Related papers: Spin Tunneling in Magnetic Molecules: Quasisingula…
We study spin tunneling in magnetic molecules, with special reference to Fe8. The article aims to give a pedagogical discussion of what is meant by the tunneling of a spin, and how tunneling amplitudes or energy level splittings may be…
Coherent state path integrals are shown in general to contain instantons with jumps at the boundaries, i.e., with boundary points lying outside classical parameter or phase space. As an example, the magnetic molecule Fe_8 is studied using a…
The perfect quenching of spin tunneling that has previously been discussed in terms of interfering instantons, and has recently been observed in the magnetic molecule \Fe8, is treated using a discrete phase integral (or…
The perfect quenching of spin tunneling first predicted for a model with biaxial symmetry, and recently observed in the magnetic molecule Fe_8, is further studied using the discrete phase integral (or Wentzel-Kramers-Brillouin) method. The…
We study spin tunnelling in molecular magnets as an instance of a mesoscopic phenomenon, with special emphasis on the molecule Fe8. We show that the tunnel splitting between various pairs of Zeeman levels in this molecule oscillates as a…
Spin tunneling in the particular case of the magnetic molecular cluster octanuclear iron(III), Fe8, is treated by an effective Hamiltonian that allows for an angle-based description of the process. The presence of an external magnetic field…
Tunneling between the two lowest energy levels of single molecule magnets with Ising type anisotropy, accompanied by the emission or absorption of phonons, is considered. Quantitatively accurate calculations of the rates for such tunneling…
We investigate the topological quenching of spin tunneling in Mn_12-acetate molecules with an applied magnetic field along the hard axis. The model Hamiltonian describing this system has a fourth-order term due to the tetragonal anisotropy.…
We use an instanton approximation to the continuous-time spin coherent-state path integral to obtain the tunnel splitting of classically degenerate ground states. We show that provided the fluctuation determinant is carefully evaluated, the…
Tunnel splitting oscillations in magnetic molecules are reconsidered within the simplest model for the problem, which does not contain fourth order anisotropy. It is shown that at large magnetic field, there is only one instanton, and it is…
The ground state tunnel splitting for the biaxial spin model in the magnetic field, H = -D S_{x}^2 + E S_{z}^2 - g \mu_B S_z H_z, has been investigated using an instanton approach. We find a new type of spin instanton and a new quantum…
Starting from a phenomenological Hamiltonian originally written in terms of angular momentum operators we derive a new quantum angle-based Hamiltonian that allows for a discussion on the quantum spin tunneling. The study of the…
Intermediate spin, which occurs in the theory of anyons, can also be exhibited by mesoscopic magnetic particles. The necessary broken time reversal symmetry is due to a suitably directed magnetic field. As a function of this field a system…
This article presents a review on the theoretical and the experimental developments on macroscopic quantum tunneling and phase transition of the escape rate in spin systems. We present the basic ideas with simplified calculations so that it…
Renormalized tunnel splitting with a finite distribution in the biaxial spin model for molecular magnets is obtained by taking into account the dipolar interaction of enviromental spins. Oscillation of the resonant tunnel splitting with a…
We analyze the interference between tunneling paths that occurs for a spin system with special Hamiltonian both for dipole and quadrupole excitation. Using an instanton approach, we find that as the strength of the second-order transverse…
The quantum-classical transitions of the escape rates in a uniaxial spin model relevant to the molecular magnet Mn$_{12}$Ac and a biaxial anisotropic ferromagnetic particle are investigated by applying the periodic instanton method. The…
We have investigated analytically quantum tunneling of large spin in the biaxial spin system with the magnetic field applied along the hard and medium anisotropy axes by using a purely quantum-mechanical approach. When the magnetic field…
The spin Hamiltonian that describes the molecular magnet Fe$_8$ has biaxial symmetry with mutually perpendicular easy, medium, and hard magnetic axes. Previous calculations of the ground state tunnel splittings in the presence of a magnetic…
Quantum phase interference and spin-parity effects are studied in biaxial molecular magnets in a magnetic field at an arbitrarily directed angle. The calculations of the ground-state tunnel splitting are performed on the basis of the…