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Solar cells based on a light absorbing layer of the organometal halide perovskite CH$_3$NH$_3$PbI$_3$ have recently reached 15% conversion efficiency, though how these materials work remains largely unknown. We analyse the electronic…

Materials Science · Physics 2014-04-24 Federico Brivio , Keith T. Butler , Aron Walsh , Mark van Schilfgaarde

The recent advances in nanowire (NW) growth technology have made possible the growth of more complex structures such as core-multi-shell (CMS) NWs. We propose the approach for calculation of electron subbands in cylindrical CMS NWs within…

Mesoscale and Nanoscale Physics · Physics 2021-01-19 A. O. Rudakov , I. A. Kokurin

A modified core-to-valence band maximum approach is applied to calculate band offsets of strained III/V semiconductor hetero junctions. The method is used for the analysis of (In,Ga)As/GaAs/Ga(As,Sb) multi-quantum well structures. The…

Materials Science · Physics 2019-01-04 Jan Oliver Oelerich , Maria J. Weseloh , Kerstin Volz , Stephan W. Koch

The electronic band structure of CaSnN$_2$ in the wurtzite-based $Pna2_1$ structure is calculated using the Quasiparticle Self-consistent (QS)GW$^{BSE}$ method, including ladder diagrams in the screened Coulomb interaction W$^{BSE}$ and is…

Materials Science · Physics 2026-04-20 Ilteris K. Turan , Sarker Md. Sadman , Walter R. L. Lambrecht

We report calculated, electronic and related properties of wurtzite and zinc blende gallium nitrides (w-GaN, zb-GaN). We employed a local density approximation (LDA) potential and the linear combination of atomic orbital (LCAO) formalism.…

Although the GW approximation is recognized as one of the most accurate theories for predicting materials excited states properties, scaling up conventional GW calculations for large systems remains a major challenge. We present a powerful…

Computational Physics · Physics 2018-03-28 Weiwei Gao , Weiyi Xia , Xiang Gao , Peihong Zhang

We use fully self-consistent GW calculations on diamond and silicon carbide to reparametrize the Heyd-Scuseria-Ernzerhof exact exchange density functional for use in band structure calculations of semiconductors and insulators. We show that…

Mesoscale and Nanoscale Physics · Physics 2015-08-05 V. Zólyomi , J. Kürti

We propose an efficient reduced-order technique for electronic structure calculations of semiconductor nanostructures, suited for inclusion in full-band quantum transport simulators. The model is based on the linear combination of bulk…

Mesoscale and Nanoscale Physics · Physics 2013-04-04 Francesco Bertazzi , Xiangyu Zhou , Michele Goano , Enrico Bellotti , Giovanni Ghione

Accurate band offsets are essential for predictive continuum modeling of nanostructures such as quantum wells and quantum dots formed in strained Si/Si1-xGex and Ge/Si1-xGex heterostructures. Experimental offset data for these systems…

Mesoscale and Nanoscale Physics · Physics 2026-03-16 Nathaniel M. Vegh , Pericles Philippopoulos , Raphaël J. Prentki , Wanting Zhang , Yu Zhu , Félix Beaudoin , Hong Guo

We present theoretical calculations for the spectral functions and single-particle densities of states of the two-dimensional electron gas in semiconductor quantum wells at different electron densities using the GW+cumulant method. We…

Mesoscale and Nanoscale Physics · Physics 2015-06-18 Johannes Lischner , Derek Vigil-Fowler , Steven G. Louie

Atomic effective pseudopotentials enable atomistic calculations at the level of accuracy of density functional theory for semiconductor nanostructures with up to fifty thousand atoms. Since they are directly derived from ab-initio…

Materials Science · Physics 2024-03-14 Surender Kumar , Hanh Bui , Gabriel Bester

Ab initio electronic structure calculations of two-dimensional layered structures are typically performed using codes that were developed for three-dimensional structures, which are periodic in all three directions. The introduction of a…

Strongly Correlated Electrons · Physics 2016-06-22 Paolo E. Trevisanutto , Giovanni Vignale

Nanowires with a GaSb core and an InAs shell (and the inverted structure) are interesting for studies of electron-hole hybridization and interaction effects due to the bulk broken band-gap alignment at the material interface. We have used…

Mesoscale and Nanoscale Physics · Physics 2017-04-03 Florinda Viñas , H. Q. Xu , Martin Leijnse

X-ray photoelectron spectroscopy (XPS) measures electron removal energies, providing direct access to core and valence electron binding energies, hence probing the electronic structure. In this work, we benchmark for the first time the ab…

Other Condensed Matter · Physics 2023-10-11 Iskander Mukatayev , Benoît Sklénard , Valerio Olevano , Jing Li

We present a quasiparticle self-consistent $GW$ (QSGW) implementation for periodic systems based on crystalline Gaussian basis sets. Our QSGW approach is based on a full-frequency analytic continuation GW scheme with Brillouin zone sampling…

Chemical Physics · Physics 2022-12-21 Jincheng Lei , Tianyu Zhu

A study is presented of the electronic band structure and optical absorption spectrum of monolayer WSe$_2$ using an all-electron quasiparticle self-consistent $GW$ approach, QS$G\hat W$, in which the screened Coulomb interaction $\hat W$ is…

Materials Science · Physics 2024-02-29 Niloufar Dadkhah , Walter R. L. Lambrecht

The electronic band structure of SrTiO$_3$ is investigated in the all-electron QS$GW$ approximation. Unlike previous pseudopotential based QS$GW$ or single-shot $G_0W_0$ calculations, the gap is found to be significantly overestimated…

Materials Science · Physics 2018-01-31 Churna Bhandari , Mark van Schilfgaarde , Takao Kotani , Walter R. L. Lambrecht

Quasiparticle spectra of potentially half-metallic Co2MnSi and Co2FeSi Heusler compounds have been calculated within the one-shot GW approximation in an all-electron framework without adjustable parameters. For Co2FeSi the many-body…

Materials Science · Physics 2013-01-04 Markus Meinert , Christoph Friedrich , Günter Reiss , Stefan Blügel

We present a combined experimental and theoretical analysis of the evolution of the near-band gap electronic and optical properties of Si$_{x}$Ge$_{1-x-y}$Sn$_{y}$ alloys lattice-matched to Ge and GaAs substrates. We perform…

A multiband empirical tight-binding model for group-III-nitride semiconductors with a wurtzite structure has been developed and applied to both bulk systems and embedded quantum dots. As a minimal basis set we assume one s-orbital and three…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 Daniel Mourad , Stefan Barthel , Gerd Czycholl