Related papers: Boson peak in an harmonic scalar model
Glasses are amorphous solids, in the sense that they display elastic behaviour. In crystals, elasticity is associated with phonons, quantized sound-wave excitations. Phonon-like excitations exist also in glasses at very high frequencies…
We study a disordered vibrational model system, where the spring constants k are chosen from a distribution P(k) ~ 1/k above a cut-off value k_min > 0. We can motivate this distribution by the presence of free volume in glassy materials. We…
We show that a {\em vibrational instability} of the spectrum of weakly interacting quasi-local harmonic modes creates the maximum in the inelastic scattering intensity in glasses, the Boson peak. The instability, limited by anharmonicity,…
We show that the same physical mechanism is fundamental for two seemingly different phenomena such as the formation of two-level systems in glasses and the Boson peak in the reduced density of low-frequency vibrational states g(w)/w^2. This…
We perform molecular-dynamics simulations of the vibrational and the elasto-plastic properties of polymeric glasses and crystals and corresponding atomic systems. We evidence that the elastic scaling of the density of states in the…
We present an implementation of the analytical string theory recently applied to the description of glasses. These are modeled as continuum media with embedded elastic string heterogeneities, randomly located and randomly oriented, which…
The vibrational anomalies of glasses, in particular the boson peak, are addressed from the standpoint of heterogeneous elasticity, namely the spatial fluctuations of elastic constants caused by the structural disorder of the amorphous…
We present the results of extensive molecular dynamics computer simulations in which the high frequency dynamics of silica, nu>0.5 THz, is investigated in the viscous liquid state as well as in the glass state. We characterize the…
New temperature dependent inelastic x-ray (IXS) and Raman (RS) scattering data are compared to each other and with existing inelastic neutron scattering data in vitreous silica (v-SiO_2), in the 300 - 1775 K region. The IXS data show…
We conduct experiments on two-dimensional packings of colloidal thermosensitive hydrogel particles whose packing fraction can be tuned above the jamming transition by varying the temperature. By measuring displacement correlations between…
We present a numerical simulation study of the density-dependence (rho = 2.2 - 4.0 g/cm^3) of the high-energy collective dynamics in vitreous silica at mesoscopic wavevectors (Q = 1 - 18 nm^-1). The density-dependence of the longitudinal…
Using molecular dynamics computer simulations we investigate the dynamics of supercooled silica in the frequency range 0.5-20~THz and the wave-vector range 0.13-1.1\AA^{-1}. We find that for small wave-vectors the dispersion relations are…
Despite the presence of topological disorder, phonons seem to exist also in glasses at very high frequencies (THz) and they remarkably persist into the supercooled liquid. A universal feature of such a systems is the Boson peak, an excess…
Many theories predict a quartic acoustic attenuation increase at sub-THz frequencies in glassy media for the excess vibrational modes known as the boson peak anomaly. Here by introducing phase-sensitive acoustic spectroscopy techniques with…
Amorphous materials exhibit peculiar mechanical and vibrational properties, including non-affine elastic responses and excess vibrational states, i.e., the so-called boson peak. For polymer glasses, these properties are considered to be…
The boson peak appears in all amorphous solids and is an excess of vibrational states at low frequencies compared to the phonon spectrum of the corresponding crystal. Until recently, the consensus was that it originated from "defects" in…
The boson peak is an excess in the phonon density of states relative to the Debye Model, which occurs at frequencies below the Debye limit. It is present in most amorphous materials and, as was recently shown, can sometimes be found also in…
The boson peak (BP), a low-energy excess in the vibrational density of states over the phonon Debye contribution, is usually identified as one of the distinguishing features between ordered crystals and amorphous solid materials. Despite…
We present in this paper a numerical study of the vibrational eigenvectors of a two-dimensional amorphous material, previously deeply studied from the point of view of mechanical properties and vibrational eigen-frequencies [7-10].…
A close inspection of neutron spectra of glass formers in the frequency region above the boson peak does not show the constant eigenvalue density expected for a random dynamical matrix, but a slow decrease towards higher eigenvalues. In…