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The liquid-vapour phase transition near a weakly attractive surface is studied by simulations of the coexistence curves of water in hydrophobic pores. There is a pronounced gradual density depletion of the liquid phase near the surface…

Statistical Mechanics · Physics 2009-11-10 I. Brovchenko , A. Geiger , A. Oleinikova

The gas-liquid phase transition of the three-dimensional Lennard-Jones particles system is studied by molecular dynamics simulations. The gas and liquid densities in the coexisting state are determined with high accuracy. The critical point…

Statistical Mechanics · Physics 2013-11-28 Hiroshi Watanabe , Nobuyasu Ito , Chin-Kun Hu

The density profile and Gibbs adsorption of a near-critical fluid confined between two identical planar walls is studied by means of Monte Carlo simulation and by density functional theory for a Lennard-Jones fluid. By reducing the strength…

Statistical Mechanics · Physics 2016-08-31 A. Maciolek , R. Evans , N. B. Wilding

Depletion of the liquid density near a solid surface with a weak long-range fluid-surface interaction was studied by computer simulations of the liquid-vapor coexistence of a LJ fluid confined in slitlike pores. In a wide temperature range…

Statistical Mechanics · Physics 2015-06-25 A. Oleinikova , I. Brovchenko , A. Geiger

Close to a solid surface, the properties of a fluid deviate significantly from their bulk values. In this context, we study the surface adsorption profiles of a symmetric binary liquid confined to a slit pore by means of molecular dynamics…

Soft Condensed Matter · Physics 2025-01-15 Sutapa Roy , Felix Höfling

We report a theoretical and simulation study of the drying and wetting phase transitions of a truncated Lennard-Jones fluid at a flat structureless wall. Binding potential calculations predict that the nature of these transitions depends on…

Statistical Mechanics · Physics 2017-09-13 Robert Evans , Maria C. Stewart , Nigel B. Wilding

We present the results of a Molecular Dynamics computer simulation of a binary Lennard-Jones liquid confined in a narrow pore. The surface of the pore has an amorphous structure similar to that of the confined liquid. We find that the…

Statistical Mechanics · Physics 2007-05-23 Peter Scheidler , Walter Kob , Kurt Binder

The approach of global isomorphism between the fluid and the Ising model is applied to obtain an expression for the surface tension of the Lennard-Jones fluid on the basis of the information about the Ising model. This is done in a broad…

Chemical Physics · Physics 2018-12-24 A. Maslechko , K. Glavatskiy , V. Kulinskii

We study the surface critical behavior of semi-infinite systems belonging to the bulk universality class of the Ising model. Special attention is paid to the local behavior of experimentally relevant quantities such as the order parameter…

Condensed Matter · Physics 2009-10-28 A. Ciach , U. Ritschel

The properties of a fluid, or Ising magnet, confined in a $L \times \infty$ geometry with opposing surface fields at the walls are studied by density matrix renormalization techniques. In particular we focus on the effect of gravity on the…

Statistical Mechanics · Physics 2009-10-30 Enrico Carlon , Andrzej Drzewinski

Water's unique anomalies are vital in various applications and biological processes, yet the molecular mechanisms behind these anomalies remain debated, particularly in the metastable liquid phase under supercooling and stretching…

Statistical Mechanics · Physics 2024-05-17 Luis Enrique Coronas , Giancarlo Franzese

Wetting and drying of a rigid substrate by a Lennard-Jones fluid in molecular dynamics simulations is reported. The size of the substrate particles, being smaller than the fluid particles in former simulations, is now taken to be equal to,…

Soft Condensed Matter · Physics 2015-06-25 C. Bruin

We consider the contact process near an extended surface defect, where the local control parameter deviates from the bulk one by an amount of $\lambda(l)-\lambda(\infty) = A l^{-s}$, $l$ being the distance from the surface. We concentrate…

Statistical Mechanics · Physics 2018-01-12 R. Juhász , F. Iglói

The behavior of energy polydisperse $2d$ Lennard-Jones fluid (in thin-film geometry) is studied subjected to linear flow field using molecular dynamics simulations. By considering neutral and selective substrates we systematically explore…

Soft Condensed Matter · Physics 2020-07-01 Lenin S. Shagolsem

Using a liquid-state approach based on Ornstein-Zernike equations, we study the behavior of a fluid inside a porous disordered matrix near the liquid-gas critical point.The results obtained within various standard approximation schemes such…

Condensed Matter · Physics 2009-10-28 E. Pitard , M. L. Rosinberg , G. Stell , G. Tarjus

We report a detailed simulation and classical density functional theory study of the drying transition in a realistic model fluid at a smooth substrate. This transition (in which the contact angle $\theta\to 180^\circ$) is shown to be…

Statistical Mechanics · Physics 2016-10-26 Robert Evans , Maria C. Stewart , Nigel B. Wilding

We present a computer simulation study of a (6,12)-Lennard-Jones fluid confined to a slit pore, formed by two uniform planes. These interact via (3,9)-Lennard-Jones potential with the fluid particles. When the fluid approaches the…

Soft Condensed Matter · Physics 2009-02-20 N. Gribova , H. Maleki , A. Arnold , C. Holm , T. Schilling

We examine the phase behavior of a quasi-one-dimensional system of hard squares with side-length $\sigma$, where the particles are confined between two parallel walls and only nearest neighbor interactions occur. As in our previous work…

Statistical Mechanics · Physics 2017-05-03 Peter Gurin , Gerardo Odriozola , Szabolcs Varga

The influence of temperature on interfacial fluid slip, as measured by molecular-dynamics simulations of a Couette flow comprising a Lennard-Jones fluid and rigid crystalline walls, is examined as a function of the fluid-solid interaction…

Fluid Dynamics · Physics 2021-06-30 Thiago F. Viscondi , Adriano Grigolo , Iberê L. Caldas , Julio R. Meneghini

Linearly-sloped or `ramp' potentials belong to a class of core-softened models which possess a liquid-liquid critical point (LLCP) in addition to the usual liquid-gas critical point. Furthermore they exhibit thermodynamic anomalies in the…

Statistical Mechanics · Physics 2009-11-11 Helen M. Gibson , Nigel B. Wilding
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