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I consider the effects of polymers on the smectic phase of a host liquid crystal matrix. Focusing on the regime in which the polymers are predominately confined between the smectic layers, I find that the presence of the polymers can lead…

Soft Condensed Matter · Physics 2009-10-28 Leo Radzihovsky

In this work, we introduce a simple modification of the Monte Carlo algorithm, which we call step Monte Carlo (sMC). The sMC approach allows to simulate processes far from equilibrium and obtain information about the dynamic properties of…

Other Condensed Matter · Physics 2023-12-15 Dariusz Sztenkiel

Certain models with purely repulsive pair interactions can form cluster crystals with multiply-occupied lattice sites. Simulating these models' equilibrium properties is, however, quite challenging. Here, we develop an expanded…

Soft Condensed Matter · Physics 2015-03-20 Kai Zhang , Patrick Charbonneau

Weakly attractive interactions between the tips of rod-like colloidal particles affect their liquid-crystal phase behaviour due to a subtle interplay between enthalpy and entropy. Here, we employ molecular dynamics simulations on…

Soft Condensed Matter · Physics 2019-10-16 Mariana Oshima Menegon , Guido L. A. Kusters , Paul van der Schoot

The effects of dipolar interactions and molecular flexibility on the structure and phase behavior of bent-core molecular fluids are studied using Monte Carlo computer simulations. Some calculations of flexoelectric coefficients are also…

Soft Condensed Matter · Physics 2007-05-23 Alastair Dewar , Philip J. Camp

Under an electric field, chiral smectic liquid crystals transit usually to the unwound SmC* phase where the helical structure is completely unrolled. Sometimes the sample transits initially towards an intermediate polar state before the…

Soft Condensed Matter · Physics 2019-10-02 H. Dhaouadi , O. Riahi , R. Zgueb , F. Trabelsi , T. Othman

We explore the phase behavior and structure of orthogonal smectic liquid crystals consisting of bent-core molecules (BCMs) by means of Monte Carlo molecular simulations. A simple athermal molecular model is introduced that describes the…

Soft Condensed Matter · Physics 2016-07-26 Stavros D. Peroukidis , Alexandros G. Vanakaras , Demetri J. Photinos

Using particle-resolved molecular-dynamics simulations, we compute the phase diagram for soft repulsive spherocylinders confined on the surface of a sphere. While crystal (K), smectic (Sm), and isotropic (I) phases exhibit a stability…

Soft Condensed Matter · Physics 2025-11-03 Jaydeep Mandal , Hartmut Löwen , Prabal K. Maiti

By employing Molecular Dynamics computer simulations, the phase behavior of systems of rodlike particles with varying degree of internal flexibility has been traced from the perfectly rigid rod limit till very flexible particles, and from…

Soft Condensed Matter · Physics 2009-11-13 Giorgio Cinacchi , Luca De Gaetani

Recent liquid-crystalline (LC) research is focused on structurally new molecular systems distinct from simple nematic or smectic phases. Sophisticated molecular shape may reveal structural complexity, combining helicity and polarity.…

We perform extensive Monte Carlo simulations of a two-dimensional bent hard-needle model in both its chiral zig-zag and its achiral bow-shape configurations and present their phase diagrams. We find evidence for a variety of stable phases:…

Statistical Mechanics · Physics 2016-04-15 Raffaele Tavarone , Patrick Charbonneau , Holger Stark

The crystallization of a metastable melt is one of the most important non equilibrium phenomena in condensed matter physics, and hard sphere colloidal model systems have been used for several decades to investigate this process by…

Soft Condensed Matter · Physics 2015-05-20 Tanja Schilling , Sven Dorosz , Hans Joachim Schoepe , George Opletal

Ionic liquid crystals (ILCs) are anisotropic mesogenic molecules which carry charges and therefore combine properties of liquid crystals, e.g., the formation of mesophases, and of ionic liquids, such as low melting temperatures and tiny…

Soft Condensed Matter · Physics 2017-10-31 Hendrik Bartsch , Markus Bier , Siegfried Dietrich

The rich mesophase polymorhism and the phase sequence of board-like colloids depends critically on their shape anisometry. Implementing extensive Monte Carlo simulations, we calculated the full phase diagram of sterically interacting…

Soft Condensed Matter · Physics 2013-09-10 Stavros D. Peroukidis , Alexandros G. Vanakaras

Using Monte Carlo simulations, we investigate the structural characteristics of an interacting hard sphere system with shifted charge to elucidate the effect of the non-centrosymmetric interaction on its phase behavior. Two different phase…

Chemical Physics · Physics 2014-04-28 Luis E. Sánchez-Díaz , Chwen-Yang Shew , Xin Li , Bin Wu , Gregory S. Smith , Wei-Ren Chen

The order parameters for the phenomenological description of the smectic-{\it A} to smectic-{\it C} phase transition are formulated on the basis of molecular symmetry and structure. It is shown that, unless the long molecular axis is an…

Soft Condensed Matter · Physics 2016-08-31 P. K. Karahaliou , A. G. Vanakaras , D. J. Photinos

We report a molecular dynamics simulation demonstrating that a columnar liquid crystal, commonly formed by disc-shaped molecules, can be formed by identical particles interacting via a spherically symmetric potential. Upon isochoric cooling…

Soft Condensed Matter · Physics 2015-03-20 Alfredo Metere , Tomas Oppelstrup , Sten Sarman , Mikhail Dzugutov

We study smectic-liquid-crystal order in a cell with a heterogeneous substrate imposing surface random positional and orientational pinnings. Proposing a minimal random elastic model, we demonstrate that, for a thick cell, the smectic state…

Soft Condensed Matter · Physics 2015-03-20 Quan Zhang , Leo Radzihovsky

The dynamics of active smectic liquid crystals confined on a spherical surface is explored through an active phase field crystal model. Starting from an initially randomly perturbed isotropic phase, several types of topological defects are…

Soft Condensed Matter · Physics 2025-03-11 Michael Nestler , Simon Praetorius , Zhi-Feng Huang , Hartmut Löwen , Axel Voigt

We study the effect of fluctuations in opening angle of bent-core molecules on stability of the nematic phases. The molecules are built out of two Gay-Berne centers of $\kappa = 4$, $\kappa ' = 5$, $\mu = 1$ and $\nu = 2$, each…

Soft Condensed Matter · Physics 2009-04-07 W. Jozefowicz , L. Longa