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The static and dynamic structure of liquid Al is studied using the orbital free ab-initio molecular dynamics method. Two thermodynamic states along the coexistence line are considered, namely T = 943 K and 1323 K for which X-ray and neutron…

Disordered Systems and Neural Networks · Physics 2009-11-07 David J. Gonzalez , Luis Enrique Gonzalez , Jose Manuel Lopez , Malcolm J. Stott

Ab initio simulations carried out in different atomic cluster configurations in bcc Fe matrix containing Zr and Al suggest energetic favorability of Y-Zr-O phase nucleation, preferably with trigonal Y4Zr3O12 structure. Subsequently, the…

Materials Science · Physics 2022-03-03 Sruthi Mohan , Gurpreet Kaur , C. David , R. Vijay , G. Amarendra

A comparative study between PbTiO$_3$, PbZrO$_3$, and the solid solution PbZr$_{0.5}$Ti$_{0.5}$O$_3$ is performed on the soft mode lattice dynamics within the first Brillouin Zone. We consider the six unique B-site orderings for…

Materials Science · Physics 2019-12-25 Jack S. Baker , David Bowler

The effects of M atomic species mixing on the physical properties of newly synthesized MAX phase (Zr1-xTix)2AlC solid solutions have been studied by means of density functional theory (DFT) calculations. The lattice constants in good accord…

Ab initio calculations and a direct method are applied to derive the phonon dispersion relations and phonon density of states for the ZrC crystal. The results are in good agreement with neutron scattering data. The force constants are…

Materials Science · Physics 2013-01-28 Paweł T. Jochym , Krzysztof Parlinski

Precipitation in Mg-Zn alloys was analyzed by means of first principles calculations. Formation energies of symmetrically distinct hcp Mg1-xZnx (0 < x < 1) configurations were determined and potential candidates for Guinier-Preston zones…

Materials Science · Physics 2020-10-07 S. Liu , G. Esteban-Manzanares , J. LLorca

The electronic structures of hexagonal beta-Al9Mn3Si and phi-Al10Mn3 are investigated through self-consistent calculations carried out using the LMTO method. This ab-initio approach is combined with an analysis of a simplified hamiltonian…

Materials Science · Physics 2013-10-02 G. Trambly de Laissardiere

The ground state structures of the A$_x$B$_{1-x}$C wurtzite (WZ) alloys with $x=$0.25, 0.5, and 0.75 are revealed by a ground state search using the valence-force field model and density-functional theory total energy calculations. It is…

Materials Science · Physics 2009-09-30 H. J. Xiang , Su-Huai Wei , Shiyou Chen , X. G. Gong

We have investigated the phonon, elastic and thermodynamic properties of L1$_{2}$ phase Al$_{3}$Ta by density functional theory approach combining with quasi-harmonic approximation model. The results of phonon band structure shows that…

Materials Science · Physics 2018-04-02 W. Leini , T. Zhang , Z. Wu , N. Wei

A first-principles-derived scheme, that incorporates ferroelectric and antiferrodistortive degrees of freedom, is developed to study finite-temperature properties of PbZr1-xTixO3 solid solutions near its morphotropic phase boundary. The use…

Materials Science · Physics 2009-11-11 Igor A. Kornev , L. Bellaiche , P. -E. Janolin , B. Dkhil , E. Suard

Phonon spectrum of cubic barium zirconate is calculated from first principles using the density functional theory. Unstable phonon mode with the $R_{25}$ symmetry in the phonon spectrum indicates an instability of the cubic structure with…

Materials Science · Physics 2015-08-18 A. I. Lebedev , I. A. Sluchinskaya

Using full-potential linear augmented plane wave method (FP-LAPW) and the density functional theory, we have carried out a systematic investigation of the electronic, magnetic, and cohesive properties of the chalcogenide CrTe in three…

Materials Science · Physics 2015-03-17 Y. Liu , S. K. Bose , J. Kudrnovský

Ba(Zr,Ti)O$_3$ is a lead-free relaxor ferroelectric. Using the first-principles method, the ferroelectric dipole moments for pure BaTiO$_3$ and Ba(Zr,Ti)O$_3$ supercells have been studied. All possible ion configurations of…

Materials Science · Physics 2015-11-11 Li-Juan Yang , Lingzhi Wu , Shuai Dong

To understand the mechanisms by which Fe and Cr additions increase the corrosion rate of irradiated Zr alloys, a combination of experimental (atom probe tomography, x-ray diffraction and thermoelectric power measurements) and modelling…

Materials Science · Physics 2015-11-09 P. A. Burr , M. R. Wenman , B. Gault , M. P. Moody , M. Ivermark , M. J. D. Rushton , M. Preuss , L. Edwards , R. W. Grimes

We study the phase behaviour of the Al$_x$CrFeCoNi high-entropy alloy. Our approach is based on a perturbative analysis of the internal energy of the paramagnetic solid solution as evaluated within the Korringa-Kohn-Rostoker formulation of…

Materials Science · Physics 2024-12-02 Christopher D. Woodgate , George A. Marchant , Livia B. Pártay , Julie B. Staunton

Using the hybrid exchange-correlation functional within the density-functional theory, we have systematically investigated the structural and electronic properties of MO (M = Be, Mg, Ca, Sr, Ba, Zn, Cd) in binary rocksalt (B1), zincblende…

Materials Science · Physics 2019-03-19 Jinying Yu , Mingke Zhang , Zihan Zhang , Shangwei Wang , Yelong Wu

In this work, the elastic and thermodynamic properties of Pt$_{3}$Al under high pressure are investigated using density functional theory within the generalized gradient approximation. The results of bulk modulus and elastic constants at…

Materials Science · Physics 2015-12-25 N. Wei , Ch. Zhang , S. Hou

We describe implementation and analysis of a first-principles theory, derived in an earlier work, for the leading terms in an expansion of a Gibbs free energy of a multi-component alloy in terms of order parameters that characterize…

Materials Science · Physics 2025-02-24 Christopher D. Woodgate , Julie B. Staunton

Impurity diffusion in Zr is potentially important for many applications of Zr alloys, and in particular for their use of nuclear reactor cladding. However, significant uncertainty presently exists about which elements are vacancy vs.…

Materials Science · Physics 2018-05-14 Hai-Jin Lu , Henry Wu , Nan Zou , Xiao-Gang Lu , Yan-Lin He , Dane Morgan

The density of state approach has recently been proposed as a potential route to circumvent the sign problem in systems at finite density. In this study, using the Linear Logarithmic Relaxation (LLR) algorithm, we extract the generalised…

High Energy Physics - Lattice · Physics 2020-01-22 Olmo Francesconi , Markus Holzmann , Biagio Lucini , Antonio Rago