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Related papers: Pressure-induced insulating state in (La,Sr)CoO$_{…

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We study the structural evolution of Sr$_3$Ir$_2$O$_7$ as a function of pressure using x-ray diffraction. At a pressure of 54 GPa at room temperature, we observe a first-order structural phase transition, associated with a change from…

The charge transfer antiferromagnetic (T$_{N}$ =220 K) insulator EuNiO$_{3}$ undergoes, at ambient pressure, a temperature-induced metal insulator MI transition at T$_{MI}$=463 K. We have investigated the effect of pressure (up to p~20 GPa)…

Strongly Correlated Electrons · Physics 2009-11-11 R. Lengsdorf , A. Barla , J. A. Alonso , M. J. Martinez-Lope , H. Micklitz , M. M. Abd-Elmeguid

Transport and magnetic measurements and structural and NMR studies have been carried out on (Pr1-yR'y)1-xAxCoO3 {R'=(rare earth elements and Y); A=(Ca, Ba and Sr)} at ambient pressure or under high pressure. The system exhibits a phase…

Ab initio calculations predict a metal-insulator transition at zero temperature to occur in La$_4$Ni$_3$O$_8$ at moderate pressures as a result of a pressure-induced spin-state transition. The spin-state transition that is seen at 105 K at…

Strongly Correlated Electrons · Physics 2015-05-28 Victor Pardo , Warren E. Pickett

We investigated the effect of pressure on the magnetic and thermoelectric properties of Sr$_{3.1}$Y$_{0.9}$Co$_{4}$O$_{10+\delta }$. The magnetization is reduced with the application of pressure, reflecting the spin-state modification of…

Strongly Correlated Electrons · Physics 2018-08-01 Hidefumi Takahashi , Shintaro Ishiwata , Ryuji Okazaki , Yukio Yasui , Ichiro Terasaki

We employ a combination of the \emph{ab initio} band structure methods and dynamical mean-field theory to determine the electronic structure and phase stability of paramagnetic FeO at high pressure and temperature. Our results reveal a…

Strongly Correlated Electrons · Physics 2015-09-18 I. Leonov

We sought the origin of the metal-insulator transition in Sr2-xLaxCoO4, using electron-correlation corrected density functional calculations. Our results show that Sr2CoO4 is in an intermediate-spin (IS) state and a strong Co4+ 3d-O 2p…

Strongly Correlated Electrons · Physics 2015-06-11 Hua Wu

The crystal lattice of Sr$_2$IrO$_4$ is investigated with synchrotron X-ray powder diffraction under hydrostatic pressures up to $P=43$ GPa and temperatures down to $20$ K. The tetragonal unit cell is maintained over the whole investigated…

Strongly Correlated Electrons · Physics 2020-02-26 K. Samanta , R. Tartaglia , U. F. Kaneko , N. M. Souza-Neto , E. Granado

We report results of magnetization and ac susceptibility measurements down to very low fields on a single crystal of the perovskite manganite, La$_{0.82}$Ca$_{0.18}$MnO$_3$. This composition falls in the intriguing ferromagnetic insulator…

Strongly Correlated Electrons · Physics 2014-03-17 P. Anil Kumar , R. Mathieu , P. Nordblad , Sugata Ray , Olof Karis , Gabriella Andersson , D. D. Sarma

The perovskite antiferromagnetic ($T_{\rm N}$ $\sim$ 220 K) insulator EuNiO$_3$ undergoes at ambient pressure a metal-to-insulator transition at $T_{\rm MI}$ = 460 K which is associated with a simultaneous orthorhombic-to-monoclinic…

The structural properties of LaCoO3 were studied by means of high-resolution neutron powder diffraction in the temperature range 5<T<1000 K. Changes of the Co+3 spin states in this temperature interval are shown to affect not only the unit…

Strongly Correlated Electrons · Physics 2009-11-07 Paolo G. Radaelli , Sang-Wook Cheong

We systematically investigate effect of oxygen isotope in $(Pr_{1-x}Sm_x)_{0.7}Ca_{0.3}CoO_3$ which shows a crossover with x from ferromagnetic metal to the insulator with spin-state transition. A striking feature is that effect of oxygen…

Strongly Correlated Electrons · Physics 2009-11-11 G. Y. Wang , X. H. Chen , T. Wu , G. Wu , X. G. Luo , C. H. Wang

In double perovskite oxides (A$_2$BB$^\prime$O$_6$), magnetism often arises from diluted magnetic lattices, created by combining a perovskite structure with localized 3$d$ magnetic elements (B) alongside another perovskite lattice…

Strongly Correlated Electrons · Physics 2024-08-20 Sromona Nandi , Subhadip Pradhan , Ashis K. Nandy , Rudra Sekhar Manna

We investigate the structural, magnetic and spin-state transitions, and magnetocaloric properties of Sr$_{2-x}$La$_x$CoNbO$_6$ ($x=$ 0--1) double perovskites. The structural transition from tetragonal to monoclinic phase at $x$ $\geqslant$…

Materials Science · Physics 2020-04-21 Ajay Kumar , R. S. Dhaka

Magnetization and x-ray diffraction have been measured on polycrystalline samples of LaCo$_{0.8-y}$Rh$_{0.2}$Ga$_{y}$O$_{3}$ for $0 \leq y \leq 0.15$ in order to understand the spin state of Co$^{3+}$ through the Ga$^{3+}$ substitution…

Strongly Correlated Electrons · Physics 2012-08-08 Shinichiro Asai , Noriyasu Furuta , Ryuji Okazaki , Yukio Yasui , Ichiro Terasaki

LaCoO3 thin films grown under epitaxial tensile strain exhibit a robust ferromagnetic insulating state that is absent in the bulk. Despite many studies, both experimental and computational, the microscopic origin of this phenomenon is not…

Materials Science · Physics 2026-04-08 Ali Barooni , Murod Mirzhalilov , Mohit Randeria , Patrick M. Woodward , Maryam Ghazisaeidi

We studied the Co valences and spin states in electron-doped LaCo$_{1-y}$Te$_{y}$O$_3$ by measuring x-ray absorption spectra and electron spin resonance. The low-temperature insulating state involves the low-spin Co$^{3+}$ ($S=0$) and the…

The spin state transition in LaCoO$_3$ has eluded description for decades despite concerted theoretical and experimental effort. In this study, we approach this problem using fully charge self-consistent Density Functional Theory + Embedded…

Materials Science · Physics 2017-11-15 Bismayan Chakrabarti , Turan Birol , Kristjan Haule

La$_{1.5}$Ca$_{0.5}$CoIrO$_{6}$ is a re-entrant spin-glass (SG) that exhibits antiferromagnetic and ferromagnetic couplings at $T\sim95$ and $\sim86$ K, respectively, and at $T\sim25$ K a SG phase emerges. In this work we investigated the…

Materials Science · Physics 2018-08-31 L. T. Coutrim , E. M. Bittar , L. Mendonça-Ferreira , L. Bufaiçal

We study theoretically low-temperature phases of a recently synthesized compound Sr$_2$CoO$_3$F under pressure. The analysis combining LDA+DMFT and a strong-coupling effective model points to the existence of not only normal paramagnetic…

Strongly Correlated Electrons · Physics 2019-05-15 Juan Fernández Afonso , Andrii Sotnikov , Atsushi Hariki , Jan Kuneš