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The way nuclear motion affects electronic responses has become a very hot topic in materials science. Coherent acoustic phonons can dynamically modify optical, magnetic and mechanical properties at ultrasonic frequencies, with promising…

Mesoscale and Nanoscale Physics · Physics 2018-08-29 Edoardo Baldini , Tania Palmieri , Adriel Dominguez , Pascal Ruello , Angel Rubio , Majed Chergui

Phonons are responsible for limiting both the electron mobility and the spin relaxation time in solids and provide a mechanism for thermal transport. In view of a possible transistor function as well as spintronics applications in graphene…

Mesoscale and Nanoscale Physics · Physics 2011-10-07 Matthias Droth , Guido Burkard

Silicon nanospheres are high-quality optical resonators and promising building blocks for Mie-tronic devices. While the Mie resonances of an isolated sphere are well understood, practical implementations require substrates that inevitably…

Classical continuum elastic calculations show that the acoustic vibrational modes of an embedded nanoparticle can be lightly damped even when the longitudinal plane wave acoustic impedances $Z_o=\rho v_L$ of the nanoparticle and the matrix…

Materials Science · Physics 2007-05-23 Lucien Saviot , Daniel B. Murray

Vibrational optical spectroscopies can be enhanced by surface plasmons to reach molecular-sized limits of detection and characterization. The level of enhancement strongly depends on microscopic details of the sample that are generally…

The effect of electron-phonon coupling on the current noise in a molecular junction is investigated within a simple model. The model comprises a 1-level bridge representing a molecular level that connects between two free electron…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Michael Galperin , Abraham Nitzan , Mark A. Ratner

The acoustic vibrations of single monomers and dimers of gold nanoparticles were investigated by measuring for the first time their ultra-low frequency micro-Raman scattering. This experiment provides access not only to the frequency of the…

The interplay between discrete vibrational and electronic degrees of freedom directly influences the chemical and physical properties of molecular systems. This coupling is typically studied through optical methods such as fluorescence,…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 B. J. LeRoy , S. G. Lemay , J. Kong , C. Dekker

Single-photon emitters are fundamental building blocks for quantum information processing, communication and sensing. However, unwanted interactions with bulk phonons in their host environment strongly limit their coherence and…

Vibrations in materials and nanostructures at sufficiently high temperatures result in anharmonic atomic displacements, which leads to new phenomena such as thermal expansion and multiphonon scattering processes, with a profound impact on…

Tailoring thermal properties with nanostructured materials can be of vital importance for many applications. Generally classical phonon size effects are employed to reduce the thermal conductivity, where strong phonon scattering by…

Applied Physics · Physics 2019-10-14 Yue Xiao , Qiyu Chen , Dengke Ma , Nuo Yang , Qing Hao

We investigate electron-phonon coupling in a narrow suspended metallic wire, in which the phonon modes are restricted to one dimension but the electrons behave three-dimensionally. Explicit theoretical results related to the known bulk…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 F. W. J. Hekking , A. O. Niskanen , J. P. Pekola

Boundary scattering in hierarchically disordered nanomaterials is an effective way to reduce the thermal conductivity of thermoelectric materials and increase their performance. In this work we investigate thermal transport in silicon based…

Materials Science · Physics 2019-02-27 Dhritiman Chakraborty , Laura de Sousa Oliveira , Neophytos Neophytou

We present a first-principles study of the confinement effects on the vibrational properties of thousand atoms (radii up to 16.2 {\AA}) colloidal III-V and II-VI nanoclusters. We describe how the molecular-type vibrations, such as…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Peng Han , Gabriel Bester

The coupling between a two-level system and its environment leads to decoherence. Within the context of coherent manipulation of electronic or quasiparticle states in nanostructures, it is crucial to understand the sources of decoherence.…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 P. Roulleau , S. Baer , T. Choi , F. Molitor , J. Güttinger , T. Müller , S. Dröscher , K. Ensslin , T. Ihn

Experiments have shown strong effects of some substrates on the localized plasmons of metallic nano particles but they are inconclusive on the affecting parameters. Here we have used Discrete Dipole Approximation in conjunction with…

Optics · Physics 2015-06-04 Murugesan Venkatapathi , Abhay K. Tiwari

We show that a quantum phase transition can occur in a phonon system in the presence of dislocations. Due to the competing nature between the topological protection of the dislocation and anharmonicity, phonons can reach a quantum critical…

A combination of the temporally and spatially resolved phonon spectroscopy has enabled calibration of hydrogen bond transition from the vibration mode of heavy water to the core/shelled nanodroplet and the subnanosized ionic hydration shell…

Chemical Physics · Physics 2018-11-30 Chang Q Sun

The electronic environment causes decoherence and dissipation of the collective surface plasmon excitation in metallic nanoparticles. We show that the coupling to the electronic environment influences the width and the position of the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Guillaume Weick , Gert-Ludwig Ingold , Rodolfo A. Jalabert , Dietmar Weinmann

Amorphous solids manifest puzzling effects of mysterious degrees of freedom that give rise to a heat capacity and phonon scattering in great excess over what would be expected for a solid that has a unique vibrational ground state. Of…

Disordered Systems and Neural Networks · Physics 2018-10-11 Vassiliy Lubchenko