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We report the systematic study of structural, magnetic and electrical transport properties of $Y_{2-x}Bi_xIr_2O_7$ (x = 0.0, 0.1, 0.2, 0.3) pyrochlore iridates. The chemical doping enhances electrical conductivity and antiferromagnetic…

Materials Science · Physics 2020-01-08 Vinod Kumar Dwivedi , Soumik Mukhopadhyay

Magnetic penetration depth ($\lambda$) in a pyrochlore superconductor KOs$_2$O$_6$ was studied by means of muon spin rotation (\msr). The temperature dependence of transverse spin relaxation rate, which is proportional to $\lambda ^{-2}$,…

Superconductivity · Physics 2009-11-10 A. Koda , W. Higemoto , K. Ohishi , S. R. Saha , R. Kadono , S. Yonezawa , Y. Muraoka , Z. Hiroi

We report a first-principles density-functional calculation of the electronic structure and properties of the recently discovered superconducting beta-pyrochlore oxide KOs_2O_6. We find that the electronic structure near the Fermi energy…

Superconductivity · Physics 2009-11-10 R. Saniz , J. E. Medvedeva , Lin-Hui Ye , T. Shishidou , A. J. Freeman

Recently new pyrochlore oxides superconductors AOs2O6 (A=K,Rb,Cs) were found and we measured the pressure dependence of magnetization up to 1.2 GPa in order to deduce the pressure effect of Tc in the three beta-pyrochlore oxides. It is…

Superconductivity · Physics 2009-11-10 Takaki Muramatsu , Shigeki Yonezawa , Yuji Muraoka , Zenji Hiroi

We investigate the temperature response of the alkali-metal rattling modes in {\beta}-pyrochlores, AOs2O6 (A = K, Rb, Cs), from the results of ab initio molecular dynamics (MD) simulations performed at 20 K, 100 K, and 300 K. Our results…

Materials Science · Physics 2013-10-25 Elvis Shoko , Vanessa K Peterson , Gordon J Kearley

We develop a general procedure for the analysis of bulk thermodynamic data of a superconductor for samples containing a metallic non-superconducting second phase. The method is based on the condensation energy and it allows the extraction…

Superconductivity · Physics 2009-11-11 M. Brühwiler , S. M. Kazakov , J. Karpinski , B. Batlogg

Two beta-pyrochlore oxide superconductors, CsOs2O6 and RbOs2O6, are studied thermodynamically by measuring specific heat on polycrystalline samples. It is found that a Sommerfeld coefficient ? is nearly equal, 20 mJ/K2 mol Os, in the two…

Superconductivity · Physics 2009-11-11 Zenji Hiroi , Shigeki Yonezawa , Takaki Muramatsu , Jun-Ichi Yamaura , Yuji Muraoka

Electronic properties of the metallic pyrochlore oxide Cd2Re2O7 are studied by means of electrical resistivity and Hall measurements. Semimetallic band structures are revealed as expected from band structure calculations. It is found that…

Strongly Correlated Electrons · Physics 2009-11-07 Z. Hiroi , M. Hanawa , Y. Muraoka , H. Harima

A new modification of KOs2O6, the representative of a new structural type (Pearson symbol aP18, a=5.5668(1)A, b=6.4519(2)A, c=7.2356(2)A, space group P-1, no.2) was synthesized employing high pressure technique. Its structure was determined…

Superconductivity · Physics 2010-03-03 S. Katrych , Q. F. Gu , Z. Bukowski , N. D. Zhigadlo , G. Krauss , J. Karpinski

Rattling-induced superconductivity in the beta-pyrochlore oxide RbOs2O6 is investigated under high pressures up to 6 GPa. Resistivity measurements in a high-quality single crystal show that the superconducting transition temperature Tc…

Superconductivity · Physics 2011-10-04 Nao Takeshita , Hiroki Ogusu , Jun-ichi Yamaura , Yoshihiko Okamoto , Zenji Hiroi

Heat capacity measurements on the recently discovered geometrically frustrated beta-pyrochlore superconductor RbOs2O6 (Tc=6.4 K) yield a Sommerfeld coefficient of 44 mJ/(molf.u. K^2). This is about 4 times larger than the one found in band…

Superconductivity · Physics 2009-11-11 M. Brühwiler , S. M. Kazakov , J. Karpinski , B. Batlogg

We investigate with a microscopic model anharmonic K-cation oscillation observed by neutron experiments in beta-pyrochlore superconductor KOs2O6, which also shows a mysterious first-order structural transition at Tp=7.5 K. We have…

Superconductivity · Physics 2015-05-20 Kazumasa Hattori , Hirokazu Tsunetsugu

High pressure effects on the superconducting transitions of beta-pyrochlore superconductors AOs2O6 (A = Cs, Rb, K) are studied by measuring resistivity under high pressures up to 10 GPa. The superconducting transition temperature Tc first…

Superconductivity · Physics 2009-11-11 T. Muramatsu , N. Takeshita , C. Terakura , H. Takagi , Y. Tokura , S. Yonezawa , Y. Muraoka , Z. Hiroi

We present a first-principles study of the electronic structure and superconducting parameters of the compounds $A$Os$_2$O$_6$ ($A$ = Na, K, Rb, and Cs) and at ambient and applied hydrostatic pressure. We find that the sensitivity of the…

Superconductivity · Physics 2007-05-23 R. Saniz , A. J. Freeman

We performed high-pressure transport measurements on high-quality single crystals of KOs2O6, a beta-pyrochlore superconductor. While the resistivity at high temperatures might approach saturation, there is no sign of saturation at low…

Superconductivity · Physics 2007-05-23 A. Akrap , E. Tutis , S. M. Kazakov , N. D. Zhigadlo , J. Karpinski , L. Forro

Being motivated by recent experimental studies, we investigate magnetic structures of the Mo pyrochlores $A_2$Mo$_2$O$_7$ ($A$= Y, Nd, and Gd) and their impact on the electronic properties. The latter are closely related with the behavior…

Strongly Correlated Electrons · Physics 2009-11-07 I. V. Solovyev

Microwave penetration depth $\lambda$ and surface resistance at 27 GHz are measured in high quality crystals of KOs$_2$O$_6$. Firm evidence for fully-gapped superconductivity is provided from $\lambda(T)$. Below the second transition at…

Superconductivity · Physics 2011-11-09 Y. Shimono , T. Shibauchi , Y. Kasahara , T. Kato , K. Hashimoto , Y. Matsuda , J. Yamaura , Y. Nagao , Z. Hiroi

We investigate the electronic structure of Sr$_2$FeMoO$_6$ combining photoemission spectroscopy with a wide range of photon energies and electronic structure calculations based on first-principle as well as model Hamiltonian approaches to…

Strongly Correlated Electrons · Physics 2007-05-23 Sugata Ray , Priya Mahadevan , Ashwani Kumar , D. D. Sarma , R. Cimino , M. Pedio , L. Ferrari , A. Pesci

Na-based osmium oxide pyrochlore was synthesized for the first time by an ion-exchange method. KOs2O6 was used as a host compound. Elelectron probe micro-analysis, synchrotron x-ray diffraction analysis, and thermo-gravimetric analysis…

Strongly Correlated Electrons · Physics 2009-11-13 Y. G. Shi , A. A. Belik , M. Tachibana , M. Tanaka , Y. Katsuya , K. Kobayashi , K. Yamaura , E. Takayama-Muromachi

We report nuclear magnetic resonance studies on the beta-pyrochlore oxide superconductor KOs2O6. The nuclear relaxation at the K sites is entirely caused by fluctuations of electric field gradient, which we ascribe to highly anharmonic low…

Superconductivity · Physics 2009-11-11 M. Yoshida , K. Arai , R. Kaido , M. Takigawa , S. Yonezawa , Y. Muraoka , Z. Hiroi