English

Elastoplasticity Mediates Dynamical Heterogeneity Below the Mode-Coupling Temperature

Soft Condensed Matter 2021-07-28 v2 Statistical Mechanics Chemical Physics

Abstract

As liquids approach the glass transition temperature, dynamical heterogeneity emerges as a crucial universal feature of their behavior. Dynamic facilitation, where local motion triggers further motion nearby, plays a major role in this phenomenon. Here we show that long-range, elastically-mediated facilitation appears below the mode-coupling temperature, adding to the short-range component present at all temperatures. Our results suggest deep connections between the supercooled liquid and glass states, and pave the way for a deeper understanding of dynamical heterogeneity in glassy systems.

Keywords

Cite

@article{arxiv.2103.01852,
  title  = {Elastoplasticity Mediates Dynamical Heterogeneity Below the Mode-Coupling Temperature},
  author = {Rahul N. Chacko and François P. Landes and Giulio Biroli and Olivier Dauchot and Andrea J. Liu and David R. Reichman},
  journal= {arXiv preprint arXiv:2103.01852},
  year   = {2021}
}

Comments

6 pages, 4 figures. SM included as ancillary

R2 v1 2026-06-23T23:40:09.482Z