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The frustrated magnet $\alpha$-RuCl$_3$ constitutes a fascinating quantum material platform that harbors the intriguing Kitaev physics. However, a consensus on its intricate spin interactions and field-induced quantum phases has not been…

Strongly Correlated Electrons · Physics 2021-07-16 Han Li , Hao-Kai Zhang , Jiucai Wang , Han-Qing Wu , Yuan Gao , Dai-Wei Qu , Zheng-Xin Liu , Shou-Shu Gong , Wei Li

$\alpha$-RuCl$_3$ has been extensively studied recently because of potential bond-dependent Kitaev magnetic exchange interactions and the resulting quantum spin liquid phase that can be realized therein. It has been known that the covalency…

Strongly Correlated Electrons · Physics 2022-01-13 Heung-Sik Kim

NH4CuCl3 has two magnetization plateaus at one-quarter and three-quarters of the saturation magnetization, irrespective of the external field direction. Magnetic excitations in NH4CuCl3 have been investigated by means of neutron inelastic…

Strongly Correlated Electrons · Physics 2007-05-23 A. Oosawa , T. Ono , K. Kakurai , H. Tanaka

The spin gap material IPA-CuCl3 has been extensively studied as a ferromagnetic-antiferromagnetic bondalternating S = 1/2 chain. This description of the system was derived from structural considerations and bulk measurements. New inelastic…

Strongly Correlated Electrons · Physics 2009-11-11 T. Masuda , A. Zheludev , H. Manaka , J. -H. Chung

Quantum spin liquids can arise from Kitaev magnetic interactions, and exhibit fractionalized excitations with the potential for a topological form of quantum computation. This review surveys recent experimental and theoretical progress on…

Neutron elastic and inelastic scattering measurements have been performed in order to investigate the spin structure and the magnetic excitations in the impurity-induced antiferromagnetic ordered phase of the doped spin gap system…

Strongly Correlated Electrons · Physics 2009-11-10 A. Oosawa , M. Fujisawa , K. Kakurai , H. Tanaka

Quasi-one-dimensional $A_2\text{Cr}_3\text{As}_3$ (with $A = \text{K, Cs, Rb}$) is an intriguing new family of superconductors which exhibit many similar features to the cuprate and iron-based unconventional superconductor families. Yet in…

Superconductivity · Physics 2017-11-29 K. M. Taddei , Q. Zheng , A. S. Sefat , C. de la Cruz

We investigate thermal and magnetic properties of the double spin chain compound KCuCl_3 via an exactly solved ladder model with strong rung interaction. Results from the analysis of the thermodynamic Bethe Ansatz equations suggests the…

Statistical Mechanics · Physics 2007-05-23 M. T. Batchelor , X. W. Guan , N. Oelkers

Recent studies have brought $\alpha$-RuCl$_3$ to the forefront of experimental searches for materials realizing Kitaev spin-liquid physics. This material exhibits strongly anisotropic exchange interactions afforded by the spin-orbit…

Strongly Correlated Electrons · Physics 2018-02-21 Stephen M. Winter , Kira Riedl , David Kaib , Radu Coldea , Roser Valenti

We report magnetization, nuclear magnetic resonance (NMR), nuclear quadrupole resonance (NQR), and transmission electron microscopy (TEM) studies on the quasi-two-dimensional spin-gap system (CuCl)LaNb2O7, a possible candidate for the J1-J2…

Strongly Correlated Electrons · Physics 2017-12-01 M. Yoshida , N. Ogata , M. Takigawa , J. Yamaura , M. Ichihara , T. Kitano , H. Kageyama , Y. Ajiro , K. Yoshimura

Alpha-phase (a-) RuCl_3 has emerged as a prime candidate for a quantum spin liquid (QSL) that promises exotic quasiparticles relevant for fault-tolerant quantum computation. Here, we report spin sensitive transport measurements to probe…

Strongly Correlated Electrons · Physics 2026-04-27 H. Idzuchi , M. Kimata , S. Okamoto , P. Laurell , N. Mohanta , M. Cothrine , S. E. Nagler , D. Mandrus , A. Banerjee , Y. P. Chen

Several Cu$^{2+}$ hydroxide minerals have recently been identified as candidate realizations of the $S=1/2$ kagome Heisenberg model. In this context, we have studied the distorted system KCu$_3$As$_2$O$_7$(OD)$_3$ using neutron scattering…

Neutron scattering has been used to study the magnetic order and spin dynamics of the colossal magnetoresistive pyrochlore Tl_2Mn_2O_7. On cooling from the paramagnetic state, magnetic correlations develop and appear to diverge at T_C (123…

Strongly Correlated Electrons · Physics 2009-10-31 J. W. Lynn , L. Vasiliu-Doloc , M. A. Subramanian

We have investigated the magnetic ground state properties of the quantum spin trimer compound strontium hydroxy copper chloride SrCu(OH)$_3$Cl using bulk magnetization, specific heat measurements, nuclear magnetic resonance (NMR), and…

The effect of exchange bond randomness on the ground state and the field-induced magnetic ordering was investigated through magnetization measurements in the spin-1/2 mixed quantum spin system (Tl$_{1-x}$K$_{x}$)CuCl$_3$ for $x<0.36$. Both…

Strongly Correlated Electrons · Physics 2016-08-31 A. Oosawa , H. Tanaka

We study the spin-wave excitations in $\alpha$-RuCl$_3$ by the spin-wave theory. Starting from the five-orbital Hubbard model and the perturbation theory, we derive an effective isospin-$1/2$ model in the large Hubbard ($U$) limit. Based on…

Strongly Correlated Electrons · Physics 2017-09-07 Wei Wang , Zhao-Yang Dong , Shun-Li Yu , Jian-Xin Li

We present a comparative study of the coupled-tetrahedra quantum spin systems Cu2Te2O5X2, X=Cl, Br (Cu-2252(X)) and the newly synthesized Cu4Te5O12Cl4 (Cu-45124(Cl)) based on ab initio Density Functional Theory calculations. The magnetic…

Strongly Correlated Electrons · Physics 2009-11-11 R. Valenti , T. Saha-Dasgupta , H. O. Jeschke , B. Rahaman , H. Rosner , P. Lemmens , R. Takagi , M. Johnsson

We study detailed classical-quantum correspondence for a cluster system of three spins with single-axis anisotropic exchange coupling. With autoregressive spectral estimation, we find oscillating terms in the quantum density of states…

Condensed Matter · Physics 2007-05-23 P. A. Houle , N. G. Zhang , C. L. Henley

Quantum criticality is a fundamental organizing principle for studying strongly correlated systems. Nevertheless, understanding quantum critical dynamics at nonzero temperatures is a major challenge of condensed matter physics due to the…

Strongly Correlated Electrons · Physics 2018-06-19 Jianda Wu , Wang Yang , Congjun Wu , Qimiao Si

The combination of electronic correlation and spin-orbit coupling is thought to precipitate a variety of highly unusual electronic phases in solids, including topological and quantum spin liquid states. We report a Raman scattering study…

Strongly Correlated Electrons · Physics 2015-04-22 Luke J. Sandilands , Yao Tian , Kemp W. Plumb , Young-June Kim , Kenneth S. Burch