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To assess electron correlation and electron-phonon coupling in the recently discovered beta-pyrochlores KOs2O6 and RbOs2O6, we have performed specific heat measurements in magnetic fields up to 14 T. We present data from high quality single…

Superconductivity · Physics 2009-11-11 M. Brühwiler , S. M. Kazakov , J. Karpinski , B. Batlogg

We report the single-crystal X-ray analysis of the structure of the pyrochlore oxide superconductor KOs$_2$O$_6$. The structure was identified as the $\beta$-pyrochlore structure with space group $Fd\bar{3}m$ and lattice constant $a$ =…

Superconductivity · Physics 2009-11-11 Jun-Ichi Yamaura , Shigeki Yonezawa , Yuji Muraoka , Zenji Hiroi

Superconductivity in the potassium osmium oxide KOs2O6 crystallizing in the beta-pyrochlore structure is studied by means of electrical resistivity, magnetic susceptibility and specific heat. It is the second superconductor in the family of…

Superconductivity · Physics 2009-11-10 Z. Hiroi , S. Yonezawa , Y. Muraoka

Chemical trends of fundamental superconducting parameters and normal-state properties are described for a family of pyrochlore oxide superconductors. Particularly, the change of Tc from 1.0 K for alpha-pyrochlore Cd2Re2O7 to 3.3 K (A = Cs),…

Superconductivity · Physics 2009-11-11 Zenji Hiroi , Jun-Ichi Yamaura , Shigeki Yonezawa , Hisatomo Harima

Rattling-induced superconductivity in the {\beta}-pyrochlore oxide KOs2O6 is investigated under high pressure up to 5 GPa. Resistivity measurements in a high-quality single crystal reveal a gradual decrease in the superconducting transition…

The superconducting properties of two beta-pyrochlore oxides, CsOs2O6 and RbOs2O6, are studied by thermodynamic and transport measurements using high-quality single crystals. It is shown that the character of superconductivity changes…

Superconductivity · Physics 2009-08-05 Yohei Nagao , Jun-ichi Yamaura , Hiroki Ogusu , Yoshihiko Okamoto , Zenji Hiroi

To elucidate the nature of the superconducting ground state of the geometrically frustrated pyrochlore KOs2O6 (Tc=9.6K), the thermal conductivity was measured down to low temperatures (~Tc/100). We found that the quasiparticle mean free…

Superconductivity · Physics 2009-11-11 Y. Kasahara , Y. Shimono , T. Shibauchi , Y. Matsuda , S. Yonezawa , Y. Muraoka , Z. Hiroi

Single crystals of KOs2O6 have been grown in a sealed quartz ampoule. Detailed single crystal X-ray diffraction studies at room temperature show Bragg peaks that violate Fd-3m symmetry. With a comparative structure refinement the structure…

Superconductivity · Physics 2009-11-11 G. Schuck , S. M. Kazakov , K. Rogacki , N. D. Zhigadlo , J. Karpinski

We report the discovery of a new pyrochlore oxide superconductor RbOs2O6. The compound crystallizes in the same beta-pyrochlore structure as the recently discovered superconductor KOs2O6, where Os atoms form a corner-sharing tetrahedral…

Superconductivity · Physics 2009-11-10 S. Yonezawa , Y. Muraoka , Y. Matsushita , Z. Hiroi

Pressure dependence of superconducting transition temperature $T_{\rm c}$ has been determined through the DC magnetic measurements under pressure up to $P$=10 GPa for $\beta$-pyrochlore oxides AOs$_2$O$_6$ with A=Cs ($T_{\rm c}$=3.3 K), Rb…

Superconductivity · Physics 2009-11-13 K. Miyoshi , Y. Takaichi , Y. Takamatsu , M. Miura , J. Takeuchi

Resistivity and specific heat have been measured on a single crystalline sample of the beta-pyrochlore oxide superconductor, KOs2O6. It is found that a second peak in specific heat, which may evidence an unknown phase transition, appears…

Superconductivity · Physics 2009-11-11 Zenji Hiroi , Shigeki Yonezawa , Jun-Ichi Yamaura , Takaki Muramatsu , Yuji Muraoka

Superconducting and normal-state properties of the beta-pyrochlore oxide KOs2O6 are studied by means of thermodynamic and transport measurements. It is shown that the superconductivity is of conventional s-wave type and lies in the…

Superconductivity · Physics 2009-11-13 Z. Hiroi , S. Yonezawa , Y. Nagao , J. Yamaura

We report the results of 87Rb NMR measurements on RbOs2O6, a new member of the family of the superconducting pyrochlore-type oxides with a critical temperature Tc = 6.4 K. In the normal state, the nuclear spin-lattice relaxation time T1…

Superconductivity · Physics 2009-11-10 K. Magishi , J. L. Gavilano , B. Pedrini , J. Hinderer , M. Weller , H. R. Ott , S. M. Kazakov , J. Karpinski

The discovery of a new beta-pyrochlore oxide superconductor CsOs2O6 with Tc = 3.3 K is reported. It is the third superconductor in the family of beta-pyrochlore oxides, following KOs2O6 with Tc = 9.6 K and RbOs2O6 with Tc = 6.3 K. The Tc of…

Superconductivity · Physics 2009-11-10 Shigeki Yonezawa , Yuji Muraoka , Zenji Hiroi

{\ss}-pyrochore KOs2O6, which shows superconductivity below ~ 9.7K, has been converted into KxOs2O6 (x < 2/3 - 1/2) electrochemically to show spin glass-like behavior below ~ 6.1K. Room temperature sample surface potential versus charge…

Superconductivity · Physics 2015-05-27 C. C. Lee , W. L. Lee , J. -Y. Lin , C. C. Tsuei , J. G. Lin , F. C. Chou

We study the influence of the rattling phonons on superconductivity in $\beta$-pyrochlore KOs$_{2}$O$_{6}$ compound based on the strong-coupling Eliashberg approach. In particular, analyzing the specific heat data we find that the rattling…

Superconductivity · Physics 2009-05-29 Jun Chang , Ilya Eremin , Peter Thalmeier

We report the basic thermodynamic properties of the new geometrically frustrated beta-pyrochlore bulk superconductor RbOs2O6 with a critical temperature Tc = 6.4 K. Specific heat measurements are performed in magnetic fields up to 12 T. The…

Superconductivity · Physics 2009-11-10 M. Brühwiler , S. M. Kazakov , N. D. Zhigadlo , J. Karpinski , B. Batlogg

Another phase transition that is probably of first order is found in the beta-pyrochlore oxide superconductor KOs2O6 with a superconducting transition temperature Tc of 9.6 K. It takes place at Tp=7.5 K in the superconducting state in a…

Superconductivity · Physics 2015-06-25 Z Hiroi , S Yonezawa , J Yamaura

The superconducting transition of the ?-pyrochlore oxide KOs2O6 with Tc = 9.60 K is studied by resistivity measurements under various magnetic fields using a high-quality single crystal. The reentrant behavior of superconductivity is…

Superconductivity · Physics 2009-11-11 Zenji Hiroi , Shigeki Yonezawa

The entire temperature dependence of the upper critical field $H_{\rm c2}$ in the $\beta$-pyrochlore KOs$_2$O$_6$ is obtained from high-field resistivity and magnetic measurements. Both techniques identically give $H_{\rm c2}(T \simeq 0…

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