English

Tight-Binding Parametrization of First-Principles Electronic Dispersion in Orientationally Disordered A3c60

Condensed Matter 2009-10-22 v1

Abstract

We derive numerical tight-binding hopping parameters to describe conduction-band dispersion in arbitrary orientational phases of A3A_3C60_{60}. The parameters are obtained by direct Fourier inversion of the spectra from self-consistent electronic-structure calculations for K3_3C60_{60} using the local-density approximation, including the effects of orientational dependence. Using the new parameters, we revisit several earlier investigations of the orientational ordering in A3A_3C60_{60}; some of the earlier results are substantiated, while others are slightly modified.

Keywords

Cite

@article{arxiv.cond-mat/9402004,
  title  = {Tight-Binding Parametrization of First-Principles Electronic Dispersion in Orientationally Disordered A3c60},
  author = {S. C. Erwin and E. J. Mele},
  journal= {arXiv preprint arXiv:cond-mat/9402004},
  year   = {2009}
}

Comments

12 pages + 3 postscript figures (by request), REVTeX 3.0