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Through a combination of neutron diffraction and Landau theory we describe the spin ordering in the ground state of the quadruple perovskite manganite CaMn7O12 - a magnetic multiferroic supporting an incommensurate orbital density wave that…

Strongly Correlated Electrons · Physics 2016-05-25 R. D. Johnson , D. D. Khalyavin , P. Manuel , A. Bombardi , C. Martin , L. C. Chapon , P. G. Radaelli

We demonstrate that the half-doped bilayer manganite La_{1}Sr_{2}Mn_{2}O_{7} exhibits CE-type charge-ordered and spin-ordered states below $T_{N, CO}^A = 210$ K and below $T_{N}^{CE} \sim 145$ K, respectively. However, the volume fraction…

Strongly Correlated Electrons · Physics 2009-10-31 M. Kubota , H. Yoshizawa , Y. Moritomo , H. Fujioka , K. Hirota , Y. Endoh

The ferromagnetic and insulating state observed in La$_{1-x}$Ca$_{x}$MnO$_3$, 0.125$<$x$<$0.2, is characterized by structural and magnetic anomalies below T$_C$, similar to those observed in the x$_{Sr}$$\approx$1/8. A neutron scattering…

Strongly Correlated Electrons · Physics 2016-08-16 M. Hennion , F. Moussa , F. Wang , J. Rodríguez-Carvajal , Y. M. Mukovskii , D. Shulyatev

Experimental evidence supports the double-exchange (DE) mechanism for both in-plane and c-axis conductivity in the colossal-magnetoresistive (CMR) layered manganite La1.4Sr1.6Mn2O7. Below TC, the data determine both the DE and…

Condensed Matter · Physics 2007-05-23 Q. A. Li , K. E. Gray , J. F. Mitchell , A. Berger , R. Osgood

We report predominantly zero field muon spin relaxation measurements in a series of Ca-doped LaMnO_3 compounds which includes the colossal magnetoresistive manganites. Our principal result is a systematic study of the spin-lattice…

Strongly Correlated Electrons · Physics 2009-10-31 R. H. Heffner , J. E. Sonier , D. E. MacLaughlin , G. J. Nieuwenhuys , G. M. Luke , Y. J. Uemura , S-W. Cheong , G. Balakrishnan

The complicated electronic, magnetic, and colossal magnetoresistant (CMR) properties of Sr and Ca doped lanthanum manganites can be understood by spin-polarized first-principles calculations. The electronic properties can be attributed to a…

Strongly Correlated Electrons · Physics 2007-05-23 M. -H. Tsai , Y. -H. Tang , H. Chou , W. T. Wu

We report on the magnetic properties of the manganite Bi_{1-x}Ca_{x}MnO_3 (x=0.33) at low temperature. The analysis of the field expansion of the ac susceptibility and the observation of aging properties make clear that a spin glass phase…

Materials Science · Physics 2009-11-13 M. Giot , A. Pautrat , G. Andre , D. Saurel , M. Hervieu , J. Rodriguez-Carvajal

Recent DFT calculations for Ba2CoO4 (BCO) and neutron scattering experiments for SrRuO3 (SRO) have shown that oxygen develops a magnetic polarization. Moreover, DFT calculations for these compounds also unveiled unexpected nodes in the spin…

Strongly Correlated Electrons · Physics 2021-05-20 Ling-Fang Lin , Nitin Kaushal , Cengiz Şen , Andrew D. Christianson , Adriana Moreo , Elbio Dagotto

We report inelastic neutron scattering results on the spin dynamics in the 50 % hole-doped manganites, Pr{1/2}Sr{1/2}MnO3 and Nd{1/2}Sr{1/2}MnO3. In the paramagnetic phase, these systems exhibit a ridge-type diffuse scattering, indicating a…

Strongly Correlated Electrons · Physics 2007-05-23 H. Kawano , R. Kajimoto , H. Yoshizawa , Y. Tomioka , H. Kuwahara , Y. Tokura

An effective one-band Hamiltonian for colossal-magnetoresistance (CMR) manganites is constructed and the spin excitations are determined. Fitting the experimental data by the derived spin-wave dispersion gives an e_g -electron hopping…

Strongly Correlated Electrons · Physics 2016-08-31 J. Loos , H. Fehske

The spin correlations of the bilayer manganite $La_{1.2}Sr_{1.8}Mn_{2}O_{7}$ have been studied using neutron scattering. On cooling within the paramagnetic state, we observe purely two-dimensional behavior with a crossover to…

Strongly Correlated Electrons · Physics 2007-05-23 S. Rosenkranz , R. Osborn , L. Vasiliu-Doloc , J. W. Lynn , S. K. Sinha , J. F. Mitchell

We present diffraction data on a single-layered manganite La(0.42)Sr(1.58)MnO4 with hole doping (x>0.5). Overdoped La(0.42)Sr(1.58)MnO4 exhibits a complex ordering of charges, orbitals and spins. Single crystal neutron diffraction…

Strongly Correlated Electrons · Physics 2012-01-12 H. Ulbrich , D. Senff , P. Steffens , O. J. Schumann , Y. Sidis , P. Reutler , A. Revcolevschi , M. Braden

Neutron scattering investigations of the paramagnetic correlations in the layered manganite La$_{1.2}$Sr$_{1.8}$Mn$_{2}$O$_{7}$, which exhibits colossal magnetoresistance above the Curie transition at T$_C$ = 112 K, show that spins in…

Strongly Correlated Electrons · Physics 2009-10-30 R. Osborn , S. Rosenkranz , D. N. Argyriou , L. Vasiliu-Doloc , J. W. Lynn , S. K. Sinha , J. F. Mitchell , K. E. Gray , S. D. Bader

We investigate the high temperature phase of layered manganites, and demonstrate that the charge-orbital phase transition without magnetic order in La$_{0.5}$Sr$_{1.5}$MnO$_4$ can be understood in terms of the density wave instability. The…

Strongly Correlated Electrons · Physics 2013-04-17 Zi-Jian Yao , Wei-Qiang Chen , Jin-Hua Gao , Hong-Min Jiang , Fu-Chun Zhang

We have investigated orbital ordering in the half-doped manganite La$_{0.5}$Sr$_{1.5}$MnO$_4$, which displays spin, charge and orbital ordering, by means of unrestricted Hartree-Fock calculations on the multiband $p$-$d$ model. From recent…

Strongly Correlated Electrons · Physics 2009-11-11 K. Ebata , T. Mizokawa , A. Fujimori

When holes are doped into a Mott-Hubbard type insulator, like lightly doped manganites of the La(1-x)CaxMnO3 family, the cooperative Jahn-Teller distortions and the appearance of orbital ordering require an arrangement of Mn(3+)/Mn(4+) for…

Strongly Correlated Electrons · Physics 2009-11-10 G. Papavassiliou , M. Pissas , M. Belesi , M. Fardis , J. P. Ansermet , D. Carlier , C. Dimitropoulos , J. Dolinsek

Neutron spectroscopy measurements reveal short-range spin correlations near and above the ferromagnetic-paramagnetic phase transition in manganite materials of the form La$_{1-x}A_{x}$MnO$_{3}$, including samples with an insulating ground…

The magnetic and electrical properties of high quality single crystals of $A$-site disordered (solid solution) Ln$_{0.5}$Ba$_{0.5}$MnO$_3$ are investigated near the phase boundary between the spin glass insulator and…

Materials Science · Physics 2009-11-10 R. Mathieu , D. Akahoshi , A. Asamitsu , Y. Tomioka , Y. Tokura

Using x-ray and neutron scattering, we have studied the structural and magnetic properties of the single-layer manganite La{1-x}Sr{1+x}MnO4 (0 < x < 0.7). Single crystals were grown by the traveling-solvent floating-zone method at 18 La/Sr…

Strongly Correlated Electrons · Physics 2009-11-10 S. Larochelle , A. Mehta , L. Lu , P. K. Mang , O. P. Vajk , N. Kaneko , J. W. Lynn , L. Zhou , M. Greven

We discuss magnetotransport in a low density electron gas coupled to spin fluctuations near and above a ferromagnetic transition. Provided the density is low enough ($n \lesssim 1/\xi^{3}(T)$, with $\xi(T)$ the ferromagnetic correlation…

Materials Science · Physics 2009-10-30 Pinaki Majumdar , Peter Littlewood