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We present a quaternion inspired formalism specifically developed to evaluate the intensity of the electrical current that traverses a single molecule connected to two semi-infinite electrodes as the applied external bias is varied. The…

Mesoscale and Nanoscale Physics · Physics 2012-01-18 Augusto C. L. Moreira , Celso P. de Melo

The conditions necessary for a nanotube junction connecting a metallic and semiconducting nanotube to rectify the current are theoretically investigated. A tight binding model is used for the analysis, which includes the Hartree-Fock…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Ryo Tamura

The problem of two magnetic impurities in a normal metal exposes the two opposite tendencies in the formation of a singlet ground state, driven respectively by the single-ion Kondo effect with conduction electrons to screen impurity spins…

Strongly Correlated Electrons · Physics 2015-04-24 Rong-Qiang He , Jianhui Dai , Zhong-Yi Lu

We examine the robustness of single-molecule tunneling diodes to thermal-environmental effects. The diode comprises three fragments: two different conjugated chemical groups at the boundaries, and a saturated moiety in between, breaking…

Mesoscale and Nanoscale Physics · Physics 2015-12-29 Michael Kilgour , Dvira Segal

We use the scattering states numerical renormalization group (SNRG) approach to calculate the current $I(V)$ through a single molecular level coupled to a local molecular phonon. The suppression of $I$ for asymmetric junctions with…

Mesoscale and Nanoscale Physics · Physics 2015-10-09 Andre Jovchev , Frithjof B. Anders

We compute the spin current rectification coefficient of a non-equilibrium quantum dot subject to a spin bias and an {\it ac} charge bias with small amplitude. As a function of the position of the resonant level the spin current…

Mesoscale and Nanoscale Physics · Physics 2012-08-21 T. I. Ivanov

Devices for nano- and molecular size electronics are currently a focus of research aimed at an efficient current rectification and switching. Current switching due to conformational changes in the molecules is slow, on the order of a few…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 A. S. Alexandrov , A. M. Bratkovsky

Electron transport through a diatomic molecular tunnel junction shows wave like interference phenomenon. By using Keldysh non-equilibrium Green's function (NEGF) theory, we have explicitly presented current and differential conductance…

Mesoscale and Nanoscale Physics · Physics 2012-12-18 Muhammad Imran

We study the rectification of spin current in $XXZ$ chains segmented in two parts, each with a different anisotropy parameter. Using exact diagonalization and a matrix product states algorithm we find that a large rectification (of the…

Statistical Mechanics · Physics 2018-05-23 Vinitha Balachandran , Giuliano Benenti , Emmanuel Pereira , Giulio Casati , Dario Poletti

The sinh-Gordon model on a half-line with integrable boundary conditions is considered in low order perturbation theory developed in affine Toda field theory. The quantum corrections to the classical reflection factor of the model are…

High Energy Physics - Theory · Physics 2009-11-07 A. Chenaghlou

Relativistic exchange current corrections to the impulse approximation in low and intermediate energy neutrino--nucleus scattering are presented assuming non--vanishing strange quark form factors for constituent nucleons. Two--body exchange…

Nuclear Theory · Physics 2008-11-26 Y. Umino , J. M. Udias

We develop a consistent method for calculating non-equilibrium Green's functions for a nano-sized dot coupled to electron reservoirs by tunneling. The leads are generally at different chemical potentials (non-equilibrium), and the dot may…

Strongly Correlated Electrons · Physics 2007-05-23 Jung Hoon Han

Density functional theory calculations of electronic transport based on local exchange and correlation functionals contain self-interaction errors. These originate from the interaction of an electron with the potential generated by itself…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 C. Toher , S. Sanvito

The electronic spectrum of a chemically contacted molecule in the junction of a scanning tunneling microscope can be modified by tip retraction. We analyze this effect by a combination of density functional, many-body perturbation and…

Materials Science · Physics 2015-05-19 A. Greuling , M. Rohlfing , R. Temirov , F. S. Tautz , F. B. Anders

It is illustrated that semiconductor quantum dots (QDs) embedded into an insulating matrix connected with metallic electrodes and some vacuum space can lead to significant thermal rectification effect. A multilevel Anderson model is used to…

Mesoscale and Nanoscale Physics · Physics 2010-01-11 David M. -T. Kuo , Yia-chung Chang

We study computationally the electron transport properties of dithiocarboxylate terminated molecular junctions. Transport properties are computed self-consistently within density functional theory and nonequilibrium Green's functions…

Materials Science · Physics 2007-05-23 Zhenyu Li , D. S. Kosov

We provide an integration of the universal, perturbative explicitly correlated [2]$_\text{R12}$-correction in the context of the Variational Quantum Eigensolver (VQE). This approach is able to increase the accuracy of the underlying…

Quantum Physics · Physics 2022-07-08 Philipp Schleich , Jakob S. Kottmann , Alán Aspuru-Guzik

We investigated a mechanism of rectification in di-block oligomer diode molecules that have recently been synthesized and showed a pronounced asymmetry in the measured I-V spectrum. The observed rectification effect is due to the resonant…

Other Condensed Matter · Physics 2009-11-11 I. I. Oleynik , M. A. Kozhushner , V. S. Posvyanskii , L. Yu

The transport properties of serially coupled quantum dots (SCQDs) embedded in a matrix connected to metallic electrodes are theoretically studied in the linear and nonlinear regimes. The current rectification and negative differential…

Mesoscale and Nanoscale Physics · Physics 2015-06-12 Yen-Chun Tseng , David M. -T. Kuo

Within the diagrammatic real time approach \cite{K\"onig96, Schoeller97}, the current across a quantum dot which is tunnel coupled to two leads at different chemical potentials is calculated by the use of two objects referred to as kernels.…

Strongly Correlated Electrons · Physics 2014-11-18 Johannes Kern