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Related papers: Evidence for short range orbital order in paramagn…

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We report the magnetic and electronic properties of the bilayer ruthenate Sr$_3$Ru$_2$O$_7$ upon Fe substitution for Ru. We find that Sr$_3$(Ru$_{1-x}$Fe$_x$)$_2$O$_7$ shows a spin-glass-like phase below 4 K for $x$ = 0.01 and commensurate…

Strongly Correlated Electrons · Physics 2018-02-21 M. Zhu , Y. Wang , P. G. Li , J. J. Ge , W. Tian , D. Keavney , Z. Q. Mao , X. Ke

The orbital, which represents the shape of the electron cloud, very often strongly influences the manifestation of various exotic phenomena, e.g., magnetism, metal-insulator transition, colossal magnetoresistance, unconventional…

Layered organic conductors (BEDO-TTF)_2ReO_4*H_2O (metal) and (BEDT-TTF)_xDy(NO_3)_z (paramagnetic insulator) are studied by CW-EPR and SQUID methods. A correlation in resonance and transport properties of both compounds is attributed to a…

Materials Science · Physics 2007-05-23 Yu. N. Shvachko , D. V. Starichenko , A. V. Korolyov , N. D. Kushch , E. B. Yagubskii

We have investigated possible spin and charge ordered states in 3d transition-metal oxides with small or negative charge-transfer energy, which can be regarded as self-doped Mott insulators, using Hartree-Fock calculations on d-p-type…

Strongly Correlated Electrons · Physics 2009-10-31 T. Mizokawa , D. I. Khomskii , G. A. Sawatzky

We found, using density-functional theory calculations within the generalized gradient approximation, that Cs$_2$AgF$_4$ is stabilized in the insulating orthorhombic phase rather than in the metallic tetragonal phase. The lattice distortion…

Materials Science · Physics 2007-10-23 Hua Wu , D. I. Khomskii

Resonant x-ray diffraction performed at the $\rm L_{II}$ and $\rm L_{III}$ absorption edges of Ru has been used to investigate the magnetic and orbital ordering in Ca$_2$RuO$_4$ single crystals. A large resonant enhancement due to electric…

Disentangling the relationship between the insulating state with a charge gap and the magnetic order in an antiferromagnetic (AF) Mott insulator remains difficult due to inherent phase separation as the Mott state is perturbed. Measuring…

Strongly Correlated Electrons · Physics 2022-03-17 He Zhao , Sujit Manna , Zach Porter , Xiang Chen , Andrew Uzdejczyk , Jagadeesh Moodera , Ziqiang Wang , Stephen D. Wilson , Ilija Zeljkovic

Motivated by recent results of $N$th order muffin-tin orbital (NMTO) implementation of the density functional theory (DFT), we re-examine low-temperature ground-state properties of the anti-ferromagnetic insulating phase of vanadium…

Strongly Correlated Electrons · Physics 2015-05-13 N. B. Perkins , S. Di Matteo , C. R. Natoli

The orbital, lattice, and spin ordering phenomena in KCuF3 are investigated by means of LDA+U calculations, based on ab-initio pseudopotentials.We examine the Cu-3d orbital ordering and the associated Jahn-Teller distortion in several…

Strongly Correlated Electrons · Physics 2009-11-10 N. Binggeli , M. Altarelli

The (SrTiO$_3$)$_m$/(SrVO$_3$)$_n$ $d^0-d^1$ multilayer system is studied with first principles methods through the observed insulator-to-metal transition with increasing thickness of the SrVO$_3$ layer. When correlation effects with…

Strongly Correlated Electrons · Physics 2015-05-19 Victor Pardo , Warren E. Pickett

Using a point-charge calculation of the electrostatic crystal field, we determine the non-degenerate orbital ground state of the ferromagnetic Mott insulator YTiO3, which is found to agree perfectly with experiment. Based on the orbital…

Strongly Correlated Electrons · Physics 2009-11-11 Robert Schmitz , Ora Entin-Wohlman , Amnon Aharony , Erwin Mueller-Hartmann

We have investigated the antiferromagnetic insulating phase of the Mott-Hubbard insulator V$_2$O$_3$ by resonant x-ray Bragg diffraction at the vanadium K-edge. Combining the information obtained from azimuthal angle scans, linear incoming…

Recent years have seen a vast increase in research into van der Waals magnetic materials. In many of these systems, magnetism is introduced via light 3\textit{d}-transition metal elements, combined with chalcogenides or halogens. Despite…

This article reports a detailed x-ray resonant scattering study of the bilayer iridate compound, Sr3Ir2O7, at the Ir L2 and L3 edges. Resonant scattering at the Ir L3 edge has been used to determine that Sr3Ir2O7 is a long-range ordered…

Strongly Correlated Electrons · Physics 2012-08-31 S. Boseggia , R. Springell , H. C. Walker , A. T. Boothroyd , D. Prabhakaran , D. Wermeille , L. Bouchenoire , S. P. Collins , D. F. McMorrow

We investigated the form of the orbital ordering in the electronic nematic phase of the Iron-based superconductors by applying a group theoretical analysis on a realistic five-band model. We find the orbital order can be either of the…

Superconductivity · Physics 2015-06-18 Yuehua Su , Haijun Liao , Tao Li

We present first-principles studies on the orbital states of the layered perovskites Ca$_{2-x}$Sr$_x$RuO$_4$. The crossover from antiferromagnetic (AF) Mott insulator for $x < 0.2$ to nearly ferromagnetic (FM) metal at $x=0.5$ is…

Strongly Correlated Electrons · Physics 2009-11-10 Zhong Fang , Naoto Nagaosa , Kiyoyuki Terakura

CuFeO_2 is one of the multiferroic materials and is the first case that the electric polarization is not explained by the magnetostriction model or the spin-current model. We have studied this material using soft x-ray resonant diffraction…

In the light of recent interesting experimental work on MgV$_2$O$_4$ we employ the density functional theory to investigate the crucial role played by different interaction parameters in deciding its electronic and magnetic properties. The…

Strongly Correlated Electrons · Physics 2011-09-15 Sudhir K. Pandey

The iron(III) center in ferroelectric PbTiO3 together with an oxygen vacancy forms a charged defect associate, oriented along the crystallographic c-axis. Its microscopic structure has been analyzed in detail comparing results from a…

The electronic structure and magnetism in the sodium nickelate NaNiO_2 in the low-temperature phase is studied from density-functional calculations using the linear muffin-tin orbitals method. An antiferromagnetic solution with a magnetic…

Strongly Correlated Electrons · Physics 2009-11-10 H. Meskine , S. Satpathy