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Magnetic materials with the spinel structure (A$^{2+}$B$^{3+}_2$O$^4$) form the core of numerous magnetic devices, but ZnFe$_2$O$_4$ constitutes a peculiar example where the nature of the magnetism is still unresolved. Susceptibility…

Alkali superoxides differ from conventional transition metal magnets, exhibit magnetism from partially occupied oxygen molecular $\pi^*$-orbitals. Among them, CsO$_2$ stands out for its potential to exhibit novel quantum collective…

Strongly Correlated Electrons · Physics 2024-11-12 Ryota Ono , Ravi Kaushik , Sergey Artyukhin , Martin Jansen , Igor Solovyev , Russell A. Ewings

TmVO$_{4}$ exhibits ferroquadrupolar order of the Tm 4f electronic orbitals at low temperatures, and is a model system for Ising nematicity that can be tuned continuously to a quantum phase transition via magnetic fields along the $c$-axis.…

Strongly Correlated Electrons · Physics 2022-07-04 I. Vinograd , K. R. Shirer , P. Massat , Z. Wang , T. Kissikov , D. Garcia , M. D. Bachmann , M. Horvatić , I. R. Fisher , N. J. Curro

The structural and magnetic properties of the hexagonal four-layer form of SrMnO$_3$ have been investigated by combining magnetization measurements, electron diffraction and high-resolution synchrotron X-ray and neutron powder diffraction.…

Strongly Correlated Electrons · Physics 2007-05-23 A. Daoud-Aladine , C. Martin , L. C. Chapon , M. Hervieu , K. S. Knight , M. Brunelli , P. G. Radaelli

Correlated materials with competing spin-orbit and crystal-field interactions can host composite spin-orbital magnons that are highly susceptible to structural and electronic perturbations, enabling the control of magnetic dynamics beyond…

We consider the superstructures, which can be formed in spinels containing on B-sites the transition-metal ions with partially filled t2g levels. We show that, when such systems are close to itinerant state (e.g. have an insulator-metal…

Strongly Correlated Electrons · Physics 2009-11-10 D. I. Khomskii , T. Mizokawa

An extensive {\it ab initio} study of the physical properties of both linear and zigzag atomic chains of all 4$d$ and 5$d$ transition metals (TM) within the GGA by using the accurate PAW method, has been carried out. All the TM linear…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 J. C. Tung , G. Y. Guo

The crystal structure of the double tungstate NaFe(WO$_4$)$_2$ arises from that of the spin-driven multiferroic MnWO$_4$ by inserting non-magnetic Na layers. NaFe(WO$_4$)$_2$ exhibits a three-dimensional incommensurate spin-spiral structure…

Strongly Correlated Electrons · Physics 2022-05-17 S. Holbein , M. Ackermann , L. Chapon , P. Steffens , A. Gukasov , A. Sazonov , O. Breunig , Y. Sanders , P. Becker , L. Bohaty , T. Lorenz , M. Braden

We study the magnetic order and excitations in strong spin-orbit coupled, Van Vleck-type, $d^4$ Mott insulators on a square lattice. Extending the previous work, we include the tetragonal crystal field splitting and explore its effects on…

Strongly Correlated Electrons · Physics 2014-07-29 Alireza Akbari , Giniyat Khaliullin

Neutron scattering studies and measurements of the dielectric susceptibility and ferroelectric polarization P have been carried out in various magnetic fields H for single-crystal samples of the multiferroic system LiVCuO4 with quasi…

Strongly Correlated Electrons · Physics 2015-05-13 Yukio Yasui , Yutaka Naito , Kenji Sato , Taketo Moyoshi , Masatoshi Sato* , Kazuhisa Kakurai

Cubic to tetragonal distortion in spinel compounds have been a contentious issue for last two decades. Different groups have proposed different mechanisms to understand such a distortion in these spinels, which are: (i) spin lattice…

Strongly Correlated Electrons · Physics 2017-04-24 Sohan Lal , Sudhir K. Pandey

Dielectric and magnetic phenomena in spin and charge frustrated system RFe2O4 (R is a rare-earth metal ion) are studied. An electronic model for charge, spin and orbital degrees in a pair of triangular-lattice planes is derived. We analyze…

Strongly Correlated Electrons · Physics 2009-11-13 Makoto Naka , Aya Nagano , Sumio Ishihara

The mechanisms of magnetic and orbital interactions due to double exchange (DE) and superexchange (SE) in transition metal oxides with degenerate e_g orbitals are presented. Specifically, we study the effective spin-orbital models derived…

Strongly Correlated Electrons · Physics 2009-10-31 A. M. Oles , M. Cuoco , N. B. Perkins

Recent DFT calculations for Ba2CoO4 (BCO) and neutron scattering experiments for SrRuO3 (SRO) have shown that oxygen develops a magnetic polarization. Moreover, DFT calculations for these compounds also unveiled unexpected nodes in the spin…

Strongly Correlated Electrons · Physics 2021-05-20 Ling-Fang Lin , Nitin Kaushal , Cengiz Şen , Andrew D. Christianson , Adriana Moreo , Elbio Dagotto

The 3d electronic structure and phase transition in pure and Cr doped V2O3 are theoretically investigated in relation to the 3d spin-orbit interaction and lattice distortion. A model consisting of the nearest-neighbor V ion pair with full…

Strongly Correlated Electrons · Physics 2016-08-31 Arata Tanaka

This review discusses the multifaceted electronic properties of spinel oxides with a particular focus on Lithium Vanadate (LiV2O4), Lithium Titanate (LiTi2O4), and Magnesium Titanate (MgTi2O4). We selected LiTi2O4, LiV2O4, and MgTi2O4…

Materials Science · Physics 2025-12-03 Jagadis Prasad Nayak , Raju Saini , Sourav Dash , Gopi Nath Daptary

A toroidal dipole moment appears independent of the electric and magnetic dipole moment in the multipole expansion of electrodynamics. It arises naturally from vortex-like arrangements of spins. Observing and controlling spontaneous…

We studied temperature and magnetic field dependence of magnetization, $M(T)$ and $M(B)$, on thiospinel FeCr$_{2}$S$_{4}$. We observed a step-like anomaly at $T_{OO} \sim$ 9 K for $M$($T$) attributed to an orbital order transition in…

Strongly Correlated Electrons · Physics 2015-05-28 Masakazu Ito , Yuji Nagi , Naotoshi Kado , Shinpei Urakawa , Takuro Ogawa , Akihiro Kondo , Keiichi Koyama , Kazuo Watanabe , Koichi Kindo

We elucidate the pivotal role of the bandstructure's orbital content in deciding the type of commensurate magnetic order stabilized within the itinerant scenario of iron-pnictides. Recent experimental findings in the tetragonal magnetic…

Superconductivity · Physics 2017-08-01 Morten H. Christensen , Daniel D. Scherer , Panagiotis Kotetes , Brian M. Andersen

We present the results of broadband dielectric spectroscopy of GaMo$_4$S$_8$, a lacunar spinel system that recently was shown to exhibit non-canonical, orbitally-driven ferroelectricity. Our study reveals complex relaxation dynamics of this…

Strongly Correlated Electrons · Physics 2018-12-26 K. Geirhos , S. Krohns , H. Nakamura , T. Waki , Y. Tabata , I. Kézsmárki , P. Lunkenheimer