Elastoplasticity Mediates Dynamical Heterogeneity Below the Mode-Coupling Temperature
Soft Condensed Matter
2021-07-28 v2 Statistical Mechanics
Chemical Physics
Abstract
As liquids approach the glass transition temperature, dynamical heterogeneity emerges as a crucial universal feature of their behavior. Dynamic facilitation, where local motion triggers further motion nearby, plays a major role in this phenomenon. Here we show that long-range, elastically-mediated facilitation appears below the mode-coupling temperature, adding to the short-range component present at all temperatures. Our results suggest deep connections between the supercooled liquid and glass states, and pave the way for a deeper understanding of dynamical heterogeneity in glassy systems.
Cite
@article{arxiv.2103.01852,
title = {Elastoplasticity Mediates Dynamical Heterogeneity Below the Mode-Coupling Temperature},
author = {Rahul N. Chacko and François P. Landes and Giulio Biroli and Olivier Dauchot and Andrea J. Liu and David R. Reichman},
journal= {arXiv preprint arXiv:2103.01852},
year = {2021}
}
Comments
6 pages, 4 figures. SM included as ancillary