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We consider correlation-assisted tunnel ionization of a small molecule by an intense low-frequency laser pulse. In this mechanism, the departing electron excites the state of the ion via a Coulomb interaction. We show that the angular…

Atomic Physics · Physics 2014-04-25 Emilio Pisanty , Misha Ivanov

We analyze the communication efficiency of quantum information transfer along unmodulated spin chains by computing the communication rates of various protocols. The effects of temporal correlations are discussed, showing that they can be…

Quantum Physics · Physics 2011-11-09 Davide Rossini , Vittorio Giovannetti , Rosario Fazio

Photochromic molecular structures constitute a unique platform for constructing molecular switches, sensors and memory devices. One of their most promising applications is as light-switchable electron acceptor or donor units. Here, we…

Chemical Physics · Physics 2020-07-21 Jakub K. Sowa , Emily A. Weiss , Tamar Seideman

Vibrationally inelastic electron transport through a flexible molecular junction is investigated. The study is based on a mechanistic model for a biphenyl molecule between two metal electrodes. Employing methods from electron-molecule…

Mesoscale and Nanoscale Physics · Physics 2023-07-26 Martin Cizek , Michael Thoss , Wolfgang Domcke

We estimate rate coefficients for charge transfer between neutral hydrogen and helium and moderate to highly ionized heavy elements. Although charge transfer does not have much influence on hot collisionally ionized plasmas, its effects on…

Astrophysics · Physics 2009-10-30 G. J. Ferland , K. T. Korista , D. A. Verner , A. Dalgarno

Using molecular simulation and continuum dielectric theory, we consider how electrochemical kinetics are modulated by twist angle in bilayer graphene electrodes. By establishing a connection between twist angle and the screening length of…

Statistical Mechanics · Physics 2024-11-06 Leonardo Coello Escalante , David T. Limmer

We develop a theoretical model for how organic molecules can control the electronic and transport properties of an underlying transistor channel to whose surface they are chemically bonded. The influence arises from a combination of…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Smitha Vasudevan , Neeti Kapur , Tao He , Matthew Neurock , James M. Tour , Avik W. Ghosh

We calculate non-perturbatively the inelastic effects on the conductance through a conjugated molecular wire-metal heterojunction, including realistic electron-phonon coupling. We show that at sub-band-gap energies the current is dominated…

Materials Science · Physics 2009-10-31 H. Ness , A. J. Fisher

The description of the chemical bond between a solid surface and an atom or a molecule is the fundamental basis for understanding a broad range of scientific problems in heterogeneous catalysis, semiconductor device fabrication, and fuel…

Materials Science · Physics 2019-10-02 Liping Yu , Qimin Yan , Adrienn Ruzsinszky

The effects of different contact geometries, bond dimerization, and gate voltage on quantum transport through a C$_{60}$ molecule are studied by the Landauer-B\"{u}ttiker formula based on the Green's function technique. It is shown that the…

Mesoscale and Nanoscale Physics · Physics 2008-08-12 Alireza Saffarzadeh

Controlling the direction and magnitude of both heat and electronic currents using rectifiers has significant implications for the advancement of molecular circuit design. In order to facilitate the implementation of new transport phenomena…

Mesoscale and Nanoscale Physics · Physics 2019-08-02 Galen T. Craven , Dahai He , Abraham Nitzan

Microscopic theory of the nonradiative energy transfer in a system of III-V semiconductor quantum dots is elaborated in our work. The energy transfer both due to direct Coulomb and due to exchange interactions between two quantum dots…

Mesoscale and Nanoscale Physics · Physics 2017-11-22 O. P. Chikalova-Luzina , D. M. Samosvat , V. M. Vyatkin , G. G. Zegrya

Light-induced charge transmission through a molecular junction (molecular diode) is studied in the framework of a HOMO-LUMO model and in using a kinetic description. Expressions are presented for the sequential (hopping) and direct…

Mesoscale and Nanoscale Physics · Physics 2013-04-19 E. G. Petrov , V. O. Leonov , V. May , P. Hänggi

We present dynamics calculations showing how electron-correlation-driven charge migration occurring in the correlation band of ionized molecules can lead to a redistribution of the charge increasing the stability of the system. These…

Chemical Physics · Physics 2022-08-31 Victor Despré , Alexander I. Kuleff

It was shown that tunneling current flowing through a system with Coulomb correlations leads to charge redistribution between the different localized states. Simple model consisting of two electron levels have been analyzed by means of…

Other Condensed Matter · Physics 2012-07-02 P. I. Arseyev , N. S. Maslova , V. N. Mantsevich

Electron capture by {\it isolated} atoms and ions proceeds by photorecombination. In this process a species captures a free electron by emitting a photon which carries away the excess energy. It is shown here that in the presence of an {\it…

Quantum Physics · Physics 2010-03-18 Kirill Gokhberg , Lorenz S. Cederbaum

This work inspects the thermally activated transfer of solute particles across the interface between two interstitial solid solution phases that equilibrate internally by fast diffusion on conserved arrays of sites. When each phase is…

Materials Science · Physics 2026-01-30 Jörg Weissmüller

Based on the reduced density matrix method, we compare two different approaches to calculate the dynamics of the electron transfer in systems with donor, bridge, and acceptor. In the first approach a vibrational substructure is taken into…

Quantum Physics · Physics 2009-10-31 M. Schreiber , D. Kilin , U. Kleinekathoefer

A rate equation formalism is used to determine the effect of electron-phonon coupling on the conductance of a molecule. Interplay between the phonon-induced renormalization of the density of states on the quantum dot and the phonon-induced…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 A. Mitra , I. Aleiner , A. J. Millis

We consider exciton effects on current in molecular nanojunctions, using a model comprising a two two-level sites bridge connecting free electron reservoirs. Expanding the density operator in the many-electron eigenstates of the uncoupled…

Strongly Correlated Electrons · Physics 2015-05-14 GuangQi Li , Boris D. Fainberg , Abraham Nitzan , Sigmund Kohler , Peter Hänggi