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Motivated by recent angle-resolved photoemission spectroscopy (ARPES) observations of a highly metallic two-dimensional electron gas (2DEG) at the (001) vacuum-cleaved surface of SrTiO3 and the subsequent discussion on the possible role of…

Materials Science · Physics 2013-02-25 Juan Shen , Hunpyo Lee , Roser Valenti , Harald O. Jeschke

The energy to desorb atomic oxygen from an interstellar dust grain surface, $E_{\rm des}$, is an important controlling parameter in gas-grain models; its value impacts the temperature range over which oxygen resides on a dust grain.…

Astrophysics of Galaxies · Physics 2015-06-23 Jiao He , Jianming Shi , Tyler Hopkins , Gianfranco Vidali , Michael J. Kaufman

Oxygen vacancies at the SnO2(110) and (101) surface and subsurface sites have been studied in the framework of density functional theory by using both all-electron Gaussian and pseudopotential plane-wave methods. The all-electron…

Materials Science · Physics 2008-06-06 F. Trani , M. Causa' , D. Ninno , G. Cantele , V. Barone

First-principles calculations using density functional theory based on norm-conserving pseudopotentials have been performed to investigate the Cs adsorption on the Si(001) surface for 0.5 and 1 ML coverages. We found that the saturation…

Strongly Correlated Electrons · Physics 2007-05-23 R. Shaltaf , E. Mete , S. Ellialtioglu

The effect of oxygen adsorption on the local structure and electronic properties of monolayer graphene grown on SiC(0001) has been studied by means of Low Energy Electron Microscopy (LEEM), microprobe Low Energy Electron Diffraction…

Materials Science · Physics 2015-06-05 C. Mathieu , B. Lalmi , T. O. Mentes , E. Pallecchi , A. Locatelli , S. Latil , R. Belkhou , A. Ouerghi

While the small sticking coefficient for molecular hydrogen on the Si(001) surface apparently requires a large energy barrier of adsorption, no such barrier is observed in desorption experiments. We have calculated the potential-energy…

mtrl-th · Physics 2009-10-28 E. Pehlke , M. Scheffler

Using density functional theory and an exchange-correlationfunctional that includes the van der Waals interaction, we study the coadsorption of CO on Ru(0001) saturated with 0.5 ML of oxygen. Different coexisting CO coverages are considered…

Materials Science · Physics 2021-06-09 Auguste Tetenoire , J. Iñaki Juaristi , Maite Alducin

In the present work, we study the structures and molecular geometries of $CH_{4}$, $SO_{2}$ and $O_{2}$ adsorbed on $Cr_{2}O_{3}(0001)$. Using computational calculations based on the density functional theory (DFT), we analyze the most…

Chemical Physics · Physics 2016-12-05 S. N. Hernández Guiance , D. Coria , I. M. Irurzun , E. E. Mola

Ab initio self-consistent total energy calculations using second order Moller-Plesset perturbation theory and Hay-Wadt effective core potentials for gallium and arsenic have been used to investigate the chemisorption of atomic oxygen on the…

Condensed Matter · Physics 2007-05-23 Michael L. Mayo , Asok K. Ray

We present a density-functional theory study addressing the on-surface adsorption of oxygen at the Pd(11N) (N =3,5,7) vicinal surfaces, which exhibit (111) steps and (100) terraces of increasing width. We find the binding to be…

Materials Science · Physics 2007-05-23 Yongsheng Zhang , Jutta Rogal , Karsten Reuter

Improving reactivity on an insulating surface is crucial due to their important applications in surface catalytic reactions. In this work, we carried out first-principles calculations to investigate the adsorption of O2 on a single-layer…

Materials Science · Physics 2017-09-20 Cequn Li , Jing Fan , Bin Xu , Hu Xu

We present a comprehensive density-functional theory study addressing the adsorption, dissociation and successive diffusion of water molecules on the two regular terminations of SrTiO3(001). Combining the obtained supercell-geometry…

Materials Science · Physics 2015-05-18 Hannes Guhl , Wolfram Miller , Karsten Reuter

A plane-wave density functional theory is used to predict the work functions of Au/Mg decorated Au(100), Mg(001), and stochiometric AuMg alloy surfaces. We find, that irrespective of the details, all Au/Mg systems containing Mg on the…

Materials Science · Physics 2014-09-09 Matúš Dubecký , František Dubecký

The adsorption of volatile molecules onto dust grain surfaces fundamentally influences dust-related processes, including condensation of gas-phase molecules, dust coagulation, and planet formation in protoplanetary disks. Using advanced…

Earth and Planetary Astrophysics · Physics 2026-03-05 Lile Wang , Feng Long , Haifeng Yang , Ruobing Dong , Shenzhen Xu

When two or more atoms bind to a solid surface, the substrate can mediate an interaction between them. In this paper, we use density-functional theory to quantify the substrate-mediated pair interaction between two adatoms on a…

Materials Science · Physics 2007-05-23 Kristen A. Fichthorn , Matthias Scheffler

First principles electronic structure calculations based on density functional theory have been used to study the thermodynamic, structural and transport properties of solid solutions and liquid alloys of iron and oxygen at Earth's core…

Geophysics · Physics 2009-10-31 Dario Alfe` , G. David Price , Michael J. Gillan

The density functional theory (DFT) is used in a study of point defects on both UN (001) surface and sub-surface layers. We compare results for slabs of different thicknesses (both perfect and containing nitrogen or uranium vacancies) with…

Materials Science · Physics 2012-11-27 Dmitry Bocharov , Denis Gryaznov , Yuri F. Zhukovskii , Eugene A. Kotomin

First-principles density-functional theory and supercell models are employed to calculate the adsorption of water molecules on the Cu(100) surface. In agreement with the experimental observations, the calculations show that a H2O molecule…

Materials Science · Physics 2009-09-29 Sanwu Wang , Yanzhao Cao , P. A. Rikvold

Silver chromate ($\mathrm{Ag_{2}CrO_{4}}$) has attracted considerable attention in recent years due to its promising photocatalytic performance, which strongly depends on the crystallographic orientation of its exposed surfaces. A detailed…

Materials Science · Physics 2026-05-20 Augusto Facundes , Thiago T. Dorini , Theodora W. von Zuben , Miguel A. San-Miguel

Diamond displays outstanding chemical, physical, and tribological properties, making it attractive for numerous applications ranging from biomedicine to tribology. However, the reaction of the materials with molecules present in the air,…

Materials Science · Physics 2023-04-28 Nam V. Tran , M. C. Righi
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