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We describe a fully broadband approach for electron spin resonance (ESR) experiments where it is possible to not only tune the magnetic field but also the frequency continuously over wide ranges. Here a metallic coplanar transmission line…

Microwave radiation applied to single-molecule magnets can induce large magnetization changes when the radiation is resonant with transitions between spin levels. These changes are interpreted as due to resonant heating of the sample by the…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 M. Bal , Jonathan R. Friedman , E. M. Rumberger , S. Shah , D. N. Hendrickson , N. Avraham , Y. Myasoedov , H. Shtrikman , E. Zeldov

Detection of electron paramagnetic resonance (EPR) using a microwave cavity resonating at a fixed frequency (between 9 and 10 GHz) remains the most popular method until now. Here, we report a cavity-less technique which makes use of only an…

Applied Physics · Physics 2020-02-06 Ushnish Chaudhuri , R. Mahendiran

Magnetic nanoparticles of gamma-Fe2O3 coated by organic molecules and suspended in liquid and solid matrices, as well as a non-diluted magnetic fluid have been studied by electron magnetic resonance (EMR) at 77-380 K. Slightly asymmetric…

Materials Science · Physics 2009-11-11 N. Noginova , F. Chen , T. Weaver , E. P. Giannelis , A. B. Bourlinos , V. A. Atsarkin

We present pulsed electrically detected magnetic resonance (EDMR) measurements at low magnetic fields using posphorus-doped silicon with natural isotope composition as a model system. Our measurements show that pulsed EDMR experiments, well…

Materials Science · Physics 2015-06-23 L. Dreher , F. Hoehne , H. Morishita , H. Huebl , M. Stutzmann , K. M. Itoh , M. S. Brandt

Electron paramagnetic resonance (EPR) spectroscopy interrogates unpaired electron spins in solids and liquids to reveal local structure and dynamics; for example, EPR has elucidated parts of the structure of protein complexes that have…

Other Condensed Matter · Physics 2012-05-08 S. Takahashi , L. -C. Brunel , D. T. Edwards , J. van Tol , G. Ramian , S. Han , M. S. Sherwin

We present pump-probe measurements on the single-molecule magnet Fe_8 with microwave pulses having a length of several nanoseconds. The microwave radiation in the experiments is located in the frequency range between 104 GHz and 118 GHz.…

Mesoscale and Nanoscale Physics · Physics 2008-02-05 S. Bahr , K. Petukhov , V. Mosser , W. Wernsdorfer

We present a broadband microwave setup for electrically detected magnetic resonance (EDMR) based on microwave antennae with the ability to apply arbitrarily shaped pulses for the excitation of electron spin resonance (ESR) and nuclear…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 F. M. Hrubesch , G. Braunbeck , A. Voss , M. Stutzmann , M. S. Brandt

The influence of the intrinsic spin of electrons on the propagation of circularly polarized waves in a magnetized plasma is considered. New eigenmodes are identified, one of which propagates below the electron cyclotron frequency, one above…

Plasma Physics · Physics 2015-05-19 A. P. Misra , G. Brodin , M. Marklund , P. K. Shukla

On-chip Electron Spin Resonance (ESR) of magnetic molecules requires the ability to precisely position nanosized samples in antinodes of the electro-magnetic field for maximal magnetic interaction. A method is developed to entrap…

Mesoscale and Nanoscale Physics · Physics 2009-08-28 N. Groll , S. Bertaina , M. Pati , N. S. Dalal , I. Chiorescu

It is shown that our multi-high-frequency (40-200 GHz) resonant cavity technique yields distortion-free high field EPR spectra for single crystal samples of the uniaxial and biaxial spin S = 10 single molecule magnets (SMMs)…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 S. Hill , S. Maccagnano , K. Park , R. M. Achey , J. M. North , N. S. Dalal

Magnetic resonance with ensembles of electron spins is nowadays performed in frequency ranges up to 240 GHz and in corresponding magnetic fields of up to 10 T. However, experiments with single electron and nuclear spins so far only reach…

The electron paramagnetic resonance (EPR) linewidths of B acceptors in Si are found to reduce dramatically in isotopically purified 28Si single crystals. Moreover, extremely narrow substructures in the EPR spectra are visible corresponding…

In this study, novel use of the electromagnetic field profile of a localized spoof surface plasmonic mode to detect electron spin resonance is being reported. The mode is supported on a resonator with a complementary metallic spiral…

Applied Physics · Physics 2021-05-04 Subhadip Roy , Anuvab Nandi , Pronoy Das , Chiranjib Mitra

We describe a simple experimental method to detect electron paramagnetic resonance (EPR) in polycrystalline 2,2-diphenyl-1-picrylhydrazyl (DPPH) sample, the standard g-marker for EPR spectroscopy, without using a cavity resonator or a…

Materials Science · Physics 2021-04-23 Lee Yong Heng , Ushnish Chaudhuri , Ramanathan Mahendiran

Electron paramagnetic resonance (EPR) spectroscopy is widely employed to characterize paramagnetic complexes. Recently, EPR combined with scanning tunneling microscopy (STM) achieved single-spin sensitivity with sub-angstrom spatial…

Mesoscale and Nanoscale Physics · Physics 2020-10-09 Tom S. Seifert , Stepan Kovarik , Dominik M. Juraschek , Nicola A. Spaldin , Pietro Gambardella , Sebastian Stepanow

Magnetic nanoparticles (MNPs) have excellent magnetic-temperature characteristic. However, current temperature measurement based on MNPs is interfered by concentration. Utilizing the electron spin resonance (ESR), we propose a highly…

Mesoscale and Nanoscale Physics · Physics 2021-08-25 Shuai Wang , Jing Zhong , Wenzhong Liu

The use of superconducting micro-resonators in combination with quantum-limited Josephson parametric amplifiers has in recent years lead to more than four orders of magnitude improvement in the sensitivity of pulsed Electron Spin Resonance…

Performing nanoscale scanning electron paramagnetic resonance (EPR) requires three essential ingredients. First, a static magnetic field together to field gradients to Zeeman split the electronic energy levels with spatial resolution.…

Mesoscale and Nanoscale Physics · Physics 2024-01-16 Carlos A. González-Gutiérrez , David García-Pons , David Zueco , María José Martínez-Pérez

We demonstrate a novel detection method for the cyclotron resonance frequency of an electron plasma in a Penning-Malmberg trap. With this technique, the electron plasma is used as an in situ diagnostic tool for measurement of the static…