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We present inelastic neutron scattering experiments on the $S=1/2$ frustrated gapped quantum magnet piperazinium hexachlorodicuprate under applied hydrostatic pressure. These results show that at 9 kbar the magnetic triplet excitations in…

Strongly Correlated Electrons · Physics 2015-09-02 G. Perren , J. S. Möller , D. Hüvonen , A. A. Podlesnyak , A. Zheludev

We report magnetic susceptibility, specific heat, and neutron scattering measurements as a function of applied magnetic field and temperature to characterize the $S=1/2$ quasi-two-dimensional frustrated magnet piperazinium…

Strongly Correlated Electrons · Physics 2009-11-11 M. B. Stone , C. Broholm , D. H. Reich , P. Schiffer , O. Tchernyshyov , P. Vorderwisch , N. Harrison

We report a comprehensive microscopic study of the frustrated quantum magnet PHCC, (C$_4$H$_{12}$N$_2$)Cu$_2$Cl$_6$, using density-functional band-structure calculations combined with numerical quantum many-body simulations of the…

Strongly Correlated Electrons · Physics 2025-12-22 Alexander A. Tsirlin , Oleg Janson , Ioannis Rousochatzakis

Inelastic neutron scattering measurements are reported for the quantum antiferromagnetic material Cu_2(C_5H_12N_2)_2Cl_4 (CuHpCl). The magnetic excitation spectrum forms a band extending from 0.9 meV to 1.4 meV. The spectrum contains two…

Strongly Correlated Electrons · Physics 2009-11-07 M. B. Stone , Y. Chen , J. Rittner , H. Yardimci , D. H. Reich , C. Broholm , D. V. Ferraris , T. Lectka

Frustrated three dimensional quantum magnets are notoriously impervious to theoretical analysis. Here we use a combination of three computational methods to investigate the three dimensional pyrochlore $S=1/2$ quantum antiferromagnet, an…

Strongly Correlated Electrons · Physics 2020-08-10 Robin Schäfer , Imre Hagymási , Roderich Moessner , David J. Luitz

We report inelastic neutron scattering study of a quasi-two-dimensional S=1/2 dimer system Piperazinium Hexachlorodicuprate under hydrostatic pressure. The spin gap {\Delta} becomes softened with the increase of the hydrostatic pressure up…

Strongly Correlated Electrons · Physics 2010-12-01 Tao Hong , C. Stock , I. Cabrera , C. Broholm , Y. Qiu , J. B. Leao , S. J. Poulton , J. R. D. Copley

Neutron scattering experiment on NiS2 single crystal revealed a honeycomb pattern of the intensity distribution in reciprocal lattice space (continuous-line structure along the fcc zone boundary) providing the first direct evidence for…

Strongly Correlated Electrons · Physics 2007-05-23 M. Matsuura , Y. Endoh , H. Hiraka , K. Yamada , K. Hirota , A. S. Mishchenko , N. Nagaosa , I. V. Solovyev

We report a study of the magnetic ground state and crystal electric field (CEF) scheme in the triangular-lattice antiferromagnet NdCd$_3$P$_3$. Combined neutron scattering, magnetization, and heat capacity measurements demonstrate that the…

We report on recent results for strongly frustrated quantum $J_1$-$J_2$ antiferromagnets in dimensionality d=1,2,3 obtained by the coupled cluster method (CCM). We demonstrate that the CCM in high orders of approximation allows us to…

Strongly Correlated Electrons · Physics 2009-11-11 J. Richter , R. Darradi , R. Zinke , R. F. Bishop

Exchange interactions between $S=\frac{1}{2}$ sites in piperazinium hexachlorodicuprate produce a frustrated bilayer magnet with a singlet ground state. We have determined the field-temperature phase diagram by high field magnetization and…

Strongly Correlated Electrons · Physics 2009-11-11 M. B. Stone , C. Broholm , D. H. Reich , O. Tchernyshyov , P. Vorderwisch , N. Harrison

Frustrated magnets with a strong spin-lattice coupling can show rich magnetic phases and the associated fascinating phenomena. A promising platform is the breathing pyrochlore magnet CuInCr$_{4}$S$_{8}$ with localized $S=3/2$ Cr$^{3+}$…

We examine the $S=1/2$ Heisenberg magnet on four three-dimensional lattices - simple-cubic, diamond, pyrochlore, and hyperkagome ones - for ferromagnetic and antiferromagnetic signs of the exchange interaction in order to illustrate the…

Strongly Correlated Electrons · Physics 2025-12-30 T. Krokhmalskii , T. Hutak , O. Derzhko

The metallic compound FeP belongs to the class of materials that feature a complex noncollinear spin order driven by magnetic frustration. While its double-helix magnetic structure with a period $\lambda_{\text{s}} \approx 5c$, where $c$ is…

We report magnetization and specific heat measurements in the 2D frustrated spin-1/2 Heisenberg antiferromagnet Cs2CuCl4 at temperatures down to 0.05 K and high magnetic fields up to 11.5 T applied along a, b and c-axes. The low-field…

Strongly Correlated Electrons · Physics 2013-06-25 Y. Tokiwa , T. Radu , R. Coldea , H. Wilhelm , Z. Tylczynski , F. Steglich

Magnetic frustration in metals is scarce and hard to pinpoint, but exciting due to the possibility of the emergence of fascinating novel phases. The cubic intermetallic compound HoInCu$_4$ with all holmium atoms on an fcc lattice, exhibits…

We consider the spin-1/2 antiferromagnetic Heisenberg model on a bilayer honeycomb lattice including interlayer frustration in the presence of an external magnetic field. In the vicinity of the saturation field, we map the low-energy states…

Strongly Correlated Electrons · Physics 2017-03-22 Taras Krokhmalskii , Vasyl Baliha , Oleg Derzhko , Jörg Schulenburg , Johannes Richter

Specific heat and ac magnetic susceptibility measurements, spanning low temperatures ($T \geq 40$ mK) and high magnetic fields ($B \leq 14$ T), have been performed on a two-dimensional (2D) antiferromagnet Cu(tn)Cl$_{2}$ (tn =…

Neutron diffraction and calorimetric measurements are used to study the field-induced quantum phase transition in piperazinium-Cu$_2$(Cl$_{1-x}$Br$_x$)$_6$ ($x=0$, x=3.5% and x=7.5%), a prototypical quantum antiferromagnet with random…

Strongly Correlated Electrons · Physics 2013-07-02 D. Hüvonen , S. Zhao , M. Månsson , T. Yankova , E. Ressouche , C. Niedermayer , M. Laver , S. N. Gvasaliya , A. Zheludev

Spin wave dispersion in the frustrated fcc type-III antiferromagnet MnS$_2$ has been determined by inelastic neutron scattering using a triple-axis spectrometer. Existence of multiple spin wave branches, with significant separation between…

Strongly Correlated Electrons · Physics 2019-02-20 T. Chatterji , L. P. Regnault , S. Ghosh , A. Singh

Magnetic excitations of the quasi-1D S=1/2 Heisenberg antiferromagnet (HAF) Cs2CuCl4 have been measured as a function of magnetic field using neutron scattering. For T<0.62 K and B=0 T the weak inter-chain coupling produces 3D…

Strongly Correlated Electrons · Physics 2009-10-30 R. Coldea , D. A. Tennant , R. A. Cowley , D. F. McMorrow , B. Dorner , Z. Tylczynski
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