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A quantum-mechanical model to calculate the electron energy-loss spectra (EELS) for the system of a closely located metallic nanoshell and a molecule has been developed. At the resonance between the molecular excitation and plasmon modes in…

Atomic Physics · Physics 2014-10-07 I. Yu. Goliney , Ye. V. Onykienko

Inelastic losses are crucial to a quantitative analysis of x-ray absorption spectra. However, current treatments are semi-phenomenological in nature. Here a first-principles, many-pole generalization of the plasmon-pole model is developed…

Materials Science · Physics 2009-11-13 J. J. Kas , A. P. Sorini , M. P. Prange , L. W. Cambell , J. A. Soininen , J. J. Rehr

The orbital distribution of the spin fluctuation in the iron-based superconductors(IBSs) is the key information needed to understand the magnetism, superconductivity and electronic nematicity in these multi-orbital systems. In this work, we…

Superconductivity · Physics 2021-07-28 Da-Wei Yao , Tao Li

A new method is presented for describing vibrational effects in x-ray absorption spectroscopy (XAS) and resonant inelastic x-ray scattering (RIXS) using a combination of the classical Franck-Condon (FC) approximation and classical…

Materials Science · Physics 2017-12-20 Mathias P. Ljungberg

Despite the widespread use of Scanning Transmission Electron Microscopy (STEM) for observing the structure of materials at the atomic scale, a detailed understanding of some relevant electron beam damage mechanisms is limited. Recent…

We have developed a theory of the one-phonon intraband resonance Raman scattering (IRRS) in anisotropic quantum dots subjected to an arbitrarily directed magnetic field. The differential Raman cross section is obtained. The resonance…

Mesoscale and Nanoscale Physics · Physics 2010-01-08 A. V. Shorokhov , V. A. Margulis

Resonant inelastic X-ray scattering (RIXS) has become an important scientific tool. Nonetheless, conventional high-resolution RIXS measurements (<100 meV), especially in the soft x-ray range, require large and low-throughput grating…

Materials Science · Physics 2020-06-22 Daniel J. Higley , Hirohito Ogasawara , Sioan Zohar , Georgi L. Dakovski

We study the magnetic excitation spectra of resonant inelastic x-ray scattering (RIXS) at the $L$-edge from undoped cuprates beyond the fast collision approximation. We analyse the effect of the symmetry breaking ground state on the RIXS…

Strongly Correlated Electrons · Physics 2015-06-24 Jun-ichi Igarashi , Tatsuya Nagao

A electron of mass $m$, when electrically scatters of nucleus, of mass $M$, transfers momentum $q$ to the nucleus. The energy lost by electron is more than the energy gained by the nucleus. The resulting energy goes in exciting the atom to…

Quantum Physics · Physics 2023-09-20 Navin Khaneja

We compare several different ways of measuring the energy resolution for meV-resolved inelastic x-ray scattering (IXS): using scattering from poly(methyl methacrylate), PMMA, using scattering from borosilicate glass (Tempax), and using…

Materials Science · Physics 2021-03-17 Daisuke Ishikawa , Alfred Q. R. Baron

Strong multiple scattering of the probe in scanning transmission electron microscopy (STEM) means image simulations are usually required for quantitative interpretation and analysis of elemental maps produced by electron energy-loss…

Materials Science · Physics 2019-12-25 Hamish G. Brown , Jim Ciston , Colin Ophus

Recent experiments on La$_2$CuO$_4$ suggest that indirect resonant inelastic X-ray scattering (RIXS) might provide a probe for transversal spin dynamics. We present in detail a systematic expansion of the relevant magnetic RIXS cross…

Strongly Correlated Electrons · Physics 2011-07-22 Filomena Forte , Luuk J. P. Ament , Jeroen van den Brink

Young's archetypal double-slit experiment forms the basis for modern diffraction techniques: the elastic scattering of waves yields an interference pattern that captures the real-space structure. Here, we report on an inelastic incarnation…

We analyze a recent work of Mayers and Abdul-Redah,[J.Phys.: Condens. Matter {\bf 16}, 4811 (2004)] in which the autors report the existence of anomalous neutron cross sections in several systems. In the present work we show that the Deep…

Data Analysis, Statistics and Probability · Physics 2007-05-23 J. J. Blostein , J. Dawidowski , J. R. Granada

Waves scattered by a weakly inhomogeneous random medium contain a predominant single scattering contribution as well as a multiple scattering contribution which is usually neglected, especially for imaging purposes. A method based on random…

Classical Physics · Physics 2015-03-13 Alexandre Aubry , Arnaud Derode

We study the magnetic resonant x-ray scattering (RXS) spectra around the $K$ edge of Cu in KCuF$_3$ on the basis of an {\em ab initio} calculation. We use the full-potential linearlized augmented plane wave method in the LDA$+U$ scheme, and…

Strongly Correlated Electrons · Physics 2009-11-07 M. Takahashi , M. Usuda , J. Igarashi

Scattering experiments can be leveraged to extract the effective properties of a heterogeneous metamaterial slab based on multi-point measurements in surrounding media. In this technique, two measurements are made in the ambient media on…

Applied Physics · Physics 2023-07-14 Joshua Morris , Alireza V. Amirkhizi

This paper theoretically treats the spontaneous resonant inelastic scattering of Laguerre-Gauss (LG) beams from the totally symmetric vibrations of complex polyatomic molecules within the semi-classical framework. We develop an interaction…

Optics · Physics 2015-06-17 Aaron S. Rury

Resonant inelastic x-ray scattering (RIXS) at the copper K absorption edge has been performed for heavily overdoped samples of La$_{2-x}$Sr$_{x}$CuO$_{4}$ with $x= 0.25$ and 0.30. We have observed the charge transfer and molecular-orbital…

Superconductivity · Physics 2009-11-11 S. Wakimoto , Young-June Kim , Hyunkyung Kim , H. Zhang , T. Gog , R. J. Birgeneau

The resonant inelastic x-ray scattering (RIXS) was measured in an insulating SrCuO$_{2}$ with changing the incident photon energy ($h\nu$) near the Cu $1s$ absorption edge (K-edge). Complex structures and their dependences on the momentum…