English

Observation of a rotational transition in trapped and sympathetically cooled molecular ions

Quantum Physics 2013-11-05 v1 Atomic Physics

Abstract

We demonstrate rotational excitation of molecular ions that are sympathetically cooled by laser-cooled atomic ions to a temperature as low as ca. 10 mK. The molecular hydrogen ions HD+ and the fundamental rotational transition (v=0,N=0)(v=0,N=1)(v=0,\, N=0)\rightarrow(v'=0,\, N'=1) at 1.3 THz, the most fundamental dipole-allowed rotational transition of any molecule, are used as a test case. This transition is here observed for the first time directly. Rotational laser cooling was employed in order to increase the signal, and resonance-enhanced multiphoton dissociation was used as detection method. The black-body-radiation-induced rotational excitation is also observed. The extension of the method to other molecular species is briefly discussed.

Keywords

Cite

@article{arxiv.1202.5672,
  title  = {Observation of a rotational transition in trapped and sympathetically cooled molecular ions},
  author = {J. Shen and A. Borodin and M. Hansen and S. Schiller},
  journal= {arXiv preprint arXiv:1202.5672},
  year   = {2013}
}