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The 3d electronic structure and phase transition in pure and Cr doped V2O3 are theoretically investigated in relation to the 3d spin-orbit interaction and lattice distortion. A model consisting of the nearest-neighbor V ion pair with full…

Strongly Correlated Electrons · Physics 2016-08-31 Arata Tanaka

Spin correlations in metallic and insulating phases of $V_2O_3$ and its derivatives are investigated using magnetic neutron scattering. Metallic samples have incommensurate spin correlations varying little with hole doping. Paramagnetic…

Strongly Correlated Electrons · Physics 2009-10-28 Wei Bao , C. Broholm , G. Aeppli , P. Dai , J. M. Honig , P. Metcalf

We have performed x-ray linear and circular magnetic dichroism experiments at the Mn L2,3-edge of the La0.7Sr0.3MnO3 ultra thin films. Our measurements show that the antiferromagnetic (AF) insulating phase is stabilized by the interfacial…

Strongly Correlated Electrons · Physics 2009-07-29 C. Aruta , G. Ghiringhelli , V. Bisogni , L. Braicovich , N. B. Brookes , A. Tebano , G. Balestrino

Sm{0.5-x}Pr{x}Sr{0.5}MnO{3} exhibits variety of ground states as x is varied from 0 to 0.5. At an intermediate doping of x = 0.3 a charge-ordered CE type antiferromagnetic insulating (AFI) ground state is seen. The transition to this ground…

Strongly Correlated Electrons · Physics 2009-11-13 K. R. Priolkar , Vishwajeet Kulkarni P. R. Sarode , S. Emura

Vanadium Sesquioxide (V$_2$O$_3$) is an antiferromagnetic insulator below $T_{\mathrm N}\approx$ 155 K. The magnetic order is not of C- or G-type as one would infer from the bipartite character of the hexagonal basal plane in the…

Materials Science · Physics 2015-08-19 Daniel Grieger , Michele Fabrizio

Motivated by recent neutron, X-ray absorption and resonant scattering experiments, we revisit the electronic structure of V2O3. We propose a model in which S=1 V3+ ions are coupled in the vertical V-V pairs forming two-fold orbitally…

Strongly Correlated Electrons · Physics 2009-10-31 F. Mila , R. Shiina , F. -C. Zhang , A. Joshi , M. Ma , V. Anisimov , T. M. Rice

The short-range organization around Ni atoms in orthorhombic $R$NiO$_{3}$ ($R$=Pr,Nd,Eu) perovskites has been studied over a wide temperature range by Ni K-edge x-ray absorption spectroscopy. Our results demonstrate that two different Ni…

V2O3 famously features all four combinations of paramagnetic vs antiferromagnetic, and metallic vs insulating states of matter in response to %-level doping, pressure in the GPa range, and temperature below 300 K. Using time-of-flight…

Using the multi-band $d-p$ model and unrestricted Hartree-Fock approximation we investigate the electronic structure and spin-orbital order in three-dimensional VO$_3$ lattice. The main aim of this investigation is testing if simple $d-p$…

Strongly Correlated Electrons · Physics 2018-08-14 Krzysztof Rościszewski , Andrzej M. Oleś

Magnetic correlations in all four phases of pure and doped vanadium sesquioxide V_2O_3 have been examined by magnetic thermal neutron scattering. While the antiferromagnetic insulator can be accounted for by a Heisenberg localized spin…

Strongly Correlated Electrons · Physics 2009-10-31 Wei Bao , C. Broholm , G. Aeppli , S. A. Carter , P. Dai , T. F. Rosenbaum , J. M. Honig , P. Metcalf , S. F. Trevino

The electronic structure of vanadium sesquioxide in its different phases has been calculated using the screened exchange (sX) hybrid functional. The hybrid functional reproduces the electronic properties of all three phases, the…

Strongly Correlated Electrons · Physics 2013-03-22 Yuzheng Guo , Stewart J. Clark , John Robertson

We study URu$_{2-x}$Fe$_x$Si$_2$, in which two types of staggered phases compete at low temperature as the iron concentration $x$ is varied: the nonmagnetic "hidden order" (HO) phase below the critical concentration $x_c$, and…

Strongly Correlated Electrons · Physics 2016-11-30 H. -H. Kung , S. Ran , N. Kanchanavatee , V. Krapivin , A. Lee , J. A. Mydosh , K. Haule , M. B. Maple , G. Blumberg

We present a detailed ab initio study of the electronic structure and magnetic order of an Fe monolayer on the Ir(001) surface covered by adsorbed oxygen and hydrogen. The results are compared to the clean Fe/Ir(001) system, where recent…

Materials Science · Physics 2013-06-26 Frantisek Maca , Josef Kudrnovsky , Vaclav Drchal , Josef Redinger

Among the numerous 2D system that can be prepared via exfoliation, iron phosphorus trisulfide (FePS3) attracts a lot of attention recently due to its broad-range photoresponse, its unusual Ising-type magnetic order and possible applications…

Materials Science · Physics 2023-01-16 Mohammad Amirabbasi , Peter Kratzer

Polarization dependent x-ray absorption spectroscopy was used to study the magnetic ground state and the orbital occupation in bulk-phase VI$_3$ van der Waals crystals below and above the ferromagnetic and structural transitions. X-ray…

Strongly Correlated Electrons · Physics 2023-07-19 R. Sant , A. De Vita , V. Polewczyk , G. Pierantozzi , F. Mazzola , G. Vinai , G. van der Laan , G. Panaccione , N. B. Brookes

The effect of strong confinement on the positional and orientational ordering is examined in a system of hard rectangular rods with length L and diameter D (L>D) using the Parsons-Lee modification of the second virial density functional…

Soft Condensed Matter · Physics 2018-01-24 Roohollah Aliabadi , Peter Gurin , Enrique Velasco , Szabolcs Varga

The oxygen-deficient (double) perovskite YBaMn$_2$O$_5$, containing corner-linked MnO$_5$ square pyramids, is found to exhibit ferrimagnetic ordering in its ground state. In the present work we report generalized-gradient-corrected,…

Strongly Correlated Electrons · Physics 2009-11-07 R. Vidya , P. Ravindran , A. Kjekshus , H. Fjellvåg

We report evidence for phase coexistence of orbital orderings of different symmetry in SmVO$_3$ by high resolution X-Ray powder diffraction. The phase coexistence is triggered by an antiferromagnetic ordering of the vanadium spins near…

Strongly Correlated Electrons · Physics 2009-11-11 M. H. Sage , G. R. Blake , G. J. Nieuwenhuys , T. T. M. Palstra

We demonstrate that angle-resolved soft x-ray spectroscopy can resolve absorption by inequivalent oxygen sites and by different orbitals belonging to the same site in NaV2O5. By rotating the polarization direction, we see a dramatic change…

Strongly Correlated Electrons · Physics 2009-11-07 G. P. Zhang , G. T. Woods , Eric L. Shirley , T. A. Callcott , L. Lin , G. S. Chang , B. C. Sales , D. Mandrus , J. He

We report x-ray scattering studies of short-range structural correlations and diffuse scattering in Nd0.5Sr0.5MnO3. On cooling, this material undergoes a series of transitions, first from a paramagnetic insulating (PI) to a ferromagnetic…

Condensed Matter · Physics 2009-11-07 V. Kiryukhin , B. G. Kim , T. Katsufuji , J. P. Hill , S-W. Cheong
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