Related papers: Escape-Rate Crossover between Quantum and Classica…
Quantum-classical escape rate transition has been studied for uniaxial antiferromagnetic particles with an arbitrarily directed magnetic field. In the case that the transverse and longitudinal fileds coexist, we calculate the phase boundary…
We have found a novel feature of the bistable large-spin model described by the Hamiltonian H = -DS_z^2 - H_xS_x.The crossover from thermal to quantum regime for the escape rate can be either first (H_x<SD/2) or second (SD/2<H_x<2SD) order,…
We study the model of a biaxial single ferromagnetic spin Hamiltonian with an external magnetic field applied along the medium axis. The phase transition of the escape rate is investigated. Two different but equivalent methods are…
We investigate the escape rate of the biaxial nanospin particle with a magnetic field applied along the easy axis. The model studied here is described by the Hamiltonian ${\cal H} = -AS_z^2 - BS_x^2 - HS_z, (A>B>0)$. By reducing this…
Employing the method of mapping the spin problem onto a particle one, we have derived the particle Hamiltonian for a biaxial spin system with a transverse or longitudinal magnetic field. Using the Hamiltonian and introducing the parameter…
We investigate the escape rate of a biaxial spin particle with an arbitrarily dierected magnetic field in the easy plane, described by Hamiltonian ${\cal H} = -AS_z^2 - BS_x^2 -H_x S_x -H_z S_z, (A>B>0)$. We derive an effective particle…
Quantum-classical escape-rate transition has been studied for two general forms of magnetic anisotropy in ferrimagnetic or antiferromagnetic particles. It is found that the range of the first-order transition is greatly reduced as the…
We have investigated the escape rate of the nanospin particle with a magnetic field applied along the easy axis. The model studied here is described by the Hamiltonian $\hat{\cal H} = K_1 \hat{S}_z^2 + K_2 \hat{S}_y^2 + g\mu_b H \hat{S}_x…
The escape rate \Gamma of the large-spin model described by the Hamiltonian H = -DS_z^2 - H_zS_z - H_xS_x is investigated with the help of the mapping onto a particle moving in a double-well potential U(x). The transition-state method…
The quantum-classical transitions of the escape rates in a uniaxial spin model relevant to the molecular magnet Mn$_{12}$Ac and a biaxial anisotropic ferromagnetic particle are investigated by applying the periodic instanton method. The…
This article presents a review on the theoretical and the experimental developments on macroscopic quantum tunneling and phase transition of the escape rate in spin systems. We present the basic ideas with simplified calculations so that it…
We study the motion of a particle in a particular magnetic field configuration both classically and quantum mechanically. For flux-free radially symmetric magnetic fields defined on circular regions, we establish that particle escape speeds…
The quantum-classical transition of the escape rate of the spin model \cal H= -DS_z^2 - H_zS_z + B S_x^2 is investigated by a perturbative approach with respect to B [D. A. Garanin, J. Phys A {\bf 24}, L61 (1991)]. The transition is first…
The escape rates of the biaxial single domain spin particles with and without an applied magnetic field are investigated. Using the strict potential field description of spin systems developed by Ulyanov and Zaslavskii we obtain new…
In a coupled system of one classical and one quantum mechanical degree of freedom, the quantum degree of freedom can facilitate the escape of the whole system. Such unusual escape characteristics have been theoretically predicted as…
We study the phase transition of the escape rate of exchange-coupled dimer of single-molecule magnets which are coupled either ferromagnetic ally or antiferromagnetically in a staggered magnetic field and an easy $z$-axis anisotropy. The…
Classical escape rates of uniaxial spin systems are characterized by a prefactor differing from and much smaller than that of the particle problem, since the maximum of the spin energy is attained everywhere on the line of constant…
The decay of metastable states is dominated by quantum tunneling at low temperatures and by thermal activation at high temperatures. The escape rate of a particle out of a square well is calculated within a semi-classical approximation and…
Quantum nanomagnets can show a field dependence of the relaxation time very different from their classical counterparts, due to resonant tunneling via excited states (near the anisotropy barrier top). The relaxation time then shows minima…
We study quantum-classical escape-rate transitions for uniaxial and biaxial models with finite spins S=10 (such as Mn_12Ac and Fe_8) and S=100 by a direct numerical approach. At second-order transitions the level making a dominant…