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We present the results of theoretical investigation on the electronic structure, bonding nature and ground state properties of Th$_2$Al and Th$_2$AlH$_4$ using generalized-gradient-corrected first-principles full-potential…

Materials Science · Physics 2009-11-07 P. Vajeeston , R. Vidya , P. Ravindran , H. Fjellvåg , A. Kjekshus , A. Skjeltorp

In electrochemical systems, the structure of electrical double layers (EDLs) near electrode surfaces is crucial for energy conversion and storage functions. While the electrodes in real-world systems are usually heterogeneous, to date the…

Photoionization from atom-C60 hybrid levels in halogen endufullerene molecules, Cl@C60, Br@C60 and I@C60, are calculated using a linear response density functional method. Both the ordinary electron-configuration where the open shell…

Atomic and Molecular Clusters · Physics 2021-06-08 Dakota Shields , Ruma De , Esam Ali , Mohamed E Madjet , Steven T Manson , Himadri S. Chakraborty

Physical quilities such as electronic, mechanical, thermal, and optical properties of Al and P codoped silicene forming AlSi$_6$P nanosheets are investigated by first-principle calculations within density functional theory. A particular…

Mesoscale and Nanoscale Physics · Physics 2023-07-18 Nzar Rauf Abdullah , Hunar Omar Rashid , Andrei Manolescu , Vidar Gudmundsson

Three fundamentally different electronic structures for 3d electron states in LaCoO3, discussed in the current literature, have been presented. We are in favour of the localized electron atomic- like approach that yields the discrete energy…

Strongly Correlated Electrons · Physics 2007-05-23 Z. Ropka , R. J. Radwanski

A polymorph of RuI$_3$ synthesized under high pressure was found to have a two-layered honeycomb structure. The resistivity of RuI$_3$ exhibits a semimetallic behavior, in contrast to insulating properties in $\alpha$-RuCl$_3$. In addition,…

In this paper, we investigate the ground state properties of the $\rm{RMnO}_3/\rm{AMnO}_3$ ($\rm{RMO/AMO}$) heterostructures (R=trivalent cation, and A=divalent cation) by using a two-orbital double-exchange model supplemented by the…

Strongly Correlated Electrons · Physics 2015-05-13 Rong Yu , Seiji Yunoki , Shuai Dong , Elbio Dagotto

In the isostructural oxides Ca3CoMO6 (M = Co, Rh, Ir), the CoMO6 chains made up of face-sharing CoO6 trigonal prisms and MO6 octahedra are separated by Ca atoms. We analyzed the magnetic and electronic properties of these oxides on the…

Strongly Correlated Electrons · Physics 2011-01-05 Yuemei Zhang , Erjun Kan , Hongjun Xiang , Antoine Villesuzanne , Myung-Hwan Whangbo

Ionic behaviors, including ion distributions and hydration characteristics at solid-liquid interfaces, are important research interests in many important applications, such as electric double-layer capacitors and water lubrication. Here, we…

Chemical Physics · Physics 2025-12-08 Bowen Ai , Zekun Gong , Long Ma , Hongwen Zhang , Tianyi Sui , Yinghua Qiu

Density-functional studies of the electronic structures and exchange interaction parameters have been performed for a series of ferromagnetic full Heusler alloys of general formula Co$_2$MnZ (Z = Ga, Si, Ge, Sn), Rh$_2$MnZ (Z = Ge, Sn, Pb),…

Materials Science · Physics 2009-11-10 Yasemin Kurtulus , Richard Dronskowski , German Samolyuk , Vladimir P. Antropov

Lithium metasilicate (Li2SiO3) has attracted considerable interest as a promising electrolyte material for potential use in lithium batteries. However, its electronic properties are still not thoroughly understood. In this work, density…

Computational Physics · Physics 2020-01-22 Nguyen Thi Han , Vo Khuong Dien , Ngoc Thanh Thuy Tran , Duy Khanh Nguyen , Wu-Pei Su , Ming-Fa Lin

The Electron Localization Function (ELF) by Becke and Edgecombe [J. Chem. Phys. {\bf 92}, 5397 (1990)] is routinely adopted as a descriptor of atomic shells and covalent bonds. Since the ELF and its related quantities find useful…

Materials Science · Physics 2018-08-29 Stefano Pittalis , Daniele Varsano , Alain Delgado , Carlo Andrea Rozzi

In this paper, density functional theory calculations are used to explore the electronic and atomic reconstruction at interfaces between III-III/I-V oxides. In particular, at these interfaces, two dimensional electron gases (2DEGs) with…

Materials Science · Physics 2012-06-06 Valentino R. Cooper

Alkali-doped fullerides A$_n$C$_{60}$ show a remarkably wide range of electronic phases in function of A= Li, Na, K, Rb, Cs and the degree of doping, $n=1-5$. While the presence of strong electron correlations is well established, recent…

Strongly Correlated Electrons · Physics 2016-10-10 Naoya Iwahara , Liviu F. Chibotaru

Hydrogenated silicenes possess peculiar properties owing to the strong H-Si bonds, as revealed by an investigation using first principles calculations. The various charge distributions, bond lengths, energy bands, and densities of states…

Materials Science · Physics 2015-10-28 Shih-Yang Lin , Shen-Lin Chang , Ngoc Thanh Thuy Tran , Po-Hua Yang , Ming-Fa Lin

Analysis of the electron density distribution in clusters composed of hydrogen fluoride, water, and ammonia molecules, especially within the hydrogen-bond domains, reveals the existence of both \sigma- and \pi-binding between molecules. The…

Chemical Physics · Physics 2024-05-08 Yulia V. Novakovskaya

We present the results of self-consistent calculations of the electronic shell and supershell structure for clusters having up to 6000 valence electrons. The ionic background is described in terms of a homogeneous jellium. The calculations…

Condensed Matter · Physics 2009-10-28 Erik Koch , Olle Gunnarsson

We have carried out a comparative theoretical study of the electronic structure of the novel one-dimensional Ca$_3$CoRhO$_6$ and Ca$_3$FeRhO$_6$ systems. The insulating antiferromagnetic state for the Ca$_3$FeRhO$_6$ can be well explained…

Strongly Correlated Electrons · Physics 2007-06-21 Hua Wu , Z. Hu , D. I. Khomskii , L. H. Tjeng

The organization of water molecules and ions between charged mineral surfaces determines the stability of colloidal suspensions and the strength of phase-separated particulate gels. In this article we assemble a density functional that…

Soft Condensed Matter · Physics 2024-05-15 Thomas Petersen

It is of great importance to develop inorganic solid electrolytes with high ionic conductivity, thus enabling solid state Li-ion batteries to address the notorious safety issue about the current technology due to use of highly flammable…

Chemical Physics · Physics 2017-07-17 Zhuo Wang , Min Jie Xuan , Hong Jie Xu , Guosheng Shao