English

Periodic Instanton and Phase Transition in Quantum Tunneling of Spin Systems

Soft Condensed Matter 2009-10-31 v2 Mesoscale and Nanoscale Physics

Abstract

The quantum-classical transitions of the escape rates in a uniaxial spin model relevant to the molecular magnet Mn12_{12}Ac and a biaxial anisotropic ferromagnetic particle are investigated by applying the periodic instanton method. The effective free energies are expanded around the top of the potential barrier in analogy to Landau theory of phase transitions. We show that the first-order transitions occur below the critical external magnetic field hx=1/4h_x = 1/4 for the uniaxial spin model and beyond the critical anisotropy constant ratio λ=1/2\lambda = 1/2 for the biaxial ferromagnetic grains, which are in good agreement with earlier works.

Keywords

Cite

@article{arxiv.cond-mat/9901325,
  title  = {Periodic Instanton and Phase Transition in Quantum Tunneling of Spin Systems},
  author = {Y. -B. Zhang and Y. -H. Nie and S. -P. Kou and J. -Q. Liang and H. J. W. Mueller-Kirsten and F. -C. Pu},
  journal= {arXiv preprint arXiv:cond-mat/9901325},
  year   = {2009}
}

Comments

14 pages, revtex, 5 postscript figures