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Using Monte Carlo simulation methods, we explore the role of molecular shape in the phase behavior of liquid crystals and the electroclinic effect. We study a "bent-rod" mesogen shaped like the letter Z, composed of seven soft spheres…

Soft Condensed Matter · Physics 2009-10-31 J. Xu , R. L. B. Selinger , J. V. Selinger , B. R. Ratna , R. Shashidhar

We have used Monte Carlo NPT computer simulations to study a system of spherical fan shaped particles made of three hard discs fused along a common diameter. The calculated equation of state indicates a strong, entropy driven, first order…

Soft Condensed Matter · Physics 2016-08-31 A. G. Vanakaras , D. J. Photinos

Recently, a new class of smectic liquid crystal phases (SmCP phases) characterized by the spontaneous formation of macroscopic chiral domains from achiral bent-core molecules has been discovered. We have carried out Monte Carlo simulations…

Statistical Mechanics · Physics 2009-11-07 Yves Lansac , Prabal K. Maiti , Noel A. Clark , Matthew A. Glaser

We report a molecular dynamics simulation demonstrating that the Smectic B crystalline phase (Cr-B), commonly observed in mesogenic systems of anisotropic molecules, can be formed by a system of identical particles interacting via a…

Soft Condensed Matter · Physics 2013-12-16 A. Metere , T. Oppelstrup , S. Sarman , A. Laaksonen , M. Dzugutov

We present the phase diagram of a system of mesogenic top-shaped molecules based on the Parsons- Lee density functional theory and Monte Carlo simulation. The molecules are modeled as a hard spherocylinder with a hard sphere embedded in its…

Soft Condensed Matter · Physics 2011-06-13 D. de las Heras , S. Varga , F. J. Vesely

The smectic C (smC) phase represents a unique class of liquid crystal phases characterised by the layered arrangement of molecules with tilted orientations with respect to layer normals. Building upon the real-valued tensorial smectic A…

Soft Condensed Matter · Physics 2024-08-09 Jingmin Xia , Yucen Han

We carry out Monte Carlo simulations to investigate the effect of molecular shape on liquid-crystal order. In our approach, each model mesogen consists of several soft spheres bonded rigidly together. The arrangement of the spheres may be…

Soft Condensed Matter · Physics 2009-11-07 J. Xu , R. L. B. Selinger , J. V. Selinger , R. Shashidhar

Using the classical density functional theory of freezing and Monte Carlo computer simulations, we explore the liquid-crystalline phase behavior of hard rectangles on flat and cylindrical manifolds. Moreover, we study the effect of a static…

Soft Condensed Matter · Physics 2018-02-19 Christoph E. Sitta , Frank Smallenburg , Raphael Wittkowski , Hartmut Löwen

We numerically investigate two-dimensional systems of hard rectangles at constant pressure through extensive hard-particle Monte Carlo simulations. We determine the complete phase diagram as a function of packing fraction and aspect ratio,…

Soft Condensed Matter · Physics 2025-05-15 Denis Dertli , Thomas Speck

We report Monte-Carlo simulation studies of some systems consisting of polar rod-like molecules interacting via a pair potential that exhibit liquid crystal phases, attributed with tilt angles of large magnitude. For theoretical…

Soft Condensed Matter · Physics 2012-04-11 Tushar Kanti Bose , Jayashree Saha

We have numerically studied a liquid composed of achiral, bent-shaped molecules built of tangent spheres. The system is known to spontaneously break mirror symmetry, as it forms a macroscopically chiral, twist-bend nematic phase [Phys. Rev.…

Soft Condensed Matter · Physics 2022-09-27 Piotr Kubala , Wojciech Tomczyk , Michał Cieśla

Hard spherocylinders (cylinders of length $L$ and diameter $D$ capped at both ends with two hemispheres) provide a suitable model for investigating entropy-driven, mesophase formations in real colloidal fluids that are composed of rigid…

Statistical Mechanics · Physics 2011-10-26 D. Costa , F. Micali , F. Saija , P. V. Giaquinta

We studied equilibrium systems composed of wedge-shaped monodisperse molecules using hard-particle Monte Carlo simulations. Each model molecule was made up of six colinear tangent spheres with linearly decreasing diameters. Thus, the shape…

Soft Condensed Matter · Physics 2023-06-26 Piotr Kubala , Michał Cieśla , Lech Longa

Computer simulation study of phase transitional behaviour of cholesterol molecules embedded with terminal dipole is reported. In this work, coarse-grained modeling of cholesteric molecules is done to study the influence of the coupled…

Soft Condensed Matter · Physics 2018-10-01 Tanay Paul Jayashree Saha

Pressure-induced phase transitions of spin-crossover materials were simulated by a Monte Carlo simulation in the constant pressure ensemble for the first time. Here, as the origin of the cooperative interaction, we adopt elastic interaction…

Materials Science · Physics 2008-04-09 Yusuke Konishi , Hiroko Tokoro , Masamichi Nishino , Seiji Miyashita

We present a self-consistent field theory (SCFT) of semiflexible (wormlike) diblock copolymers, each consisting of a rigid and a flexible part. The segments of the polymers are otherwise identical, in particular with regard to their…

Soft Condensed Matter · Physics 2009-11-07 Dominik Düchs , D. E. Sullivan

Solid-solid collapse transition in open framework structures is ubiquitous in nature. The real difficulty in understanding detailed microscopic aspects of such transitions in molecular systems arises from the interplay between different…

Soft Condensed Matter · Physics 2015-06-15 Rakesh S. Singh , Biman Bagchi

In recent work we revisited the phase diagram of hard ellipsoids of revolution (spheroids) by means of replica exchange Monte Carlo simulations. This was done by setting random initial configurations, and allows to confirm the formation of…

Statistical Mechanics · Physics 2015-06-12 Gustavo Bautista-Carbajal , Arturo Moncho-Jordá , Gerardo Odriozola

We investigated the nematic to smectic transition undergone by parallel hard spherocylinders in the framework provided by the residual multi-particle entropy (RMPE) formalism. The RMPE is defined as the sum of all contributions to the…

Soft Condensed Matter · Physics 2011-10-26 D. Costa , F. Saija , P. V. Giaquinta

We propose a continuum tensorial model for chiral smectic C (SmC$^*$) liquid crystals using a tensor-valued order parameter $\mathbf{Q}$ to describe orientational order and a real-valued order parameter $\delta\rho$ to capture layer…

Soft Condensed Matter · Physics 2025-09-09 Jingmin Xia , Jinbing Wu , Yucen Han
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