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The stability of graphene nanoribbons in the presence of typical atmospheric molecules is systematically investigated by means of density functional theory. We calculate the edge formation free energy of five different edge configurations…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 M. Vanin , J. Gath , K. S. Thygesen , K. W. Jacobsen

Several dissociated and two non-dissociated adsorption structures of the phenol molecule on the Si(001)-(2 \times 1) surface are studied using density functional theory with various exchange and correlation functionals. The relaxed…

Computational Physics · Physics 2015-05-19 Karen Johnston , Andris Gulans , Tuukka Verho , Martti J. Puska

We present a density functional study of the structural and electronic properties of small Cu_n (n=1,4) aggregates on defect-free MgO(100). The calculations employ a slab geometry with periodic boundary conditions, supercells with up to 76…

Materials Science · Physics 2009-10-30 V. Musolino , A. Selloni , R. Car

We report an experimental and theoretical analysis of the sqrt(3)x sqrt(3)-R30 and 2x2 reconstructions on the NiO (111) surface combining transmission electron microscopy, x-ray photoelectron spectroscopy, and reasonably accurate density…

Materials Science · Physics 2015-05-13 J. Ciston , A. Subramanian , D. M. Kienzle , L. D. Marks

To help understand the high activity of silver as an oxidation catalyst, e.g., for the oxidation of ethylene to epoxide and the dehydrogenation of methanol to formaldehyde, the interaction and stability of oxygen species at the Ag(111)…

Materials Science · Physics 2009-11-10 Wei-Xue Li , Catherine Stampfl , Matthias Scheffler

Using first-principles calculations based on density-functional theory (DFT) we investigated the effects of the van der Waals (vdW) interactions on the structural and electronic properties of anthracene and pentacene adsorbed on the Ag(111)…

Materials Science · Physics 2017-03-16 Juliana M. Morbec , Peter Kratzer

CO adsorption on Cu(111) and Cu(001) surfaces has been studied within ab-initio density functional theory (DFT). The structural, vibrational and thermodynamic properties of the adsorbate-substrate complex have been calculated. Calculations…

Materials Science · Physics 2009-11-10 M. Gajdos , J. Hafner

Epitaxial silicene, which is one single layer of silicon atoms packed in a honeycomb structure, demonstrates a strong interaction with the substrate that dramatically affects its electronic structure. The role of electronic coupling in the…

Mesoscale and Nanoscale Physics · Physics 2014-12-08 Xun Xu , Jincheng Zhuang , Yi Du , Haifeng Feng , Nian Zhang , Chen Liu , Tao Lei , Jiaou Wang , Michelle Spencer , Tetsuya Morishita , Xiaolin Wang , Shi Xue Dou

The vibrational properties of carbon monoxide adsorbed to the copper (100) surface are explored within density functional theory. Atoms of the substrate and adsorbate are treated on an equal footing in order to examine the effect of…

mtrl-th · Physics 2009-10-30 Steven P. Lewis , Andrew M. Rappe

Density-functional theory calculations are used to verify the atomic structure of the $\sqrt{3}$$\times$$\sqrt{3}$ silicene phase grown on the Ag(111) surface. Recent experimental studies strongly suggested that the previous double-layer…

Materials Science · Physics 2016-02-29 Se Gab Kwon , Myung Ho Kang

Extensive density-functional calculations are performed for chemisorption of atoms in the three first periods (H, B, C, N, O, F, Al, Si, P, S, and Cl) on the polar TiC(111) surface. Calculations are also performed for O on TiC(001), for…

Materials Science · Physics 2007-05-23 Carlo Ruberto , Bengt I. Lundqvist

We present an ab initio investigation of the interaction between methane, its dehydrogenated forms and the cerium oxide surface. In particular, the stoichiometric CeO2(111) surface and the one with oxygen vacancies are considered. We study…

Materials Science · Physics 2019-11-21 Marco Fronzi , Simone Piccinin , Bernard Delley , Enrico Traversa , Catherine Stampfl

We present a systematic theoretical investigation of the surface properties, stability and reactivity, of rock-salt type alkaline-earth metal oxides including MgO, CaO, SrO, and BaO. The accuracy of commonly used exchange-correlation…

Materials Science · Physics 2015-06-23 Michal Bajdich , Jens K. Nørskov , Aleksandra Vojvodic

Large scale first-principles calculations based on density functional theory (DFT) employing two different methods (atomic orbitals and plane wave basis sets) were used to study the energetics, geometry, the electronic charge redistribution…

Materials Science · Physics 2010-05-27 Vitaly Alexandrov , Sergei Piskunov , Yuri F. Zhukovskii , Eugene A. Kotomin , Joachim Maier

Using first-principles calculations, we systematically study the adsorption behavior of a single molecular H$_{2}$O on the Be(0001) surface. We find that the favored molecular adsorption site is the top site with an adsorption energy of…

Materials Science · Physics 2015-05-27 Shuang-Xi Wang , Peng Zhang , Jian Zhao , Shu-Shen Li , Ping Zhang

We present and discuss the results of ab initio DFT plane-wave supercell calculations of the atomic and molecular oxygen adsorption and diffusion on the LaMnO3 (001) surface which serves as a model material for a cathode of solid oxide fuel…

Materials Science · Physics 2008-02-04 Eugene A. Kotomin , Yuri A. Mastrikov , Eugene Heifets , Joachim Maier

A combination of Photoemission, Atomic Force and Scanning Tunneling Microscopy/Spectroscopy measurements shows that excess electrons in TiO2 anatase (101) surface are trapped at step edges. Consequently, steps act as preferred adsorption…

The electronic structure and optical absorption spectrum of V^{0} and V^{-} center in MgO are investigated using first-principles calculations based on density functional theory. It is demonstrated that the configuration with distortion is…

Materials Science · Physics 2017-03-16 Jie Zhang , Xian Long Wang , Kai Shuai Yang , Ya Cheng , Chuan Guo Zhang , Zhi Zeng , Xian Ming Zhou , Hai Qing Lin

We study the adsorption geometry of 3,4,9,10-perylene-tetracarboxylic-dianhydride (PTCDA) on Ag(111) and Cu(111) using X-ray standing waves. The element-specific analysis shows that the carbon core of the molecule adsorbs in a planar…

Materials Science · Physics 2011-04-13 A. Gerlach , S. Sellner , F. Schreiber , N. Koch , J. Zegenhagen

We investigate the adsorption of a single tetracyanoethylene (TCNE) molecule on the silver (001) surface. Adsorption structures, electronic properties, and scanning tunneling microscopy (STM) images are calculated within density-functional…

Mesoscale and Nanoscale Physics · Physics 2016-06-22 Thorsten Deilmann , Peter Krüger , Michael Rohlfing , Daniel Wegner
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