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We propose a model of a heterogeneous glass forming liquid and compute the low-temperature behavior of a tagged molecule moving within it. This model exhibits stretched-exponential decay of the wavenumber-dependent, self intermediate…

Materials Science · Physics 2009-11-13 J. S. Langer , S. Mukhopadhyay

We investigate the dynamics of kinetically constrained models of glass formers by analysing the statistics of trajectories of the dynamics, or histories, using large deviation function methods. We show that, in general, these models exhibit…

Statistical Mechanics · Physics 2009-01-21 J. P. Garrahan , R. L. Jack , V. Lecomte , E. Pitard , K. van Duijvendijk , F. van Wijland

Over times shorter than that required for relaxation of enthalpy, a liquid can exhibit striking heterogeneities. The picture of these heterogeneities is complex with transient patches of rigidity, irregular yet persistent, intersected by…

Soft Condensed Matter · Physics 2010-09-30 Peter Harrowell

Despite the enormous theoretical and application interests, a fundamental understanding of the glassy dynamics remains elusive. The static properties of glassy and ordinary liquids are similar, but their dynamics are dramatically different.…

Soft Condensed Matter · Physics 2023-11-21 Puneet Pareek , Monoj Adhikari , Chandan Dasgupta , Saroj Kumar Nandi

Granular simulations are used to probe the particle scale dynamics at short, intermediate, and long time scales for gravity driven, dense granular flows down an inclined plane. On approach to the angle of repose, where motion ceases, the…

Soft Condensed Matter · Physics 2009-11-11 L. E. Silbert

We study several examples of kinetically constrained lattice models using dynamically accessible volume as an order parameter. Thereby we identify two distinct regimes exhibiting dynamical slowing, with a sharp threshold between them. These…

Statistical Mechanics · Physics 2009-11-11 Aonghus Lawlor , Paolo De Gregorio , Phil Bradley , Mauro Sellitto , Kenneth A. Dawson

We study concentrated binary colloidal suspensions, a model system which has a glass transition as the volume fraction $\phi$ of particles is increased. We use confocal microscopy to directly observe particle motion within dense samples…

Soft Condensed Matter · Physics 2011-05-20 Takayuki Narumi , Scott V. Franklin , Kenneth W. Desmond , Michio Tokuyama , Eric R. Weeks

Using molecular dynamics simulations, we have determined that the nature of dynamical heterogeneity in jammed liquids is very sensitive to short-ranged attractions. Weakly attractive systems differ little from dense hard-sphere and…

Soft Condensed Matter · Physics 2007-05-23 David R. Reichman , Eran Rabani , Phillip L. Geissler

We perform molecular dynamics simulations of a model glass-forming liquid to measure the size of kinetic heterogeneities, using a dynamic susceptibility $\chi_{\rm ss}(a, t)$ that quantifies the number of particles whose dynamics are…

Soft Condensed Matter · Physics 2014-04-04 T. K. Haxton , A. J. Liu

We study the lattice random walk dynamics in a heterogeneous space of two media separated by an interface and having different diffusivity and bias. Depending on the position of the interface, there exist two exclusive ways to model the…

Statistical Mechanics · Physics 2023-01-06 Debraj Das , Luca Giuggioli

Performing molecular dynamics simulations, we find that the structural relaxation dynamics of viscous silica, the prototype of a strong glass former, are spatially heterogeneous and cannot be understood as a statistical bond breaking…

Disordered Systems and Neural Networks · Physics 2009-11-10 Michael Vogel , Sharon C. Glotzer

Many biological processes are supported by special molecules, called motor proteins or molecular motors, that transport cellular cargoes along linear protein filaments and can reversibly associate to their tracks. Stimulated by these…

Statistical Mechanics · Physics 2021-11-17 Akriti Jindal , Anatoly B. Kolomeisky , Arvind Kumar Gupta

The dramatic slowdown of dynamics in supercooled liquids approaching the glass transition remains one of the central unresolved problems in condensed matter physics. We review approaches that attribute this slowdown to growing thermodynamic…

Soft Condensed Matter · Physics 2026-03-06 Massimo Pica Ciamarra , Jeppe C. Dyre , Edan Lerner , Matthieu Wyart

As approaching the glass transition, particle motion in liquids becomes highly heterogeneous and regions with virtually no mobility coexist with liquid-like domains. This complex dynamics is believed to be responsible for different…

Soft Condensed Matter · Physics 2018-03-28 F. Puosi , N. Jakse , A. Pasturel

We use computer simulations to study the microscopic dynamics of an athermal assembly of soft particles near the fluid-to-solid, jamming transition. Borrowing tools developed to study dynamic heterogeneity near glass transitions, we…

Materials Science · Physics 2010-06-24 Claus Heussinger , Ludovic Berthier , Jean-Louis Barrat

Non-Gaussian displacement distributions are universal predictors of dynamic heterogeneity in slowly varying environments. Here, we explore heterogeneous dynamics in supercooled liquid using molecular dynamics simulations and show the…

Soft Condensed Matter · Physics 2023-08-29 Vinay Vaibhav , Suman Dutta

We study heterogeneities in a binary Lennard-Jones system below the glass transition using molecular dynamics simulations. We identify mobile and immobile particles and measure their distribution of vibrational amplitudes. For temperatures…

Disordered Systems and Neural Networks · Physics 2013-05-29 Katharina Vollmayr-Lee , Annette Zippelius

We present a simple mechanical model for dynamic wetting phenomena. Metallic balls spread along a periodically corrugated surface simulating molecules of liquid advancing along a solid substrate. A vertical stack of balls mimics a liquid…

Condensed Matter · Physics 2009-10-28 S. F. Burlatsky , J. G. Berberian , J. Shore , W. P. Reinhardt

We study the local dynamical fluctuations in glass-forming models of particles embedded in $d$-dimensional space, in the mean-field limit of $d\to\infty$. Our analytical calculation reveals that single-particle observables, such as squared…

Disordered Systems and Neural Networks · Physics 2022-04-27 Giulio Biroli , Patrick Charbonneau , Giampaolo Folena , Yi Hu , Francesco Zamponi

We consider one component lattice gases with a local dynamics and a stationary product Bernoulli measure. We give upper and lower bounds on the diffusivity at an equilibrium point depending on the dimension and the local behavior of the…

Probability · Mathematics 2015-06-12 Jeremy Quastel , Benedek Valkó