Related papers: Comment on "Hole digging in ensembles of tunneling…
Reply to the Comment of J.J. Alonso and J.F. Fernandez on the paper "'Hole-digging' in ensembles of tunneling molecular magnets" of I.S. Tupitsyn, P.C.E. Stamp and N.V. Prokof'ev (Phys. Rev. B 69, 132406, (2004)).
We study the relaxation of interacting single--molecule magnets (SMMs) in both spatially ordered and disordered systems. The tunneling window is assumed to be, as in Fe8, much narrower than the dipolar field spread. We show that relaxation…
The nuclear spin-mediated quantum relaxation of ensembles of tunneling magnetic molecules causes a 'hole' to appear in the distribution of internal fields in the system. The form of this hole, and its time evolution, are studied using Monte…
Below 360 mK, Fe8 magnetic molecular clusters are in the pure quantum relaxation regime. We showed recently that the predicted ``square-root time'' relaxation is obeyed, allowing us to develop a new method for watching the evolution of the…
We argue that to explain recent resonant tunneling experiments on crystals of Mn$_{12}$ and Fe$_8$, particularly in the low-T limit, one must invoke dynamic nuclear spin and dipolar interactions. We show the low-$T$, short-time relaxation…
Below 360 mK, Fe magnetic molecular clusters are in the pure quantum relaxation regime and we show that the predicted square-root time relaxation is obeyed, allowing us to develop a new method for watching the evolution of the distribution…
A new approach is used that allows to describe the magnetic molecules main properties in a direct and simple way. Results obtained for the Fe8 cluster show good agreement with the experimental data.
We model magnetization processes that take place through tunneling in crystals of single-molecule magnets, such as Mn_12 and Fe_8. These processes take place when a field H is applied after quenching to very low temperatures. Magnetic…
We study the magnetic relaxation of a system of localized spins interacting through weak dipole interactions, at a temperature large with respect to the ordering temperature but low with respect to the crystal field level splitting. The…
Response to the Comment by Bellessa (arXiv:cond-mat/0006441).
The spin Hamiltonian that describes the molecular magnet Fe$_8$ has biaxial symmetry with mutually perpendicular easy, medium, and hard magnetic axes. Previous calculations of the ground state tunnel splittings in the presence of a magnetic…
We report results from Monte Carlo simulations of systems of magnetic dipoles that relax through quantum tunneling, much as Fe_8 crystals at very low temperature.For short times, a hole develops in suitably defined magnetic field…
Measurements of proton NMR and the spin lattice relaxation rate 1/T1 in the octanuclear iron (III) cluster [Fe8(N3C6H15)6O2(OH)12][Br8 9H2O], in short Fe8, have been performed at 1.5 K in a powder sample aligned along the main anisotropy z…
Current theories still fail to give a satisfactory explanation of the observed quantum phenomena in the relaxation of the magnetisation of the molecular cluster Mn12 acetate. In the very low temperature regime, Prokof'ev and Stamp recently…
Spin tunneling in the particular case of the magnetic molecular cluster octanuclear iron(III), Fe8, is treated by an effective Hamiltonian that allows for an angle-based description of the process. The presence of an external magnetic field…
The Comment of A. Pelissetto and E. Vicari (cond-mat/0610113) on our article (cond-mat/0609285) is based on misunderstandings of this article as well as on unfounded implicit assumptions. We clarify here the controversial points and show…
Magnetic relaxation in molecular magnets under a sweeping field is studied by taking into account local stray fields. It is found that the randomness of local stray field leads to a distribution of the relaxation rate which subsequently…
It is shown that a single molecular magnet placed in a rapidly oscillating magnetic field displays the phenomenon of quenching of tunneling processes. The results open a way to manipulate the quantum states of molecular magnets by means of…
The low temperature relaxation of the magnetization in magnetic molecular solids such as Fe$_8$ is studied using Monte Carlo simulations. A set of rate equations is developed to understand the simulations, and the results are compared. The…
The perfect quenching of spin tunneling first predicted for a model with biaxial symmetry, and recently observed in the magnetic molecule Fe_8, is further studied using the discrete phase integral (or Wentzel-Kramers-Brillouin) method. The…