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Ionic behaviors, including ion distributions and hydration characteristics at solid-liquid interfaces, are important research interests in many important applications, such as electric double-layer capacitors and water lubrication. Here, we…

Chemical Physics · Physics 2025-12-08 Bowen Ai , Zekun Gong , Long Ma , Hongwen Zhang , Tianyi Sui , Yinghua Qiu

It is general wisdom that likely charged colloidal particles repel each other when suspended in liquids. This is in perfect agreement with mean field theories being developed more than 60 years ago. Accordingly, it was a big surprise when…

Soft Condensed Matter · Physics 2007-05-23 Joerg Baumgartl , Jose Luis Arauz-Lara , Clemens Bechinger

Within a general framework we study the effective, deformation-induced interaction between two colloids trapped at a fluid interface. As an application, we consider the interface deformation owing to the electrostatic field of charged…

Soft Condensed Matter · Physics 2007-05-23 Alvaro Dominguez , Martin Oettel , Siegfried Dietrich

Polyelectrolytes are commonly used to chelate multi-valent ions in aqueous solutions, playing a critical role in water softening and the prevention of mineralization. At sufficient ionic strength, ion-mediated…

Soft Condensed Matter · Physics 2023-11-21 Alec Glisman , Sriteja Mantha , Decai Yu , Eric Wasserman , Scott Backer , Zhen-Gang Wang

By a length scale analysis, we study the equilibrium interactions between two like-charge planes confining neutralising counter-ions. At large Coulombic couplings, approaching the two charged bodies leads to an unbinding of counter-ions, a…

Soft Condensed Matter · Physics 2012-10-23 E. Trizac , L. Samaj

Screening of a strongly charged macroion by its multivalent counterions can not be described in the framework of mean field Poisson-Boltzmann (PB) theory because multivalent counterions form a strongly correlated liquid (SCL) on the surface…

Soft Condensed Matter · Physics 2010-04-27 M. S. Loth , B. I. Shklovskii

We probe the electrostatic mechanism driving adsorption of polyelectrolytes onto like-charged membranes upon the addition of tri- and tetravalent counterions to a bathing monovalent salt solution. We develop a one-loop-dressed strong…

Soft Condensed Matter · Physics 2019-10-02 Sahin Buyukdagli , Rudolf Podgornik

We consider a one-dimensional model allowing analytical derivation of the effective interactions between two charged colloids. We evaluate exactly the partition function for an electroneutral salt-free suspension with dielectric jumps at…

Soft Condensed Matter · Physics 2021-04-23 Lucas Varela , Gabriel Tellez , Emmanuel Trizac

This study investigates the interplay between Strong Coupling (SC) attraction and hydration repulsion in nanoconfined water between like-charged phospholipid layers. It challenges the assumption that SC attraction requires multivalent…

Several statistical mechanical theories predict that colloidal suspensions of highly charged macroions and monovalent microions can exhibit unusual thermodynamic phase behavior when strongly deionized. Density-functional, extended…

Soft Condensed Matter · Physics 2009-11-11 A. R. Denton

Polaron formation plays a major role in determining the structural, electrical and chemical properties of ionic crystals. Using a combination of first principles calculations and scanning tunneling microscpoy/atomic force microscopy…

The Poisson-Boltzmann (PB) theory is extensively used to gain insight on charged colloids and biological systems as well as to elucidate fundamental properties of intermolecular forces. Many works were devoted in the past to study PB…

Soft Condensed Matter · Physics 2014-04-22 Dan Ben-Yaakov , David Andelman

Due to the strong correlations between multivalent counterions condensed on a macroion, the net macroion charge changes sign at some critical counterion concentration. This effect is known as the charge inversion. Near this critical…

Soft Condensed Matter · Physics 2009-11-07 T. T. Nguyen , B. I. Shklovskii

In many biological processes highly charged biomolecules are adsorbed into oppositely charged surfaces of macroions and membranes. They form strongly correlated structures close to the surface which can not be explained by the conventional…

Soft Condensed Matter · Physics 2016-03-23 Sandipan Dutta , Y. S. Jho

The interaction force between likely charged particles/surfaces is usually repulsive due to the Coulomb interaction. However, the counterintuitive like-charge attraction in electrolytes has been frequently observed in experiments, which has…

Soft Condensed Matter · Physics 2016-11-08 Pei Liu , Manman Ma , Zhenli Xu

We consider the van der Waals interaction between a pair of polymers with quenched heterogeneous sequences of local polarizabilities along their backbones, and study the effective pairwise interaction energy for both stiff polymers and…

Soft Condensed Matter · Physics 2016-06-17 Bing-Sui Lu , Ali Naji , Rudolf Podgornik

Counterion distribution around an isolated flexible polyelectrolyte in the presence of a divalent salt is evaluated using the adsorption model [M. Muthukumar, J. Chem. Phys. {\bf 120}, 9343 (2004)] that considers Bjerrum length, salt…

Soft Condensed Matter · Physics 2008-12-29 Arindam Kundagrami , M. Muthukumar

The persistence length of a single, strongly charged, stiff polyelectrolyte chain is investigated theoretically. Path integral formulation is used to obtain the effective electrostatic interaction between the monomers. We find significant…

Soft Condensed Matter · Physics 2009-11-07 Gil Ariel , David Andelman

The van der Waals potential of two atoms in the presence of an arbitrary arrangement of dispersing and absorbing magnetodielectric bodies is studied. Starting from a polarizable atom placed within a given geometry, its interaction with a…

Quantum Physics · Physics 2007-09-11 Stefan Yoshi Buhmann , Hassan Safari , Ho Trung Dung , Dirk-Gunnar Welsch

We calculate analytically the forces between two solvophobic solutes, considering a model system. We show that the effective interaction forces between two solvophobic solutes, mediated by the solvent, is attractive for short ranges, which…

Soft Condensed Matter · Physics 2015-06-01 J. Chakrabarti , Suman Dutta