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Single-walled carbon nanotubes are strongly correlated systems with large Coulomb repulsion between two electrons occupying the same $p_z$ orbital. Within a molecular Hamiltonian appropriate for correlated $\pi$-electron systems, we show…

Materials Science · Physics 2009-02-15 Zhendong Wang , Demetra Psiachos , Roberto F. Badilla , Sumit Mazumdar

We report first-principles calculations of the effects of quasiparticle self-energy and electron-hole interaction on the optical properties of single-walled BN nanotubes. Excitonic effects are shown to be even more important in BN nanotubes…

Materials Science · Physics 2007-08-23 Cheol-Hwan Park , Catalin D. Spataru , Steven G. Louie

One- and two-photon luminescence excitation spectroscopy showed a series of distinct excitonic states in single-walled carbon nanotubes. The energy splitting between one- and two-photon-active exciton states of different wavefunction…

Materials Science · Physics 2007-05-23 J. Maultzsch , R. Pomraenke , S. Reich , E. Chang , D. Prezzi , A. Ruini , E. Molinari , M. S. Strano , C. Thomsen , C. Lienau

We present a quantitative theory of optical absorption polarized transverse to the tube axes in semiconducting single-walled carbon nanotubes. Transverse optical absorption in semiconducting single-walled carbon nanotubes is to an exciton…

Materials Science · Physics 2009-11-13 Zhendong Wang , Hongbo Zhao , Sumit Mazumdar

Many-electron effects often dramatically modify the properties of reduced dimensional systems. We report calculations, based on an many-electron Green's function approach, of electron-hole interaction effects on the optical spectra of…

Materials Science · Physics 2009-11-10 Catalin D. Spataru , Sohrab Ismail-Beigi , Lorin X. Benedict , Steven G. Louie

The properties of excitons in semiconducting single-walled carbon nanotubes (SWCNTs), isolated in vacuum or a medium, and their contributions to the optical spectra of nanotubes are studied within the elementary potential model, in which an…

Materials Science · Physics 2010-12-15 Oleksii A. Smyrnov

Simultaneous photoluminescence and photocurrent measurements on individual single-walled carbon nanotubes reveal spontaneous dissociation of excitons into free electron-hole pairs. Correlation of luminescence intensity and photocurrent…

Mesoscale and Nanoscale Physics · Physics 2014-03-19 Y. Kumamoto , M. Yoshida , A. Ishii , A. Yokoyama , T. Shimada , Y. K. Kato

Exciton effects are studied in single-wall boron-nitride nanotubes. The Coulomb interaction dependence of the band gap, the optical gap, and the binding energy of excitons are discussed. The optical gap of the (5,0) nanotube is about 6eV at…

Materials Science · Physics 2009-07-07 Kikuo Harigaya

We study theoretically the interactions of excitonic states with surface electromagnetic modes of small-diameter (~1 nm) semiconducting single-walled carbon nanotubes. We show that these interactions can result in strong…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 I. V. Bondarev , K. Tatur , L. M. Woods

We develop a scaling relationship between the exciton binding energy and the external dielectric function in carbon nanotubes. We show that the electron-electron and electron-hole interaction energies are strongly affected by screening yet…

We use the macroscopic quantum electrodynamics approach suitable for absorbing and dispersing media to study the properties and role of collective surface excitations --- excitons and plasmons --- in single-wall and double-wall carbon…

Mesoscale and Nanoscale Physics · Physics 2017-08-14 I. V. Bondarev , L. M. Woods , A. Popescu

We present direct experimental observation of exciton-phonon bound states in the photoluminescence excitation spectra of isolated single walled carbon nanotubes in aqueous suspension. The photoluminescence excitation spectra from several…

Materials Science · Physics 2009-11-11 Flavio Plentz , Henrique B. Ribeiro , Ado Jorio , Marcos A. Pimenta , Michael S. Strano

Optical excitations in hexagonal nanonetwork materials, for example, Boron-Nitride (BN) sheets and nanotubes, are investigated theoretically. The bonding of BN systems is positively polarized at the B site, and is negatively polarized at…

Materials Science · Physics 2016-08-31 Kikuo Harigaya

Recent fluorescence spectroscopy experiments on single wall carbon nanotubes reveal substantial deviations of observed absorption and emission energies from predictions of noninteracting models of the electronic structure. Nonetheless, the…

Materials Science · Physics 2009-11-10 C. L. Kane , E. J. Mele

We show that the energy differences between the lowest optical singlet exciton and the lowest triplet exciton in semiconducting single-walled carbon nanotubes with diameter $\sim 1$ nm and graphene nanoribbons with widths $\sim 2$ nm are an…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 K. Aryanpour , Sumit Mazumdar , Hongbo Zhao

We investigate electric-field induced redshifts of photoluminescence from individual single-walled carbon nanotubes. The shifts scale quadratically with field, while measurements with different excitation powers and energies show that…

Mesoscale and Nanoscale Physics · Physics 2014-10-23 M. Yoshida , Y. Kumamoto , A. Ishii , A. Yokoyama , Y. K. Kato

We demonstrate a possibility for exciton Bose-Einstein condensation in individual small-diameter (~1-2 nm) semiconducting carbon nanotubes. The effect occurs under the exciton-interband-plasmon coupling controlled by an external…

Mesoscale and Nanoscale Physics · Physics 2015-06-15 I. V. Bondarev , A. V. Meliksetyan

Exciton effects are studied in single-wall boron-nitride (BN) nanotubes. Linear absorption spectra are calculated with changing the chiral index of the zigzag nanotubes. We consider the extended Hubbard model with atomic energies at the…

Materials Science · Physics 2009-07-07 Kikuo Harigaya

Single walled carbon nanotubes as emerging quantum-light sources may fill a technological gap in silicon photonics due to their potential use as near infrared, electrically driven, classical or non-classical emitters. Unlike in…

We consider the excitation of electrons in semiconducting carbon nanotubes by photons from the evanescent field created by a subwavelength-diameter optical fiber. The strongly changing evanescent field of such nanofibers requires dropping…

Quantum Physics · Physics 2011-11-23 S. Broadfoot , U. Dorner , D. Jaksch
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