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We report the Pockels electro-optic properties of ZrO2 and HfO2 orthorhombic Pbc21 and rhombohedral R3m ferroelectric phases, and we compare them to the well-known LiNbO3 Pockels material from density functional theory calculations using…

In recent experiments the irradiation of insulators of perovskite type with swift heavy ions under glancing incidence has been shown to provide a unique means to generate periodically arranged nanodots at the surface. The physical origin of…

Materials Science · Physics 2008-01-23 O. Osmani , A. Duvenbeck , E. Akcoeltekin , R. Meyer , H. Lebius , M. Schleberger

We report direct first-principles density-functional calculations of the piezoelectric tensor $\tensor{d}$ relating polarization to applied stress for the binary compounds AlN, GaN, and InN. The values of $\tensor{d}$ are rather sensitive…

Materials Science · Physics 2009-11-07 F. Bernardini , V. Fiorentini

A first-principles study of the vibrational modes of PbTiO_3 in the ferroelectric tetragonal phase has been performed at all the main symmetry points of the Brillouin zone (BZ). The calculations use the local-density approximation and…

mtrl-th · Physics 2009-10-30 Alberto Garcia , David Vanderbilt

In this study, an efficient first-principles approach for calculating the thermodynamic properties of mixed metal oxides at high temperatures is demonstrated. More precisely, this procedure combines density functional theory and harmonic…

Materials Science · Physics 2023-05-12 Joakim Brorsson , Ivana Staničić , Jonatan Gastaldi , Tobias Mattison , Anders Hellman

In search of a reliable methodology for the prediction of light absorption and emission of Ce$^{3+}$-doped luminescent materials, 13 representative materials are studied with first-principles and semiempirical approaches. In the…

Materials Science · Physics 2017-08-22 Yongchao Jia , Samuel Poncé , Anna Miglio , Masayoshi Mikami , Xavier Gonze

Potassium niobate (KNbO3) is a prototypical perovskite ferroelectric with large electro-optic and nonlinear optical responses, high optical damage thresholds and a rich sequence of temperature-driven phase transformations, making it a…

Materials Science · Physics 2026-01-27 Aiden Ross , Venkatraman Gopalan , Long-Qing Chen

Monte Carlo simulations with an effective Hamiltonian parametrized from first principles are performed to study the dielectric response of BaTiO3 as a function of temperature, with particular emphasis on the behavior of the dielectric…

Materials Science · Physics 2009-10-31 Alberto Garcia , David Vanderbilt

The electronic and structural properties of Li$B$O$_3$ ($B$=V, Nb, Ta, Os) are investigated via first-principles methods. We show that Li$B$O$_3$ belong to the recently proposed hyperferroelectrics, i.e., they all have unstable longitudinal…

Materials Science · Physics 2016-10-20 Pengfei Li , Xinguo Ren , Guang-Can Guo , Lixin He

The discovery of high temperature superconductivity in FeSe films on SrTiO3 substrate has inspired great experimental and theoretical interests. First-principles density functional theory calculations, which have played an important role in…

Superconductivity · Physics 2015-10-30 Kai Liu , Miao Gao , Zhong-Yi Lu , Tao Xiang

Using first-principles calculations, we analyze the structural properties of tungsten trioxide WO3 . Our calculations rely on density functional theory and the use of the B1-WC hybrid functional, which provides very good agreement with…

Materials Science · Physics 2016-12-28 Hanen Hamdi , Ekhard K. H. Salje , Philippe Ghosez , Eric Bousquet

Theoretical descriptions of the Seebeck coefficient in terms of the differential electrical conductivity given by Cutler and Mott is the foundation of later works in terms of transmission function from the thermoelectric transport theory.…

With the motive of unraveling the origin of native vacancy induced magnetization in ferroelectric perovskite oxide systems, here we explore the consequences of electronic structure modification in magnetic ordering of oxygen deficient…

The nonlinear optical properties and electro-optic effects of some oxygen-octahedric ferroelectrics are studied by the density functional theory (DFT) in the local density approximation (LDA) expressions based on first principle…

Materials Science · Physics 2011-12-30 Amirullah M. Mamedov , Ekmel Ozbay

The structural, elastic, magnetic properties, as well as electronic structure and chemical bonding picture of new oxide 3d1-perovskite BaVO3, recently synthesized, were systematically investigated involving the first-principles FLAPW-GGA…

Materials Science · Physics 2019-04-18 V. V. Bannikov

We present a first-principles method for the calculation of optical excitations in nanosystems. The method is based on solving the Bethe-Salpeter equation (BSE) for neutral excitations. The electron self-energy is evaluated within the GW…

Materials Science · Physics 2009-11-11 Murilo L. Tiago , James R. Chelikowsky

The connection between noncentrosymmetric materials' structure, electronic structure, and bulk photovoltaic performance remains not well understood. In particular, it is still unclear which photovoltaic (PV) mechanism(s) are relevant for…

Materials Science · Physics 2015-05-20 Fenggong Wang , Andrew M. Rappe

First-principles calculations combining density functional theory and many-body perturbation theory can provide microscopic insight into the dynamics of electrons and phonons in materials. We review this theoretical and computational…

Materials Science · Physics 2016-11-23 Marco Bernardi

We report our first-principles investigations on three polytypes of BaTiO3 (BTO): a paraelectric phase with cubic Pm-3m structure and two ferroelectric (FE) phases with tetragonal P4mm and rhombohedral R3m structures. We compared the…

Materials Science · Physics 2013-07-02 Yu-Seong Seo , Jai Seok Ahn

We use first-principles density-functional total energy and polarization calculations to calculate the piezoelectric tensor at zero temperature for both cubic and simple tetragonal ordered supercells of Pb_3GeTe_4. The largest piezoelectric…

Materials Science · Physics 2009-10-30 Eric Cockayne , Karin M. Rabe
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