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Related papers: Exciton-relaxation dynamics in lead halides

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We investigate the dynamics of the exciton formation and relaxation on a picosecond time scale following a pulsed photoexcitation of a semiconductor. The study is conducted in the framework of the density matrix theory complemented with the…

Mesoscale and Nanoscale Physics · Physics 2015-12-25 Veljko Janković , Nenad Vukmirović

We develop a general theory for how an exciton in an atomically thin transition metal dichacogenide (TMD) monolayer couples to spin and charge correlations in an adjacent moire lattice created by a TMD bi-layer. Virtual tunneling of charge…

Mesoscale and Nanoscale Physics · Physics 2024-08-06 Aleksi Julku , Shanshan Ding , Georg M. Bruun

Electron-hole excitations in the surface bands of GaAs(110) are analyzed using constrained density-functional theory calculations. The results show that Frenkel-type autolocalized excitons are formed. The excitons induce a local surface…

mtrl-th · Physics 2016-09-07 Oleg Pankratov , Matthias Scheffler

In order to reveal the relaxation mechanism of photogenerated charge-transfer excitations in quasi-one-dimensional halogen-bridged diplatinum complexes, we calculate the low-lying adiabatic potential energy surfaces of a one-dimensional…

Strongly Correlated Electrons · Physics 2009-11-11 Jun Ohara , Shoji Yamamoto

An exciton-polariton microcavity that incorporates magnetic ions can exhibit a spontaneous self-trapping phenomenon which is an analog of the classical polaron effect. We investigate in detail the full model of a polariton condensate that…

Quantum Gases · Physics 2018-11-14 Paweł Miętki , Michał Matuszewski

Electron-hole bound pairs, or excitons, are common excitations in semiconductors. They can spontaneously form and ``condense'' into a new insulating ground state -- the so-called excitonic insulator -- when the energy of electron-hole…

The exciton relaxation dynamics of photoexcited electronic states in poly($p$-phenylenevinylene) (PPV) are theoretically investigated within a coarse-grained model, in which both the exciton and nuclear degrees of freedom are treated…

Chemical Physics · Physics 2018-02-14 Jonathan R. Mannouch , William Barford , Sarah Al-Assam

The interplay of migration, recombination, and dissociation of excitons in disordered media is studied theoretically in the low temperature regime. An exact expression for the photoluminescence spectrum is obtained. The theory is applied to…

Condensed Matter · Physics 2009-10-28 M. C. J. M. Vissenberg , M. J. M. de Jong

We study the relaxation of the exciton spin (longitudinal relaxation time $T_{1}$) in single asymmetrical quantum dots due to an interplay of the short--range exchange interaction and acoustic phonon deformation. The calculated relaxation…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 E. Tsitsishvili , R. v. Baltz , H. Kalt

We proposed in an earlier paper [arXiv:1108.6141] an empirical formula of the electrical conductivity which agrees with experiments within 20 percent for the most of pure elemental metals at room temperature ranges. This is obtained, in…

Statistical Mechanics · Physics 2011-09-28 Tadashi Hirayama

In this paper we present a study of an exciton system where electrons and holes are confined in double quantum well structures. The dominating interaction between excitons in such systems is a dipole - dipole repulsion. We show that the…

Quantum Gases · Physics 2015-05-13 B. Laikhtman , R. Rapaport

We present a theoretical study of the formation of self-trapped excitons (STEs) and the associated broadband emission in metal-halide perovskites Cs$_4$SnBr$_6$ and Cs$_2$AgInCl$_6$, using time-dependent density functional theory (TDDFT)…

Materials Science · Physics 2024-04-10 Yu Jin , Mariami Rusishvili , Marco Govoni , Giulia Galli

Bound electron-hole excitonic states are generally not expected to form with charges of negative effective mass. We identify such excitons in a single layer of the semiconductor WSe2, where they give rise to narrow-band upconverted…

We present a detailed numerical study of the one-dimensional Holstein model with a view to understanding the self-trapping process of electrons or excitons in crystals with short-range particle-lattice interactions. Applying a very…

Strongly Correlated Electrons · Physics 2009-10-30 G. Wellein , H. Fehske

Lead-free metal halide perovskites are emerging as less-toxic alternatives to their lead-based counterparts. However, their applicability in optoelectronic devices is limited, and the charge transport dynamics remain poorly understood.…

Exciton condensation indicating the spontaneous formation of electron-hole pair can cause the phase transition from a semimetal to an excitonic insulator by gap opening at the Fermi surface. While the idea of this excitonic insulator has…

Materials Science · Physics 2022-08-23 Hsiao-Yi Chen , Takuya Nomoto , Ryotaro Arita

Excitons in semiconductors may form correlated phases at low temperatures. We report the observation of an exciton liquid in GaAs/AlGaAs coupled quantum wells. Above a critical density and below a critical temperature the photogenerated…

Mesoscale and Nanoscale Physics · Physics 2015-03-13 Michael Stern , Vladimir Umansky , Israel Bar-Joseph

We study the light-absorbing states of the mixed-halide perovskite CH$_{3}$NH$_{3}$PbI$_2$Cl and tri-iodide perovskite CH$_{3}$NH$_{3}$PbI$_3$ with density functional and many-body calculations to explain the desirable photovolatic features…

Materials Science · Physics 2014-11-06 Ravindra Nanguneri , John Parkhill

Excitons are two-particle correlated bound states that are formed due to Coulomb interaction between single-particle holes and electrons. In the solid-state, cooperative interactions with surrounding quasiparticles can strongly tailor the…

While polarons --- charges bound to a lattice deformation induced by electron-phonon coupling --- are primary photoexcitations at room temperature in bulk metal-halide hybrid organic-inorganic perovskites (HOIP), excitons --- Coulomb-bound…

Materials Science · Physics 2020-04-14 Ajay Ram Srimath Kandada , Carlos Silva
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