English

Local dynamical heterogeneity in glass formers

Disordered Systems and Neural Networks 2022-04-27 v2 Soft Condensed Matter

Abstract

We study the local dynamical fluctuations in glass-forming models of particles embedded in dd-dimensional space, in the mean-field limit of dd\to\infty. Our analytical calculation reveals that single-particle observables, such as squared particle displacements, display divergent fluctuations around the dynamical (or mode-coupling) transition, due to the emergence of nontrivial correlations between displacements along different directions. This effect notably gives rise to a divergent non-Gaussian parameter, α2\alpha_2. The dd\to\infty local dynamics therefore becomes quite rich upon approaching the glass transition. The finite-dd remnant of this phenomenon further provides a long sought-after, first-principle explanation for the growth of α2\alpha_2 around the glass transition that is \emph{not based on multi-particle correlations}.

Keywords

Cite

@article{arxiv.2109.11822,
  title  = {Local dynamical heterogeneity in glass formers},
  author = {Giulio Biroli and Patrick Charbonneau and Giampaolo Folena and Yi Hu and Francesco Zamponi},
  journal= {arXiv preprint arXiv:2109.11822},
  year   = {2022}
}

Comments

5 pages, 4 figures

R2 v1 2026-06-24T06:17:19.696Z