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The effective electrostatic interaction between a pair of colloids, both of them located close to each other at an electrolyte interface, is studied by employing the full, nonlinear Poisson-Boltzmann (PB) theory within classical density…

Soft Condensed Matter · Physics 2016-08-17 Arghya Majee , Markus Bier , S. Dietrich

We study the melting behavior of charged colloidal crystals, using a simulation technique that combines a continuous mean-field Poisson-Boltzmann description for the microscopic electrolyte ions with a Brownian-dynamics simulation for the…

Soft Condensed Matter · Physics 2009-11-13 J. Dobnikar , Y. Chen , R. Rzehak , H. H. von Grünberg

A model system of highly asymmetric polyelectrolyte with directional short-range attractive interactions was studied by canonical Monte Carlo computer simulations. Comparison of MC data with previously published theoretical results shows…

Soft Condensed Matter · Physics 2021-10-12 J. Rescic

The Landau-de Gennes free energy is used to study theoretically the interaction of parallel cylindrical colloidal particles trapped at a nematic-isotropic interface. We find that the effective interaction potential is non-monotonic. The…

Soft Condensed Matter · Physics 2015-06-24 D. Andrienko , M. Tasinkevych , S. Dietrich

The effect of fixed discrete colloidal charges in the primitive model is investigated for spherical macroions. Instead of considering a central bare charge, as it is traditionally done, we distribute \textit{discrete} charges randomly on…

Soft Condensed Matter · Physics 2009-10-31 Rene Messina , Christian Holm , Kurt Kremer

Our interest goes to the different virial contributions to the equation of state of charged colloidal suspensions. Neglect of surface effects in the computation of the colloidal virial term leads to spurious and paradoxical results. This…

Soft Condensed Matter · Physics 2009-11-13 E. Trizac , L. Belloni , J. Dobnikar , H. H. von Grunberg , R. Castaneda-Priego

We study the combined effects of electrostatic and hydrodynamic interactions (HI) on the short-time dynamics of charge-stabilized colloidal spheres. For this purpose, we calculate the translational and the rotational self-diffusion…

Soft Condensed Matter · Physics 2008-02-03 M. Watzlawek , G. Naegele

Molecular dynamics (MD) simulations are used to determine the diffusion coefficients, electrophoretic mobilities and electrical conductivity of a charged colloidal suspension in the salt-free regime as a function of the colloid charge. The…

Soft Condensed Matter · Physics 2010-12-16 Sorin Bastea

We analyze theoretically the electrostatic interaction of surface-charged colloids at water interfaces with special attention to the experimentally relevant case of large charge densities on the colloid-water interface. Whereas linear…

Soft Condensed Matter · Physics 2007-11-13 D. Frydel , S. Dietrich , M. Oettel

We are interested in rationalizing the phenomenon of like-charge attraction between charged bodies, such as a pair of colloids, in the strong coupling regime. The two colloids are modelled as uniformly charged parallel plates, neutralized…

Soft Condensed Matter · Physics 2025-01-13 L. Samaj , E. Trizac , M. Trulsson

Sedimentation-diffusion equilibrium density profiles of suspensions of charge-stabilized colloids are calculated theoretically and by Monte Carlo simulation, both for a one-component model of colloidal particles interacting through pairwise…

Soft Condensed Matter · Physics 2013-05-29 Aldemar Torres , Alejandro Cuetos , Marjolein Dijkstra , Rene van Roij

We consider the interactions between two uncharged planar macroscopic surfaces immersed in an electrolyte solution which are induced by interfacial selectivity. These forces are taken into account by introducing a depletion free-energy…

Soft Condensed Matter · Physics 2009-10-31 M. N. Tamashiro , P. Pincus

A density functional theory for a macroion suspension is examined, where the excess free energy corresponds to the macroion self energy arising from the polarisation of the supporting electrolyte solution. This is treated within a…

Soft Condensed Matter · Physics 2007-05-23 Patrick B. Warren

The addition of co-solutes to colloidal suspensions is often employed to induce tunable depletion interactions. In this work we investigate effective colloidal interactions arising from binary co-solute mixtures of hard spheres and patchy…

Soft Condensed Matter · Physics 2021-08-25 Philip H. Handle , Emanuela Zaccarelli , Nicoletta Gnan

We study the interaction between two charge regulating spherical macroions with dielectric interior and dissociable surface groups immersed in a monovalent electrolyte solution. The charge dissociation is modelled via the…

Soft Condensed Matter · Physics 2023-12-11 Hu Ruixuan , Arghya Majee , Jure Dobnikar , Rudolf Podgornik

The screened Coulomb interaction between a pair of infinite parallel planes with spatially varying surface charge is considered in the limit of small electrical potentials for arbitrary Debye lengths. A simple expression for the disjoining…

Classical Physics · Physics 2017-04-12 Sandip Ghosal , John D. Sherwood

Since the early observation of nematic phases of disc-like clay colloids by Langmuir in 1938, the phase behaviour of such systems has resisted theoretical understanding. The main reason is that there is no satisfactory generalization for…

Soft Condensed Matter · Physics 2009-11-07 E. Trizac , L. Bocquet , R. Agra , J-J. Weis , M. Aubouy

Active matter exhibits striking behaviour reminiscent of living matter and molecular fluids, and has promising applications in drug delivery or mixing at the micron scale. Active colloidal systems provide important models with simple and…

Soft Condensed Matter · Physics 2020-10-09 Nariaki Sakaï , C. Patrick Royall

Surface effects are generally prevailing in confined colloidal systems. Here we report on dispersed nanoparticles close to a fluid membrane. Exact results regarding the static organization are derived for a dilute solution of non-adhesive…

Statistical Mechanics · Physics 2009-11-10 Thomas Bickel , Mabrouk Benhamou , Hamid Kaidi

Thermoresponsive microgels find widespread use as colloidal model systems, because their temperature-dependent size allows facile tuning of their volume fraction "in situ". However, an interaction potential unifying their behavior across…

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