Local dynamical heterogeneity in glass formers
Abstract
We study the local dynamical fluctuations in glass-forming models of particles embedded in -dimensional space, in the mean-field limit of . Our analytical calculation reveals that single-particle observables, such as squared particle displacements, display divergent fluctuations around the dynamical (or mode-coupling) transition, due to the emergence of nontrivial correlations between displacements along different directions. This effect notably gives rise to a divergent non-Gaussian parameter, . The local dynamics therefore becomes quite rich upon approaching the glass transition. The finite- remnant of this phenomenon further provides a long sought-after, first-principle explanation for the growth of around the glass transition that is \emph{not based on multi-particle correlations}.
Cite
@article{arxiv.2109.11822,
title = {Local dynamical heterogeneity in glass formers},
author = {Giulio Biroli and Patrick Charbonneau and Giampaolo Folena and Yi Hu and Francesco Zamponi},
journal= {arXiv preprint arXiv:2109.11822},
year = {2022}
}
Comments
5 pages, 4 figures