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We characterize the ground state and excitation spectrum of the $S=1/2$, nominally pure and perfect kagom\'{e} system ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$ using the following measurements: magnetization, muon spin rotation frequency shift $K$,…

Strongly Correlated Electrons · Physics 2007-05-23 Oren Ofer , Amit Keren , Emily A. Nytko , Matthew P. Shores , Bart M. Bartlett , Daniel G. Nocera , Chris Baines , Alex Amato

The $T$-dependence (2- 400 K) of the electron paramagnetic resonance (EPR), magnetic susceptibility, $\chi (T)$, and specific heat, $C_{v}(T)$, of the $normal$ antiferromagnetic (AFM) spinel ZnCr$_{2}$O$_{4}$ and the spin-glass (SG)…

Collective behaviour of electrons, frustration induced quantum fluctuations and entanglement in quantum materials underlie some of the emergent quantum phenomena with exotic quasi-particle excitations that are highly relevant for…

Frustrated itinerant ferromagnets, with non-collinear static spin structures, are an exciting class of material as their spin chirality can introduce a Berry phase in the electronic scattering and lead to exotic electronic phenomena such as…

Strongly Correlated Electrons · Physics 2018-09-17 L A Fenner , A A Dee , A S Wills

Recently, a novel material with bilayer kagome lattice Ca$_{10}$Cr$_7$O$_{28}$ was proposed to be a gapless quantum spin liquid, due to the lack of long-range magnetic order and the observation of broad diffuse excitations. Here, we present…

Strongly Correlated Electrons · Physics 2018-11-02 J. M. Ni , Q. Y. Liu , Y. J. Yu , E. J. Cheng , Y. Y. Huang , Z. Y. Liu , X. J. Wang , Y. Sui , S. Y. Li

Dielectric and magnetic properties have been studied for poly-crystalline samples of quasi-one-dimensional frustrated spin-1/2 system Rb$_{2}$(Cu$_{1-x}$M$_{x}$)$_{2}$Mo$_{3}$O$_{12}$(M=Ni and Zn) which does not exhibit a three-dimensional…

Strongly Correlated Electrons · Physics 2015-06-12 Yukio Yasui , Yudai Yanagisawa , Ryuji Okazaki , Ichiro Terasaki

Muon spin rotation and relaxation experiments in the pyrochlore iridate Eu2Ir2O7 yield a well-defined muon spin precession frequency below the metal-insulator/antiferromagnetic transition temperature TM = 120 K, indicative of long-range…

Strongly Correlated Electrons · Physics 2015-03-19 Songrui Zhao. J. M. Mackie , D. E. MacLaughlin , O. O. Bernal , J. J. Ishikawa , Y. Ohta , S. Nakatsuji

Here, we report both ac and dc magnetization, thermodynamic and electric properties of hexagonal Ba$_3$NiIr$_2$O$_9$. The Ni$^{2+}$ (spin-1) forms layered triangular-lattice and interacts antiferromagnetically while Ir$^{5+}$ is believed to…

Strongly Correlated Electrons · Physics 2021-07-14 Shobha Gondh , Manju Mishra Patidar , Kranti Kumar , M. P. Saravanan , V. Ganesan , A. K. Pramanik

The compounds Sr$_{3}$Cr$_{2}$O$_{8}$ and Ba$_{3}$Cr$_{2}$O$_{8}$ are insulating dimerized antiferromagnets with Cr$^{5+}$ magnetic ions. These spin-$\frac{1}{2}$ ions form hexagonal bilayers with a strong intradimer antiferromagnetic…

Disordered Systems and Neural Networks · Physics 2017-11-15 Alsu Gazizulina , Diana Lucia Quintero-Castro , Andreas Schilling

The dynamics of magnetic moments in iron-chromium alloys with different levels of Cr clustering show unusual features resulting from the fact that even in a perfect body-centred cubic structure, magnetic moments experience geometric…

Materials Science · Physics 2019-05-22 J. B. J. Chapman , S. L. Dudarev , P. -W. Ma

The effects of magnetic dilution and applied pressure on frustrated spinel Ni$_{2-x}$Mg$_{x}$GeO$_{4}$ (0 $\leq x \leq 1.0$) are analyzed using specific heat, AC and DC magnetization and x-ray diffraction. The parent compound has two…

Materials Science · Physics 2015-11-11 J. T. Korobanik , K. Caslin , P. Reuvekamp , F. S. Razavi

Ca$_{10}$Cr$_7$O$_{28}$ is a novel spin-$1/2$ magnet exhibiting spin liquid behaviour which sets it apart from any previously studied model or material. However, understanding Ca$_{10}$Cr$_7$O$_{28}$ presents a significant challenge,…

Strongly Correlated Electrons · Physics 2021-07-28 Rico Pohle , Han Yan , Nic Shannon

Both Ba$_4$Mn$_3$O$_{10}$ and Sr$_4$Mn$_3$O$_{10}$ crystallize in an orthorhombic crystal structure consisting of corrugated layers containing Mn$_3$O$_{12}$ polydedra. The thermal variation of magnetic susceptibility of the compositions…

Strongly Correlated Electrons · Physics 2015-06-23 J. Sannigrahi , S. Chattopadhyay , A. Bhattacharyya , S. Giri , S. Majumdar , D. Venkateshwarlu , V. Ganesan

Single crystalline and polycrystalline samples of $S=1/2$ Kagom\'{e} lattices {[Cu$_{3}$(CO$_{3}$)$_{2}$$(bpe)_{3}$](ClO$_{4}$)$_2$}$_{n}$ and {[Cu$_{3}$(CO$_{3}$)$_{2}$$(bpy)_{3}$](ClO$_{4}$)$_2$}$_{n}$, respectively were synthesized.…

Materials Science · Physics 2015-06-29 M. O. Ajeesh , A. Yogi , M. Padmanabhan , R. Nath

We have performed thermodynamic and neutron scattering measurements on the S=1/2 kagome lattice antiferromagnet Zn Cu_3 (OH)_6 Cl_2. The susceptibility indicates a Curie-Weiss temperature of ~ -300 K; however, no magnetic order is observed…

Strongly Correlated Electrons · Physics 2007-05-23 J. S. Helton , K. Matan , M. P. Shores , E. A. Nytko , B. M. Bartlett , Y. Yoshida , Y. Takano , A. Suslov , Y. Qiu , J. -H. Chung , D. G. Nocera , Y. S. Lee

Recent inelastic neutron diffraction measurements on Cr$_2$(Te, W, Mo)O$_6$ have revealed that these systems consist of bilayers of spin-3/2 Cr$^{3+}$ ions with strong antiferromagnetic inter-bilayer coupling and tuneable intra-bilayer…

Strongly Correlated Electrons · Physics 2019-04-04 Kingshuk Majumdar , Subhendra D. Mahanti

The transition metal based oxide YBaCo3FeO7 is structurally related to the mineral Swedenborgite SbNaBe4O7, a polar non-centrosymmetric crystal system. The magnetic Co3Fe sublattice consists of a tetrahedral network containing kagome-like…

Materials Science · Physics 2015-05-28 Martin Valldor , Raphaël P. Hermann , Joachim Wuttke , Michaela Zamponi , Werner Schweika

The pyrochlore material Yb2Ti2O7 displays unexpected quasi-two-dimensional (2D) magnetic correlations within a cubic lattice environment at low temperatures, before entering an exotic disordered ground state below T=265mK. We report neutron…

Strongly Correlated Electrons · Physics 2012-02-13 K. A. Ross , L. R. Yaraskavitch , M. Laver , J. S. Gardner , J. A. Quilliam , S. Meng , J. B. Kycia , D. K. Singh , H. A. Dabkowska , B. D. Gaulin

In the garnet structure compound Yb3Ga5O12, the Yb3+ ions (ground state effective spin S' = 1/2) are situated on two interpenetrating corner sharing triangular sublattices such that frustrated magnetic interactions are possible. Previous…

Condensed Matter · Physics 2009-11-10 J. A. Hodges , P. Bonville , M. Rams , K. Krolas

Frustrated magnets offer a plethora of exotic magnetic ground states, including quantum spin liquids (QSLs), in which enhanced quantum fluctuations prevent a long-range magnetic ordering of the strongly correlated spins down to lowest…