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Theoretical rotational quenching cross sections and rate coefficients of ortho- and para-H$_2$O due to collisions with He atoms are presented. The complete angular momentum close-coupling approach as well as the coupled-states approximation…

Solar and Stellar Astrophysics · Physics 2015-06-15 Benhui Yang , M. Nagao , W. Satomi , M. Kimura , P. C. Stancil

We demonstrate rotational excitation of molecular ions that are sympathetically cooled by laser-cooled atomic ions to a temperature as low as ca. 10 mK. The molecular hydrogen ions HD+ and the fundamental rotational transition $(v=0,\,…

Quantum Physics · Physics 2013-11-05 J. Shen , A. Borodin , M. Hansen , S. Schiller

The absence of large cooling flows in cool core clusters appears to require self-regulated energy feedback by active galactic nuclei (AGNs) but the exact heating mechanism has not yet been identified. Here, we analyse whether a combination…

Astrophysics of Galaxies · Physics 2017-04-27 Svenja Jacob , Christoph Pfrommer

The kinetic energy of solid neon is calculated by a path-integral Monte Carlo approach with a refined Trotter- and finite-size extrapolation. These accurate data present significant quantum effects up to temperature T=20 K. They confirm…

Statistical Mechanics · Physics 2009-10-30 Alessandro Cuccoli , Alessandro Macchi , Gaia Pedrolli , Valerio Tognetti , Ruggero Vaia

We present several approximate calculations of the specific heat capacity of the model for Ca$_{10}$Cr$_7$O$_{28}$ proposed by Balz et al. [Phys. Rev. B 95, 174414 (2017)], using methods including exact diagonalization, Thermal Pure Quantum…

Strongly Correlated Electrons · Physics 2024-05-21 Joe Crossley , Chris Hooley

We present quantum dynamical calculations that describe the rotational excitation of H$_2$O due to collisions with H atoms. We used a recent, high accuracy potential energy surface, and solved the collisional dynamics with the…

Astrophysics of Galaxies · Physics 2015-06-23 F. Daniel , A. Faure , P. J. Dagdigian , M. -L. Dubernet , F. lique , G. Pineau des forêts

Using a high-sensitivity torsional oscillator technique, we mapped the rotational and relaxational dynamics of solid helium-4 throughout the parameter range of the proposed supersolidity. We found evidence that the same microscopic…

Other Condensed Matter · Physics 2011-06-16 E. J. Pratt , B. Hunt , V. Gadagkar , M. Yamashita , M. J. Graf , A. V. Balatsky , J. C. Davis

We present Submillimeter Array observations, in the 1.3 mm continuum and the CH_3CN(12-11) line of 17 hot molecular cores associated with young high-mass stars. The angular resolution of the observations ranges from 1".0 to 4".0. The…

Astrophysics of Galaxies · Physics 2015-06-18 Vicente Hernández-Hernández , Luis Zapata , Stan Kurtz , Guido Garay

Theoretical model of the nuclear spin conversion in formaldehyde (H2CO) has been developed. The conversion is governed by the intramolecular spin-rotation mixing of molecular ortho and para states. The rate of conversion has been found…

Chemical Physics · Physics 2009-11-06 Pavel L. Chapovsky

{\bf R}-matrix calculations combined with the adiabatic nuclei approximation are used to compute electron-impact rotiational excitation rates for three closed-shell diatomic cations, HeH$^+$, CH$^+$, ArH$^+$. Comparisons with previous…

Astrophysics of Galaxies · Physics 2015-12-02 James R. Hamilton , Alexandre Faure , Jonathan Tennyson

We present Submillimeter Array observations of the massive star-forming region IRAS 20126+4104 in the millimeter continuum and in several molecular line transitions. With the SMA data, we have detected nine molecular transitions, including…

Solar and Stellar Astrophysics · Physics 2015-05-30 Jin-Long Xu , Jun-Jie Wang , Chang-chun Ning

First theoretical analysis of the nuclear spin conversion in ethylene molecules (13^CCH4) has been performed. The conversion rate was found equal approx. 3x10^{-4} 1/s*Torr, which is in qualitative agreement with the recently obtained…

Chemical Physics · Physics 2009-11-06 P. L. Chapovsky , E. Ilisca

The excess heat capacity at glass transition temperature in two types of glass-forming systems of [xNaNO3\cdot(1-x)KNO3]60[Ca(NO3)2]40 (0 \leq x \leq 1) and Ca(NO3)2\cdotyH2O (4 \leq y \leq 13) is studied. In the former system, with the…

Statistical Mechanics · Physics 2011-11-22 H. B. Ke , P. Wen , W. H. Wang

A phenomenological description for the dynamical spin susceptibility $\chi({\bf q},\omega;T)$ observed in inelastic neutron scattering measurements on powder samples of LiV$_2$O$_4$ is developed in terms of the parametrized self-consistent…

Strongly Correlated Electrons · Physics 2009-11-13 V. Yushankhai , P. Thalmeier , T. Takimoto

We use molecular dynamics simulations to probe the rotational dynamics of the SPC/E model of water for a range of temperatures down to 200 K, 13 K above to the mode coupling temperature. We find that rotational dynamics is spatially…

Soft Condensed Matter · Physics 2015-06-25 Marco G. Mazza , Nicolas Giovambattista , Francis W. Starr , H. Eugene Stanley

We present quantum calculations of the rotational energy levels and spectroscopic rotational constants of the linear OCS molecule in variable size clusters of 4He, using spectral evolution quantum Monte Carlo methods that allow excited…

Condensed Matter · Physics 2009-11-07 F. Paesani , A. Viel , F. A. Gianturco , K. B. Whaley

Results for energy levels, radiative rates and electron impact excitation (effective) collision strengths for transitions in Be-like Cl XIV, K XVI and Ge XXIX are reported. For the calculations of energy levels and radiative rates the…

Solar and Stellar Astrophysics · Physics 2015-06-22 K. M. Aggarwal , F. P. Keenan

We compute the rotational quenching rates of the first 81 rotational levels of ortho- and para-H2CO in collision with ortho- and para-H2, for a temperature range of 10-300 K. We make use of the quantum close-coupling and coupled-states…

Solar and Stellar Astrophysics · Physics 2015-06-15 Laurent Wiesenfeld , Alexandre Faure

A variationally computed $^{28}$SiH$_4$ rotation-vibration line list applicable for temperatures up to $T=1200\,$K is presented. The line list, called OY2T, considers transitions with rotational excitation up to $J=42$ in the wavenumber…

Chemical Physics · Physics 2017-12-29 A. Owens , A. Yachmenev , W. Thiel , J. Tennyson , S. N. Yurchenko

The kinetic energy of H and O nuclei has been studied by path integral molecular dynamics simulations of ice Ih and water at ambient pressure. The simulations were performed by using the q-TIP4P/F model, a point charge empirical potential…

Materials Science · Physics 2011-09-01 R. Ramirez , C. P. Herrero