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From ultraviolet to mid-infrared region, light-matter interaction mechanisms in semiconductors progressively shift from electronic transitions to phononic resonances and are affected by temperature. Here, we present a parallel…

Optics · Physics 2023-06-01 Zherui Han , Changkyun Lee , Jiawei Song , Haiyan Wang , Peter Bermel , Xiulin Ruan

First principles approaches have been successful in solving many-body Hamiltonians for real materials to an extent when correlations are weak or moderate. As the electronic correlations become stronger often embedding methods based on first…

We review our recent development of a first-principles lattice dynamics method that can treat anharmonic effects nonperturbatively. The method is based on the self-consistent phonon theory and temperature-dependent phonon frequencies can be…

Materials Science · Physics 2018-01-29 Terumasa Tadano , Shinji Tsuneyuki

We investigate the thermodynamics of one-dimensional Bose gases in the strongly correlated regime. To this end, we prepare ensembles of independent 1D Bose gases in a two-dimensional optical lattice and perform high-resolution in situ…

Discoveries of topological states and topological materials reshape our understanding of physics and materials over the last 15 years. First-principles calculations have been playing a significant role in bridging the theory of topology and…

Materials Science · Physics 2021-03-25 Jiewen Xiao , Binghai Yan

Realistic thermoelectric modeling and simulation tools are needed to explain the experiments and for device design. In this paper, we present a simple computational technique to make use of rigorous band structure calculations in…

Mesoscale and Nanoscale Physics · Physics 2011-10-12 Shuaib Salamat , Abhijeet Paul , Mehdi Salmani-Jelodar , Changwook Jeong , Gerhard Klimeck , Mark Lundstrom

We examine the influence of the main approximations employed in density-functional theory descriptions of the solid phase of molecular hydrogen near dissociation. We consider the importance of nuclear quantum effects on equilibrium…

Materials Science · Physics 2015-06-15 M. A. Morales , J. M. McMahon , C. Pierleoni , D. M. Ceperley

tructural transformation, pressure dependent elasticity behaviors, phonon, and thermodynamic properties of the equiatomic TiZr alloy are investigated by using first-principles density-functional theory. Our calculated lattice parameters and…

Materials Science · Physics 2011-12-06 Bao-Tian Wang , Wei-Dong Li , Ping Zhang

Multi-temperature models are nowadays often used to quantify the ultrafast electron-phonon (boson) relaxations and coupling strengths in advanced quantum solids. To test their applicability we study the time evolution of the electron…

Materials Science · Physics 2020-01-29 Manuel Obergfell , Jure Demsar

Using ab initio molecular-dynamics simulations combined with linear-response theory, we studied the x-ray absorption near-edge spectra (XANES) of a two-temperature dense copper plasma. As the temperature increases, XANES spectra exhibit a…

Materials Science · Physics 2020-04-01 N. Jourdain , V. Recoules , L. Lecherbourg , P. Renaudin , F. Dorchies

The thermal properties of bulk copper are investigated by performing ab initio DFT and DFPT calculations and using the quasiharmonic approximation for the free energy. Using both the LDA and the GGA for the exchange-correlation potential,…

Materials Science · Physics 2009-11-07 Shobhana Narasimhan , Stefano de Gironcoli

We performed a finite-temperature quantum Monte Carlo simulation of the one-dimensional spin-1/2 Heisenberg model with nearest-neighbor interaction coupled to Einstein phonons. Our method allows to treat easily up to 100 phonons per site…

Condensed Matter · Physics 2007-05-23 Rainer W. Kühne , Ute Löw

In this work we investigate temperature dependence of electronic structure of system with strong electronic correlations and strong electron-phonon interaction modeling cuprates in the frameworks of the three-band p-d-Holstein model by a…

Strongly Correlated Electrons · Physics 2018-01-03 Ilya A. Makarov , Sergey G. Ovchinnikov

We derive numerical tight-binding hopping parameters to describe conduction-band dispersion in arbitrary orientational phases of $A_3$C$_{60}$. The parameters are obtained by direct Fourier inversion of the spectra from self-consistent…

Condensed Matter · Physics 2009-10-22 S. C. Erwin , E. J. Mele

A model of charged hole-pair bosons, with long range Coulomb interactions and very weak interlayer coupling, is used to calculate the order parameter -Phi- of underdoped cuprates. Model parameters are extracted from experimental superfluid…

Superconductivity · Physics 2010-01-12 Alexander Mihlin , Assa Auerbach

We present a first-principles study of the relationship between stress, temperature and electronic properties in piezoelectric ZnO. Our method is a plane wave pseudopotential implementation of density functional theory and density…

Materials Science · Physics 2009-10-31 Nicola A. Hill , Umesh Waghmare

Electronic and phononic thermal conductivity are involved in the thermal conduction for metals and Wiedemann-Franz law is usually employed to predict them separately. However, Wiedemann-Franz law is shown to be invalid at intermediate…

Applied Physics · Physics 2020-11-18 Shouhang Li , Zhen Tong , Xinyu Zhang , Hua Bao

Motivated by interest in the elastic properties of high strength amorphous metals, we examine the elastic properties of select crystalline phases. Using first principles methods, we calculate elastic moduli in various chemical systems…

A first-principles-based method for computing phonons of magnetic random solid solutions including thermal magnetic fluctuations is developed. The method takes fluctuations of force constants (FCs) due to magnetic excitations as well as due…

Materials Science · Physics 2019-08-07 Yuji Ikeda , Fritz Körmann , Biswanath Dutta , Abel Carreras , Atsuto Seko , Jörg Neugebauer , Isao Tanaka

We use first-principles techniques to re-examine the suggestion that transitions seen in high-P experiments on Mo are solid-solid transitions from the bcc structure to either the fcc or hcp structures. We confirm that in the harmonic…

Materials Science · Physics 2015-05-28 Claudio Cazorla , Dario Alf`e , Michael J. Gillan