temperature of T_C=55K. After hydrogenation the sample…

Materials Science · Physics 2008-07-10 C. Bihler , M. Kraus , M. S. Brandt , S. T. B. Goennenwein , M. Opel , M. A. Scarpulla , R. Farshchi , O. D. Dubon

The ferromagnetism of a thin GaMnAs layer with a perpendicular easy anisotropy axis is investigated by means of several techniques, that yield a consistent set of data on the magnetic properties and the domain structure of this diluted…

We demonstrate the manipulation of the Curie temperature of buried layers of the ferromagnetic semiconductor (Ga,Mn)As using nanolithography to enhance the effect of annealing. Patterning the GaAs-capped ferromagnetic layers into nanowires…

Materials Science · Physics 2009-11-11 K. F. Eid , B. L. Sheu , O. Maksimov , M. B. Stone , P. Schiffer , N. Samarth

(Ga,Mn)As and related diluted magnetic semiconductors play a major role in spintronics research because of their potential to combine ferromagnetism and semiconducting properties in one physical system. Ferromagnetism requires ~1-10% of…

Materials Science · Physics 2009-11-13 K. Olejnik , M. H. S. Owen , V. Novak , J. Masek , A. C. Irvine , J. Wunderlich , T. Jungwirth

We report on a monotonic reduction of Curie temperature in dilute ferromagnetic semiconductor (Ga,Mn)As upon a well controlled chemical-etching/oxidizing thinning from 15 nm down to complete removal of the ferro- magnetic response. The…

Materials Science · Physics 2012-06-29 O. Proselkov , D. Sztenkiel , W. Stefanowicz , M. Aleszkiewicz , J. Sadowski , T. Dietl , M. Sawicki

We report a clear correspondence between changes in the Curie temperature and carrier density upon annealing in epitaxially grown (Ga,Mn)As layers with thicknesses in the range between 5 nm and 20 nm. The changes are dependent on the layer…

Materials Science · Physics 2009-11-07 B. Sorensen , J. Sadowski , R. Mathieu , P. Svedlindh , P. E. Lindelof

It is demonstrated by SQUID measurements that (Ga,Mn)As films can exhibit perpendicular easy axis at low temperatures, even under compressive strain, provided that the hole concentration is sufficiently low. In such films, the easy axis…

We have synthesized Ga1-xMnxAs1-yPy and Ga1-xMnxP1-yNy by the combination of ion implantation and pulsed-laser melting. We find that the incorporation of isovalent impurities with smaller atomic radii leads to a realignment of the magnetic…

Materials Science · Physics 2008-11-13 Peter R. Stone , Jeffrey W. Beeman , Kin M. Yu , Oscar D. Dubon

We report Curie temperatures up to 150 K in annealed Ga1-xMnxAs epilayers grown with a relatively low As:Ga beam equivalent pressure ratio. A variety of measurements (magnetization, Hall effect, magnetic circular dichroism and Raman…

The effect of annealing at 250 C on the carrier depth profile, Mn distribution, electrical conductivity, and Curie temperature of (Ga,Mn)As layers with thicknesses > 200 nm, grown by molecular-beam epitaxy at low temperatures, is studied by…

Materials Science · Physics 2009-11-11 W. Limmer , A. Koeder , S. Frank , V. Avrutin , W. Schoch , R. Sauer , K. Zuern , J. Eisenmenger , P. Ziemann , E. Peiner , A. Waag

We study the controlled introduction of defects in GaMnAs by irradiating the samples with energetic ion beams, which modify the magnetic properties of the DMS. Our study focuses on the low-carrier-density regime, starting with as-grown…

Disordered Systems and Neural Networks · Physics 2010-06-14 E. H. C. P. Sinnecker , G. M. Penello , T. G. Rappoport , M. M. Sant'Anna , D. E. R. Souza , M. P. Pires , X. Liu , J. K. Furdyna

We report the magnetic and transport properties of Ga1-xMnxP synthesized via ion implantation followed by pulsed laser melting over a range of x, namely 0.018 to 0.042. Like Ga1-xMnxAs, Ga1-xMnxP displays a monotonic increase of the…

Annealing can increase the Curie temperature and net magnetization in uncapped (Ga,Mn)As films, effects that are suppressed when the films are capped with GaAs. Previous polarized neutron reflectometry (PNR) studies of uncapped (Ga,Mn)As…

Materials Science · Physics 2009-11-10 B. J. Kirby , J. A. Borchers , J. J. Rhyne , K. V. O'Donovan , T. Wojtowicz , X. Liu , Z. Ge , S. Shen , J. K. Furdyna

We examine the Mn concentration dependence of the electronic and magnetic properties of optimally annealed Ga1-xMnxAs epilayers for 1.35% < x < 8.3%. The Curie temperature (Tc), conductivity, and exchange energy increase with Mn…

Condensed Matter · Physics 2009-11-07 S. J. Potashnik , K. C. Ku , R. Mahendiran , S. H. Chun , R. F. Wang , N. Samarth , P. Schiffer

We present the manipulation of magnetic and electrical properties of (Ga,Mn)As by the adsorption of dye-molecules as a first step towards the realization of light-controlled magnetic-semiconductor/dye hybrid devices. A significant lowering…

Magnetic and magneto-transport properties of thin layers of the (Ga,Mn)(Bi,As) quaternary dilute magnetic semiconductor grown by the low-temperature molecular-beam epitaxy technique on GaAs substrates have been investigated. Ferromagnetic…

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