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We report an unprecedented quantum criticality crossover representing two different universal scaling behaviors in a Kitaev quantum magnetic material $\alpha$-RuCl$_3$. $\alpha$-RuCl$_3$ presents both a symmetry breaking antiferromagnetic…

Strongly Correlated Electrons · Physics 2023-06-13 Jae-Ho Han , Seung-Hwan Do , Kwang-Yong Choi , Sang-Youn Park , Jae-You Kim , Sungdae Ji , Ki-Seok Kim , Jae-Hoon Park

We report the crystal structure, magnetization measurements, and band-structure calculations for the spin-1/2 quantum magnet CaCu2(SeO3)2Cl2. The magnetic behavior of this compound is well reproduced by a uniform spin-1/2 chain model with…

We report $^{75}$As NMR measurements on the new quasi one-dimensional superconductor K$_{2}$Cr$_{3}$As$_{3}$ ($T_{c} \sim 6.1$~K) [J.\ K.\ Bao et al., Phys. Rev. X {\bf 5}, 011013 (2015)]. We found evidence for strong enhancement of Cr spin…

Superconductivity · Physics 2015-11-09 H. Z. Zhi , T. Imai , F. L. Ning , Jin-Ke Bao , Guang-Han Cao

Finding distinct signatures of a quantum spin liquid (QSL) is an ongoing quest in condensed matter physics, invariably complicated by the presence of disorder in real materials. In this regard the 2D Kagome system…

Strongly Correlated Electrons · Physics 2024-01-22 B. S. Shivaram , J. Prestigiacomo , Aini Xu , Zhenyuan Zeng , Trevor D. Ford , Itamar Kimchi , Shiliang Li , Patrick A. Lee

Using inelastic neutron scattering, x-ray, neutron diffraction, and the first-principle calculation techniques, we show that the crystal structure of the two-dimensional quantum spin system (CuCl)LaNb$_2$O$_7$ is orthorhombic with $Pbam$…

Strongly Correlated Electrons · Physics 2015-05-19 C. Tassel , J. Kang , C. Lee , O. Hernandez , Y. Qiu , W. Paulus , E. Collet , B. Lake , T. Guidi , M. -H. Whangbo , C. Ritter , H. Kageyama , S. -H. Lee

The quantum spin liquid (QSL) is an exotic phase of magnetic materials where the spins continue to fluctuate without any symmetry breaking down to zero temperature. Among the handful reports of QSL with spin $S\ge$1, examples with magnetic…

We report on a 203Tl and 205Tl nuclear magnetic resonance study of the chain ternary semiconductor TlTaS3. We show that spin-lattice relaxation in this compound is driven by two contributions, namely by interactions of nuclear spins with…

Other Condensed Matter · Physics 2009-11-13 A. M. Panich , C. L. Teske , W. Bensch

The dimerized S=1/2 spins of the Cu ions in TlCuCl3 are ordered antiferromagnetically in the presence of a field larger than about 54 kOe in the zero-temperature limit. Within the mean-field approximation all thermal effects are frozen out…

Strongly Correlated Electrons · Physics 2015-05-13 Jens Jensen , Henrik Smith

Crystal and magnetic structures of a series of novel quantum spin trimer system Ca3Cu3xNix(PO4)4 (x=0,1,2) were studied by neutron powder diffraction at the temperatures 1.5-290 K. The composition with one Ni per trimer (x=1) has a…

Materials Science · Physics 2009-11-13 V. Yu. Pomjakushin , A. Furrer , D. V. Sheptyakov , E. V. Pomjakushina , K. Conder

We report the results of Cu and Cl nuclear magnetic resonance experiments (NMR) and thermal expansion measurements in magnetic fields in the coupled dimer spin system TlCuCl3. We found that the field-induced antiferromagnetic transition as…

Strongly Correlated Electrons · Physics 2009-11-10 O. Vyaselev , M. Takigawa , A. Vasiliev , A. Oosawa , H. Tanaka

Inelastic neutron scattering is employed to study transverse spin correlations of a Heisenberg $S=1/2$ chain compound in a magnetic field of 7.5 T. The target compound is the antiferromagnetic Heisenberg $S=1/2$ chain material…

Strongly Correlated Electrons · Physics 2015-09-18 M. Hälg , D. Hüvonen , N. P. Butch , F. Demmel , A. Zheludev

Elastic neutron scattering experiments performed in semi-conducting La(1-x)Ca(x)MnO3 single crystals (x=0.05, 0.08), reveal new features in the problem of electronic phase separation and metal insulator transition. Below TN, the observation…

Strongly Correlated Electrons · Physics 2009-10-31 M. Hennion , F. Moussa , G. Biotteau , J. Rodriguez-Carvajal , L. Pinsard , A. Revcolevschi

Temperature-dependent x-ray diffraction of the low-dimensional spin 1/2 quantum magnet TiOCl shows that the phase transition at T_{c2} = 90 K corresponds to a lowering of the lattice symmetry. Below T_{c1} = 66 K a twofold superstructure…

Materials Science · Physics 2009-11-11 M. Shaz , S. van Smaalen , L. Palatinus , M. Hoinkis , M. Klemm , S. Horn , R. Claessen

We present a systematic inelastic neutron scattering and neutron diffraction study of the magnetic structure of the quasi-1D spin-1/2 magnet SrCo2V2O8, where the interchain coupling in the Neel-type antiferromagnetic ground state breaks the…

Strongly Correlated Electrons · Physics 2022-03-04 L. Shen , E. Campillo , O. Zaharko , P. Steffens , M. Boehm , K. Beauvois , B. Ouladdiaf , Z. He , D. Prabhakaran , A. T. Boothroyd , E. Blackburn

Quantum correlations are a fundamental property of quantum many-body states. Yet they remain experimentally elusive, hindering certification of genuine quantum behavior, especially in quantum materials. Here we show that the…

Strongly Correlated Electrons · Physics 2024-08-29 Allen Scheie , Pontus Laurell , Elbio Dagotto , D. Alan Tennant , Tommaso Roscilde

The honeycomb compound $\alpha$-RuCl$_3$ is widely discussed as a proximate Kitaev spin-liquid material. This scenario builds on spin-orbit entangled $j = 1/2$ moments arising for a $t_{2g}^5$ electron configuration with strong spin-orbit…

Strongly Correlated Electrons · Physics 2020-10-21 P. Warzanowski , N. Borgwardt , K. Hopfer , T. C. Koethe , P. Becker , V. Tsurkan , A Loidl , M. Hermanns , P. H. M. van Loosdrecht , M. Grüninger

The isostructural series of $S=1$ quantum magnets Cs$_{1-x}$Rb$_{x}$FeCl$_{3}$ is investigated, using both thermodynamic measurements and inelastic neutron scattering experiments. It is found that increasing Rb content the system evolves…

Strongly Correlated Electrons · Physics 2019-12-11 S. Hayashida , L. Stoppel , Z. Yan , S. Gvasaliya , A. Podlesnyak , A. Zheludev

I study a spin system consisting of strongly coupled dimers which are in turn weakly coupled in a plane by zigzag interactions. The model can be viewed as the strong-coupling limit of a two-dimensional zigzag chain structure typical, e.g.,…

Strongly Correlated Electrons · Physics 2009-10-31 Alexei K. Kolezhuk

In this communication we consider the doping dependence of the strong antiferromagnetic spin fluctuations in the cuprate superconductors. We investigate the effect of an incommensurate magnetic response, as recently observed in inelastic…

Superconductivity · Physics 2016-08-15 Dirk K. Morr , Jörg Schmalian , David Pines

We performed high-resolution powder neutron diffraction experiments and discovered an elliptic helical incommensurate magnetic structure in the semiconducting rare-earth magnet YbCuS2, featuring effective spin-1/2 Yb$^{3+}$ ions that form a…

Strongly Correlated Electrons · Physics 2025-01-09 T. Onimaru , Y. Ohmagari , S. Mizutani , R. Yamamoto , H. Kaneshima , C. Moriyoshi , D. T. Adroja , D. Khyalyavin , P. Manuel , H. Saito , C. Hotta