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Temperature-driven polyamorphism has been reported in various supercooled liquids and glasses. The dynamical and structural routes followed by the system during such crossovers are however not universal and appear to be related to intrinsic…

Disordered Systems and Neural Networks · Physics 2018-08-29 S. Hechler , B. Ruta , M. Stolpe , E. Pineda , Z. Evenson , O. Gross , W. Hembree , A. Bernasconi , R. Busch , I. Gallino

Based on experimental evidences we present a phenomenological description of the thermal glass transition as a dynamical phase transition. Different susceptibilities calculated on the basis of this description are in good qualitative…

Disordered Systems and Neural Networks · Physics 2016-08-16 J. K. Krüger , J. Petersson , J. Baller , M. Henkel

A core-softened model of a glass forming fluid is numerically studied in the limit of very low temperatures. The model shows two qualitatively different behaviors depending on the strength of the attraction between particles. For no or low…

Statistical Mechanics · Physics 2009-11-07 E. A. Jagla

The thermodynamic and kinetic anomalies of supercooled liquids are analyzed from the perspective of energy landscapes. A mean field model, a generalized random energy model of liquids is developed, which exhibits a dynamical transition of…

Soft Condensed Matter · Physics 2009-11-10 Masaki Sasai

We analyse numerically thermal fluctuations of the static overlap between equilibrium configurations in a glass-forming liquid approaching the glass transition. We find that the emergence of slow dynamics near the onset temperature…

Statistical Mechanics · Physics 2013-08-23 Ludovic Berthier

We review the available experimental information on the thermodynamic properties of supercooled ordinary and heavy water and demonstrate the possibility of modeling these thermodynamic properties on a theoretical basis. We show that by…

Chemical Physics · Physics 2013-02-25 V. Holten , C. E. Bertrand , M. A. Anisimov , J. V. Sengers

An equilibrated model glass-forming liquid is studied by mapping successive configurations produced by molecular dynamics simulation onto a time series of inherent structures (local minima in the potential energy). Using this ``inherent…

Soft Condensed Matter · Physics 2012-03-27 Thomas B. Schroeder , Srikanth Sastry , Jeppe C. Dyre , Sharon C. Glotzer

The description of molecular motion by macroscopic hydrodynamics has a long and continuing history. The Stokes-Einstein relation between the diffusion coefficient of a solute and the solvent viscosity predicted using macroscopic continuum…

Disordered Systems and Neural Networks · Physics 2007-05-23 Xiaoyu Xia , Peter G. Wolynes

The fragility, that controls the temperature-dependent viscous properties of liquids as the glass transition is approached, in various glass-forming liquids with different atomic interactions and densities is investigated by molecular…

Soft Condensed Matter · Physics 2016-08-03 Lijin Wang , Pengfei Guan , W. H. Wang

In this paper, we discuss theoretically the behavior of the four point nonlinear susceptibility and its associated correlation length for supercooled liquids close to the Mode Coupling instability temperature $T_c$. We work in the…

Disordered Systems and Neural Networks · Physics 2009-10-31 Silvio Franz , Giorgio Parisi

We present a mean-field theory of a coarse-grained model of a super-cooled liquid in which relaxation occurs via local plastic rearrangements. Local relaxation can be induced by thermal fluctuations or by the long-range elastic consequences…

Soft Condensed Matter · Physics 2023-12-07 Joseph W. Baron , Giulio Biroli

The dynamics of supercooled liquid and glassy systems are usually studied within the Lagrangian representation, in which the positions and velocities of distinguishable interacting particles are followed. Within this representation,…

Disordered Systems and Neural Networks · Physics 2009-09-28 Claudio Chamon , Leticia F. Cugliandolo , Gabriel Fabricius , Jose Luis Iguain , Eric R. Weeks

We introduce the ideal Gaussian glass-forming system as a model to describe the thermodynamics and dynamics of supercooled liquids on a local scale in terms of the properties of the potential energy landscape (PEL). The first ingredient is…

Materials Science · Physics 2009-11-13 A. Heuer , A. Saksaengwijit

In this work, we study the nature of transitions between inherent structures of a two-dimensional model supercooled liquid. We demonstrate that these transitions occur predominately along a small number of directions on the energy…

Statistical Mechanics · Physics 2013-03-12 Glen M. Hocky , David R. Reichman

The transition from a flowing to a static state in a granular material is studied using large-scale, 3D particle simulations. Similar to glasses, this transition is manifested in the development of a plateau in the contact normal force…

Statistical Mechanics · Physics 2007-05-23 L. E. Silbert , D. Ertas , G. S. Grest , T. C. Halsey , D. Levine

We use light microscopy to investigate the aging dynamics of a glass made of closely packed soft spheres, following a rapid transition from a fluid to a solid-like state. By measuring time-resolved, coarse-grained displacements fields, we…

Soft Condensed Matter · Physics 2009-11-13 Sylvain Mazoyer , Luca Cipelletti , Laurence Ramos

As one increases the concentration of a colloidal suspension, the system exhibits a dramatic increase in viscosity. Structurally, the system resembles a liquid, yet motions within the suspension are slow enough that it can be considered…

Soft Condensed Matter · Physics 2012-05-22 Gary L. Hunter , Eric R. Weeks

As liquids approach the glass transition temperature, dynamical heterogeneity emerges as a crucial universal feature of their behavior. Dynamic facilitation, where local motion triggers further motion nearby, plays a major role in this…

When a liquid is cooled below its melting temperature it usually crystallizes. However, if the quenching rate is fast enough, it is possible that the system remains in a disordered state, progressively losing its fluidity upon further…

Disordered Systems and Neural Networks · Physics 2009-11-10 Tullio Scopigno , Giancarlo Ruocco , Francesco Sette , Giulio Monaco

We study the dynamical melting of "hot" one-dimensional many-body localized systems. As disorder is weakened below a critical value these non-thermal quantum glasses melt via a continuous dynamical phase transition into classical thermal…

Disordered Systems and Neural Networks · Physics 2015-09-23 Andrew C. Potter , Romain Vasseur , S. A. Parameswaran
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