English

Direct numerical analysis of dynamic facilitation in glass-forming liquids

Soft Condensed Matter 2024-06-25 v2 Disordered Systems and Neural Networks Materials Science Statistical Mechanics

Abstract

We propose a computational strategy to quantify the temperature evolution of the timescales and lengthscales over which dynamic facilitation affects the relaxation dynamics of glass-forming liquids at low temperatures, that requires no assumption about the nature of the dynamics. In two glass models, we find that dynamic facilitation depends strongly on temperature, leading to a subdiffusive spreading of relaxation events which we characterize using a temperature-dependent dynamic exponent. We also establish that this temperature evolution represents a major contribution to the increase of the structural relaxation time.

Keywords

Cite

@article{arxiv.2310.16935,
  title  = {Direct numerical analysis of dynamic facilitation in glass-forming liquids},
  author = {Cecilia Herrero and Ludovic Berthier},
  journal= {arXiv preprint arXiv:2310.16935},
  year   = {2024}
}