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The interplay between competing degrees of freedom can stabilize non-trivial magnetic states in correlated electron materials. Frustration-induced strong quantum fluctuations can evade long-range magnetic ordering leading to exotic quantum…

Strongly Correlated Electrons · Physics 2023-10-12 B. Sana , M. Barik , M. Pregelj , U. Jena , M. Baenitz , J. Sichelschmidt , K. Sethupathi , P. Khuntia

We report ac susceptibility and high-frequency electron spin resonance (ESR) measurements on the geometrically frustrated compound Ba$_3$NbFe$_3$Si$_2$O$_{14}$ with the N\'{e}el temperature $T_N=27 K$. An unusually large…

Strongly Correlated Electrons · Physics 2011-08-10 K. -Y. Choi , Z. -X. Wang , A. Ozarowski , J. van Tol , H. D. Zhou , C. R. Wiebe , N. S. Dalal

A pronounced Curie-like upturn of the magnetic susceptibility chi(T) of the quasi one-dimensional spin chain compound Ba2V3O9 has been found recently. Frequently this is taken as a signature for a staggered field mechanism due to the…

Strongly Correlated Electrons · Physics 2009-11-07 B. Schmidt , V. Yushankhai , L. Siurakshina , P. Thalmeier

We have investigated the kagom\'{e} ice behavior of the dipolar spin-ice compound Dy_{2}Ti_{2}O_{7} in magnetic field along a [111] direction using neutron scattering and Monte Carlo simulations. The spin correlations show that the…

Disordered Systems and Neural Networks · Physics 2007-05-23 Y. Tabata , H. Kadowaki , K. Matsuhira , Z. Hiroi , N. Aso , E. Ressouche , B. Fak

We report muon spin relaxation ($\mu$SR) and $^{69,71}$Ga nuclear quadrupolar resonance (NQR) local-probe investigations of the kagom\'e compound Pr$_3$Ga$_5$SiO$_{14}$. Small quasi-static random internal fields develop below 40 K and…

Strongly Correlated Electrons · Physics 2015-05-14 A. Zorko , F. Bert , P. Mendels , K. Marty , P. Bordet

Using thermodynamic measurements, neutron diffraction, nuclear magnetic resonance, and muon spin relaxation, we establish putative quantum spin-liquid behavior in Ba$_3$InIr$_2$O$_9$, where unpaired electrons are localized on mixed-valence…

The magnetic behaviour of the low-dimensional Vanadium-oxides Sr2V3O9 and Ba2V3O9 was investigated by means of magnetic susceptibility and specific heat measurements. In both compounds, the results can be very well described by an S=1/2…

Condensed Matter · Physics 2009-11-07 E. E. Kaul , H. Rosner , V. Yushankhai , J. Sichelschmidt , R. V. Shpanchenko , C. Geibel

We propose a new model for the nature of the low temperature phase of a geometrically frustrated antiferromgnet (AFM) with a Kagome lattice, SrCr$_{8-x}$Ga$_{4+x}$O$_{19}$. We propose that the long-range dipolar interaction between the…

Condensed Matter · Physics 2007-05-23 Nir Gov

We report magnetization, electron spin resonance (ESR), and muon spin relaxation ($\mu $SR) measurements on single crystals of the $S=1/2$ (Cu$% ^{+2}$) kagom\'{e} compound Cu(1,3-benzendicarboxylate). The $\mu $SR is carried to…

Strongly Correlated Electrons · Physics 2015-06-18 Oren Ofer , Lital Marcipar , V. Ravi Chandra , Snir Gazit , Daniel Podolsky , Daniel P. Arovas , Amit Keren

Competing magnetic interactions, frustration driven quantum fluctuations, and spin correlations offer an ideal route for the experimental realization of emergent quantum phenomena and exotic quasi particle excitations in 3D frustrated…

Strongly Correlated Electrons · Physics 2024-07-09 J. Khatua , Suheon Lee , Gyungbin Ban , Marc Uhlarz , Kwang-Yong Choi , P. Khuntia

The three-dimensional frustrated spin lattice in MgCrGaO4, where Cr3+ ions occupy a pyrochlore-like network, exemplifies a quantum magnet with competing interactions, macroscopic degeneracy, and exotic low-energy excitations. Using…

Strongly Correlated Electrons · Physics 2026-03-17 U. Jena , S. Kundu , Suheon Lee , Q. Faure , F. Damay , S. Rols , Adam Berlie , S. Petit , Kwang-Yong Choi , P. Khuntia

We consider the archetypal frustrated antiferromagnet SrCr$_{9p}$Ga$_{12-9p}$O$_{19}$ in its well-known spin-liquid state, and demonstrate that a Cr$^{3+}$ spin $S=3/2$ ion in direct proximity to a pair of vacancies (in disordered $p<1$…

Strongly Correlated Electrons · Physics 2015-05-19 Arnab Sen , Kedar Damle , Roderich Moessner

The nature of the magnetic ground state of highly frustrated systems remained puzzling to this day. Here, we have performed multifrequency electron spin resonance (ESR) measurements on a putative quantum spin liquid compound…

We report a new kagome quantum spin liquid candidate Cu$_3$Zn(OH)$_6$FBr, which does not experience any phase transition down to 50 mK, more than three orders lower than the antiferromagnetic Curie-Weiss temperature ($\sim$ 200 K). A clear…

We study the spin dynamics of classical Heisenberg antiferromagnet with nearest neighbor interactions on a quasi-two-dimensional kagome bilayer. This geometrically frustrated lattice consists of two kagome layers connected by a…

Strongly Correlated Electrons · Physics 2021-06-09 Preetha Saha , Depei Zhang , Seung-Hun Lee , Gia-Wei Chern

Magnetization, specific heat, and electron spin resonance (ESR) measurements are carried out to clarify the low-energy excitations for the S = 1/2 polyhedral clusters {Mo$_{72}$V$_{30}$} and {W$_{72}$V$_{30}$}. The clusters provide unique…

Strongly Correlated Electrons · Physics 2019-02-26 T. Kihara , H. Nojiri , Y. Narumi , Y. Oshima , K. Kindo , C. Heesing , J. Schnack , A. Müller

We report $^{35}$Cl NMR, ESR, $\mu$SR and specific heat measurements on the $S=1/2$ frustrated kagom\'e magnet kapellasite, $\alpha-$Cu$_3$Zn(OH)$_6$Cl$_2$, where a gapless spin liquid phase is stabilized by a set of competing exchange…

Heat-capacity (C) and ac susceptibility measurements have been performed on the spin-chain compounds, Sr3ZnRhO6 and Ca3NiMnO6, to establish their magnetic behavior and to explore whether there are magnetic frustration effects due to…

Strongly Correlated Electrons · Physics 2009-11-10 S. Rayaprol , Kausik Sengupta , E. V. Sampathkumaran , Y. Matsushita

muSR experiments on the geometrically frustrated spinel oxide, Li2Mn2O4, show the development of spin correlations over a range of length scales with decreasing temperature. Increased relaxation below 150 K is consistent with the onset of…

Strongly Correlated Electrons · Physics 2009-11-11 C. R. Wiebe , P. L. Russo , A. T. Savici , Y. J. Uemura , G. J. MacDougall , G. M. Luke , S. Kuchta , J. E. Greedan

We present the first Ga(4f) NMR study of the Cr susceptibility in the archetype of Kagome based frustrated antiferromagnets, SrCr$_{8}$Ga$_{4}$O$_{19}$. Our major finding is that the susceptibility of the frustrated lattice goes through a…

Strongly Correlated Electrons · Physics 2009-10-31 P. Mendels , A. Keren , L. Limot , M. Mekata , G. Collin , M. Horvatic